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Control of spontaneous emission dynamics in microcavities with chiral exceptional surfaces

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 Added by Qi Zhong
 Publication date 2020
  fields Physics
and research's language is English




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We investigate spontaneous emission from a quantum emitter located within the mode volume of a microring resonator that features chiral exceptional points. We show that this configuration offers enough degrees of freedom to exhibit a full control to either enhance or suppress the emission process. Particularly, we demonstrate that the Purcell factor can be enhanced by a factor of two beyond its value in an identical microring operating at a diabolic point. Our conclusions, which are derived using a non-Hermitian Hamiltonian formalism, are confirmed by employing full-wave simulations of realistic photonic structures and materials. Our results offer a straightforward route to improve the performance of single photon sources using current photonics technology without the need for building optical resonators with ultrahigh quality factors or nanoscale volumes.



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Engineering the transport of radiation and its interaction with matter using non-Hermiticity, particularly through spectral degeneracies known as exceptional points(EPs), is an emerging field that has both fundamental and practical implications. Chiral behavior in the vicinity of EPs opens new opportunities in radiation control, such as unidirectional reflection or lasing with potential applications in areas ranging from cavity quantum electrodynamics and spectral filtering to sensing and thermal imaging. However, tuning and stabilizing a system to a discrete EP in parameter space is a challenging task: either the system is operated close to an EP rather than directly at the EP or the true power of EP is obscured by stability issues. Here, we circumvent this challenge by designing a photonic system that operates on a surface of exceptional points, known as an exceptional surface (ES). We achieve this by using a waveguide-coupled optical resonator with an external feedback loop that induces a nonreciprocal coupling between its frequency degenerate clockwise (CW) and counterclockwise (CCW) traveling modes. By operating the system at critical coupling on the ES, we demonstrate, for the first time, the effect of chiral and degenerate coherent perfect absorption (CPA) where input waves in only one direction are perfectly absorbed. This novel type of CPA-EP is revealed through the observation of the predicted and long-sought squared Lorentzian absorption lineshapes. We expect our results and approach to serve as a bridge between non-Hermitian physics and other fields that rely on radiation engineering.
Planar microcavities allow the control and manipulation of spin-polarization, manifested in phenomena like the optical spin Hall effect due to the intrinsic polarization mode splitting. Here, we study a transparent microcavity with broken rotational symmetry, realized by aligning the optical axis of a uniaxial cavity material in the cavity plane. We demonstrate that the in-plane optical anisotropy gives rise to exceptional points in the dispersion relation, which occur pair-wise, are circularly polarized, and are cores of polarization vortices. These exceptional points are a result of the non-Hermitian character of the system, and are in close relationship to singular optical axes in absorptive biaxial systems.
89 - J. Zou , H. Zhou , C. Jiang 2021
Chaos in semiconductor lasers or other optical systems have been intensively studied in past two decades. However, the route from period doubling to chaos is still not sufficiently visible, in particular, in gain-modulated semiconductor lasers. In this article we perform a careful investigation of the route to chaos exhibited by directly modulated semiconductor lasers near the threshold region with various values of modulation frequency and amplitude. Gain nonlinearity is included in the simulation of pulse train generation through gain switching, and a new form of phase space representation is introduced to distinctly display period doubling, tripling, quadrupling and chaos. The irregular behaviour is examined at various modulation frequencies and amplitudes, highlighting the possible route to chaos for very large amplitude modulation in the near-threshold region. The existence of deterministic trajectories below the laser threshold is rendered possible by the presence of the (average component of the) spontaneous emission, a point which has not often been explicitly considered. Furthermore, we report on the existence of a transition between similar attractors characterized by a temporal transient which depends on the amplitude of the modulation driving the pump.
Exceptional points in non-Hermitian systems have recently been shown to possess nontrivial topological properties, and to give rise to many exotic physical phenomena. However, most studies thus far have focused on isolated exceptional points or one-dimensional lines of exceptional points. Here, we substantially expand the space of exceptional systems by designing two-dimensional surfaces of exceptional points, and find that symmetries are a key element to protect such exceptional surfaces. We construct them using symmetry-preserving non-Hermitian deformations of topological nodal lines, and analyze the associated symmetry, topology, and physical consequences. As a potential realization, we simulate a parity-time-symmetric 3D photonic crystal and indeed find the emergence of exceptional surfaces. Our work paves the way for future explorations of systems of exceptional points in higher dimensions.
Sub-wavelength nanostructured systems with tunable electromagnetic properties, such as hyperbolic metamaterials (HMMs), provide a useful platform to tailor spontaneous emission processes. Here, we investigate a system comprising $Eu^{ 3+}(NO_{3})_{3}6H_{2}O$ nanocrystals on an HMM structure featuring a hexagonal array of Ag-nanowires in a porous $Al_{2}O_{3}$ matrix. The HMM-coupled $Eu^{ 3+}$ ions exhibit up to a 2.4-fold increase of their decay rate, accompanied by an enhancement of the emission rate of the $^{ 5}D_{0}rightarrow$ $^{ 7}F_{2}$ transition. Using finite-difference time-domain modeling, we corroborate these observations with the increase in the photonic density of states seen by the $Eu^{ 3+}$ ions in the proximity of the HMM. Our results indicate HMMs can serve as a valuable tool to control the emission from weak transitions, and hence hint at a route towards more practical applications of rare-earth ions in nanoscale optoelectronics and quantum devices.
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