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Register a new userVectorial light-matter interaction -- exploring spatially structured complex light fields
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Added by
Sonja Franke-Arnold
Publication date
2020
fields
Physics
and research's language is
English
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Research on spatially-structured light has seen an explosion in activity over the past decades, powered by technological advances for generating such light, and driven by questions of fundamental science as well as engineering applications. In this review we highlight work on the interaction of vector light fields with atoms, and matter in general. This vibrant research area explores the full potential of light, with clear benefits for classical as well as quantum applications.
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Optical aberrations have been studied for centuries, placing fundamental limits on the achievable resolution in focusing and imaging. In the context of structured light, the spatial pattern is distorted in amplitude and phase, often arising from optical imperfections, element misalignment, or even from dynamic processes due to propagation through perturbing media such as living tissue, free-space, underwater and optical fibre. Here we show that the polarisation inhomogeneity that defines vectorial structured light is immune to all such perturbations, provided they are unitary. By way of example, we study the robustness of vector vortex beams to tilted lenses and atmospheric turbulence, both highly asymmetric aberrations, demonstrating that the inhomogeneous nature of the polarisation remains unaltered from the near-field to far-field, even as the structure itself changes. The unitary nature of the channel allows us to undo this change through a simple lossless operation, tailoring light that appears robust in all its spatial structure regardless of the medium. Our insight highlights the overlooked role of measurement in describing classical vectorial light fields, in doing so resolving prior contradictory reports on the robustness of vector beams in complex media. This paves the way to the versatile application of vectorial structured light, even through non-ideal optical systems, crucial in applications such as imaging deep into tissue and optical communication across noisy channels.
The study of light propagation has been a cornerstone of progress in physics and technology. Recently, advances in control and shaping of light have created significant interest in the propagation of complex structures of light -- particularly under realistic terrestrial conditions. While theoretical understanding of this research question has significantly grown over the last two decades, outdoor-experiments with complex light structures are rare, and comparisons with theory have been nearly lacking. Such situations show a significant gap between theoretical models of atmospheric light behaviour and current experimental effort. Here, in an attempt to reduce this gap, we describe an interesting result of atmospheric models which are feasible for empirical observation. We analyze in detail light propagation in different spatial bases and present results of the theory that the influence of atmospheric turbulence is basis-dependent. Concretely, light propagating as eigenstate in one complete basis is stronger influenced by atmosphere than light propagating in a different, complete basis. We obtain these results by exploiting a family of the continuously adjustable, complete basis of spatial modes -- the Ince-Gauss modes. Our concrete numerical results will hopefully inspire experimental efforts and bring the theoretical and empirical study of complex light patterns in realistic scenarios closer together.
The structural versatility of light underpins an outstanding collection of optical phenomena where both geometrical and topological states of light can dictate how matter will respond or display. Light possesses multiple degrees of freedom such as amplitude, and linear, spin angular, and orbital angular momenta, but the ability to adaptively engineer the spatio-temporal distribution of all these characteristics is primarily curtailed by technologies used to impose any desired structure to light. We describe a foundational demonstration that examines a laser architecture offering integrated spatio-temporal field control and programmability, thereby presenting unique opportunities for generating light by design to exploit its topology.
Coherent light-matter interactions have recently extended their applications to the ultrafast control of magnetization in solids. An important but unrealized technique is the manipulation of magnetization vector motion to make it follow an arbitrarily designed multi-dimensional trajectory. Furthermore, for its realization, the phase and amplitude of degenerate modes need to be steered independently. A promising method is to employ Raman-type nonlinear optical processes induced by femtosecond laser pulses, where magnetic oscillations are induced impulsively with a controlled initial phase and an azimuthal angle that follows well defined selection rules determined by the materials symmetries. Here, we emphasize the fact that temporal variation of the polarization angle of the laser pulses enables us to distinguish between the two degenerate modes. A full manipulation of two-dimensional magnetic oscillations is demonstrated in antiferromagnetic NiO by employing a pair of polarization-twisted optical pulses. These results have lead to a new concept of vectorial control of magnetization by light.
We propose the concept of helicity maximization applicable to structured light and obtain a universal rela-tion for the maximum of helicity density at a given field energy density. We further demonstrate that us-ing structured light with maximized helicity density eliminates the need of the specific knowledge of en-ergy and helicity densities in determining the chirality of a nanoparticle. The helicity maximization con-cept generalizes the use of the dissymmetry factor in chirality detection to any chiral structure light il-luminating nanoparticles.
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