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Charged-particle branching ratios above the neutron threshold in $^{19}$F: constraining $^{15}$N production in core-collapse supernovae

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 Added by Philip Adsley
 Publication date 2020
  fields Physics
and research's language is English




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Spatially-correlated overabundances of $^{15}$N and $^{18}$O observed in some low-density graphite meteoritic grains have been connected to nucleosynthesis taking place in the helium-burning shell during core-collapse supernovae. Two of the reactions which have been identified as important to the final abundances of $^{15}$N and $^{18}$O are $^{18}$F($n,alpha$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O. The relative strengths of the $^{18}$F($n,alpha$)$^{15}$N and $^{18}$F($n,p$)$^{18}$O reactions depend on the relative $alpha_0$ and $p_0$ decays from states above the neutron threshold in $^{19}$F in addition to other properties. Experimental data on the charged-particle decays from these highly excited states are lacking or inconsistent. Two experiments were performed using proton inelastic scattering from LiF targets and magnetic spectrographs. The first experiment used the high-resolution Q3D spectrograph at Munich to constrain properties of levels in $^{19}$F. A second experiment using the Orsay Split-Pole spectrograph and an array of silicon detectors was performed in order to measure the charged-particle decays of neutron-unbound levels in $^{19}$F. A number of levels in $^{19}$F have been identified along with their corresponding charged-particle decays. The first state above the neutron threshold which has an observed proton-decay branch to the ground state of $^{18}$O lies 68 keV above the neutron threshold while the $alpha$-particle decays from the neutron-unbound levels are generally observed to be much stronger than the proton decays. Neutron-unbound levels in $^{19}$F are observed to decay predominantly by $alpha$-particle emission, supporting the role of $^{18}$F($n,alpha$)$^{15}$N in the production of $^{15}$N in the helium-burning shell of supernovae. Improved resonant-scattering reaction data are required in order to be able to determine the reaction rates accurately.



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Classical novae result from thermonuclear explosions producing several $gamma$-ray emitters which are prime targets for satellites observing in the MeV range. The early 511 keV gamma-ray emission depends critically on the $^{18}$F(p,$alpha$)$^{15}$O reaction rate which, despite many experimental and theoretical efforts, still remains uncertain. One of the main uncertainties in the $^{18}$F(p,$alpha$)$^{15}$O reaction rate is the contribution in the Gamow window of interference between sub-threshold $^{19}$Ne states and known broad states at higher energies. Therefore the goal of this work is to clarify the existence and the nature of these sub-threshold states. States in the $^{19}$Ne compound nucleus were studied at the Tandem-ALTO facility using the $^{19}$F($^3$He,t)$^{19}$Ne charge exchange reaction. Tritons were detected with an Enge Split-pole spectrometer while decaying protons or $alpha$-particles from unbound $^{19}$Ne states were collected, in coincidence, with a double-sided silicon strip detector array. Angular correlations were extracted and constraints on the spin and parity of decaying states established. The coincidence yield at $E_x$ = 6.29 MeV was observed to be high spin, supporting the conclusion that it is indeed a doublet consisting of high spin and low spin components. Evidence for a broad, low spin state was observed around 6 MeV. Branching ratios were extracted for several states above the proton threshold and were found to be consistent with the literature. R-matrix calculations show the relative contribution of sub-threshold states to the astrophysically important energy region above the proton threshold. The levels schemes of $^{19}$Ne and $^{19}$F are still not sufficiently well known and further studies of the analogue assignments are needed. The tentative broad state at 6 MeV may only play a role if the reduced proton width is large.
There is currently a severe discrepancy between theoretical models of dust formation in core-collapse supernovae (CCSNe), which predict $gtrsim 0.01$ M$_odot$ of ejecta dust forming within $sim 1000$ days, and observations at these epochs, which infer much lower masses. We demonstrate that, in the optically thin case, these low dust masses are robust despite significant observational and model uncertainties. For a sample of 11 well-observed CCSNe, no plausible model reaches carbon dust masses above $10^{-4}$ M$_odot$, or silicate masses above $sim 10^{-3}$ M$_odot$. Optically thick models can accommodate larger dust masses, but the dust must be clumped and have a low ($<0.1$) covering fraction to avoid conflict with data at optical wavelengths. These values are insufficient to reproduce the observed infrared fluxes, and the required covering fraction varies not only between SNe but between epochs for the same object. The difficulty in reconciling large dust masses with early-time observations of CCSNe, combined with well-established detections of comparably large dust masses in supernova remnants, suggests that a mechanism for late-time dust formation is necessary.
Neutron-capture reactions on $^{18}$F in the helium-burning shell play an important role in the production of $^{15}$N during core-collapse supernovae. The competition between the $^{18}$F($n,p/alpha$)$^{18}$O/$^{15}$N reactions controls the amount of $^{15}$N produced. The strengths of these reactions depend on the decay branching ratios of states in $^{19}$F above the neutron threshold. We report on an experiment investigating the decay branching ratios of these states in order to better constrain the strengths of the reactions.
147 - F. De Grancey 2016
Intense and purified radioactive beam of post-accelerated $^{14}$O was used to study the low-lying states in the unbound $^{15}$F nucleus. Exploiting resonant elastic scattering in inverse kinematics with a thick target, the second excited state, a resonance at E$_R$=4.757(6)(10)~MeV with a width of $Gamma$=36(5)(14)~keV was measured for the first time with high precision. The structure of this narrow above-barrier state in a nucleus located two neutrons beyond the proton drip line was investigated using the Gamow Shell Model in the coupled channel representation with a $^{12}$C core and three valence protons. It is found that it is an almost pure wave function of two quasi-bound protons in the $2s_{1/2}$ shell.
The astrophysical site of the r-process is still uncertain, and a full exploration of the systematics of this process in terms of its dependence on nuclear properties from stability to the neutron drip-line within realistic stellar environments has still to be undertaken. Sufficiently high neutron to seed ratios can only be obtained either in very neutron-rich low-entropy environments or moderately neutron-rich high-entropy environments, related to neutron star mergers (or jets of neutron star matter) and the high-entropy wind of core-collapse supernova explosions. As chemical evolution models seem to disfavor neutron star mergers, we focus here on high-entropy environments characterized by entropy $S$, electron abundance $Y_e$ and expansion velocity $V_{exp}$. We investigate the termination point of charged-particle reactions, and we define a maximum entropy $S_{final}$ for a given $V_{exp}$ and $Y_e$, beyond which the seed production of heavy elements fails due to the very small matter density. We then investigate whether an r-process subsequent to the charged-particle freeze-out can in principle be understood on the basis of the classical approach, which assumes a chemical equilibrium between neutron captures and photodisintegrations, possibly followed by a $beta$-flow equilibrium. In particular, we illustrate how long such a chemical equilibrium approximation holds, how the freeze-out from such conditions affects the abundance pattern, and which role the late capture of neutrons originating from $beta$-delayed neutron emission can play.
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