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Register a new userAnomalous spectral weight transfer in the nematic state of iron-selenide superconductor
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Nematic phase intertwines closely with high-Tc superconductivity in iron-based superconductors. Its mechanism, which is closely related to the pairing mechanism of superconductivity, still remains controversial. Comprehensive characterization of how the electronic state reconstructs in the nematic phase is thus crucial. However, most experiments focus only on the reconstruction of band dispersions. Another important characteristic of electronic state, the spectral weight, has not been studied in details so far. Here, we studied the spectral weight transfer in the nematic phase of FeSe$_{0.9}$S$_{0.1}$ using angle-resolved photoemission spectroscopy and in-situ detwinning technique. There are two elliptical electron pockets overlapping with each other orthogonally at the Brillouin zone corner. We found that, upon cooling, one electron pocket loses spectral weight and fades away, while the other electron pocket gains spectral weight and becomes pronounced. Our results show that the symmetry breaking of electronic state is manifested by not only the anisotropic band dispersion but also the band-selective modulation of spectral weight. Our observation completes our understanding of the nematic electronic state, and put strong constraints on the theoretical models. It further provide crucial clues to understand the gap anisotropy and orbital-selective pairing in iron-selenide superconductors.
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Alkali-doped iron selenide is the latest member of high Tc superconductor family, and its peculiar characters have immediately attracted extensive attention. We prepared high-quality potassium-doped iron selenide (KxFe2-ySe2) thin films by molecular beam epitaxy and unambiguously demonstrated the existence of phase separation, which is currently under debate, in this material using scanning tunneling microscopy and spectroscopy. The stoichiometric superconducting phase KFe2Se2 contains no iron vacancies, while the insulating phase has a surd5timessurd5 vacancy order. The iron vacancies are shown always destructive to superconductivity in KFe2Se2. Our study on the subgap bound states induced by the iron vacancies further reveals a magnetically-related bipartite order in the superconducting phase. These findings not only solve the existing controversies in the atomic and electronic structures in KxFe2-ySe2, but also provide valuable information on understanding the superconductivity and its interplay with magnetism in iron-based superconductors.
The role of electron-phonon interactions in iron-based superconductor is currently under debate with conflicting experimental reports on the isotope effect. To address this important issue, we employ the renormalization-group method to investigate the competition between electron-electron and electron-phonon interactions in these materials. The renormalization-group analysis shows that the ground state is a phonon-dressed unconventional superconductor: the dominant electronic interactions account for pairing mechanism while electron-phonon interactions are subdominant. Because of the phonon dressing, the isotope effect of the critical temperature can be normal or reversed, depending on whether the retarded intra- or inter-band interactions are altered upon isotope substitutions. The connection between the anomalous isotope effect and the unconventional pairing symmetry is discussed at the end.
High-quality K(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals have been grown by using KAs flux method. Instead of increasing the superconducting transition temperature $T_{rm c}$ through electron doping, we find that Co impurities rapidly suppress $T_{rm c}$ down to zero at only $x approx$ 0.04. Such an effective suppression of $T_{rm c}$ by impurities is quite different from that observed in Ba$_{0.5}$K$_{0.5}$Fe$_2$As$_2$ with multiple nodeless superconducting gaps. Thermal conductivity measurements in zero field show that the residual linear term $kappa_0/T$ only change slightly with $3.4%$ Co doping, despite the sharp increase of scattering rate. The implications of these anomalous impurity effects are discussed.
We present the first infrared and optical study in the normal state of ab-plane oriented single crystals of the iron-oxypnictide superconductor LaFePO. We find that this material is a low carrier density metal with a moderate level of correlations and exhibits signatures of electron-boson coupling. The data is consistent with the presence of coherent quasiparticles in LaFePO.
Using a variational Monte Carlo method, we investigate the nematic state in iron-base superconductors based on a three-band Hubbard model. Our results demonstrate that the nematic state, formed by introducing an anisotropic hopping order into the projected wave function, can arise in the underdoped regime when a realistic off-site Coulomb interaction $V$ is considered. {color {red} We demonstrate that the off-site Coulomb interaction $V$, which is neglected so far in the analysis of iron-base superconductors, make a dominant contribution to the stabilization of nematic state. We calculate the doping dependencies of the anisotropic properties such as the unequal occupation of $d_{xz}$ and $d_{yz}$ orbitals, anisotropies of kinetic energy and spin correlations, and show that they are all suppressed upon electron doping, which are consistent with the intrinsic anisotropies observed by optical spectrum measurement and ARPES experiments.
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