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Register a new userPore-Scale Transport and Two-Phase Fluid Structures in Fibrous Porous Layers: Application to Fuel Cells and Beyond
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Meisam Farzaneh
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We present pore-scale simulations of two-phase flows in a reconstructed fibrous porous layer. The three dimensional microstructure of the material, a fuel cell gas diffusion layer, is acquired via X-ray computed tomography and used as input for lattice Boltzmann simulations. We perform a quantitative analysis of the multiphase pore-scale dynamics and we identify the dominant fluid structures governing mass transport. The results show the existence of three different regimes of transport: a fast inertial dynamics at short times, characterised by a compact uniform front, a viscous-capillary regime at intermediate times, where liquid is transported along a gradually increasing number of preferential flow paths of the size of one-two pores, and a third regime at longer times, where liquid, after having reached the outlet, is exclusively flowing along such flow paths and the two-phase fluid structures are stabilised. We observe that the fibrous layer presents significant variations in its microscopic morphology, which have an important effect on the pore invasion dynamics, and counteract the stabilising viscous force. Liquid transport is indeed affected by the presence of microstructure-induced capillary pressures acting adversely to the flow, leading to capillary fingering transport mechanism and unstable front displacement, even in the absence of hydrophobic treatments of the porous material. We propose a macroscopic model based on an effective contact angle that mimics the effects of the such a dynamic capillary pressure. Finally, we underline the significance of the results for the optimal design of face masks in an effort to mitigate the current COVID-19 pandemic.
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We study the transport of inertial particles in water flow in porous media. Our interest lies in understanding the accumulation of particles including the possibility of clogging. We propose that accumulation can be a result of hydrodynamic effects: the tortuous paths of the porous medium generate regions of dominating strain/vorticity, which favour the accumulation/dispersion of the inertial particles. Numerical simulations show that essentially two accumulation regimes are identified: for low and for high flow velocities. When particles accumulate in high-velocity regions, at the entrance of a pore throat, a clog is formed. The formation of a clog significantly modifies the flow, as the partial blockage of the pore causes a local redistribution of pressure. This redistribution can divert the upstream water flow into neighbouring pores. Moreover, we show that accumulation in high velocity regions occurs in heterogeneous media, but not in homogeneous media, where we refer to homogeneity with respect to the distribution of the pore throat diameters.
We consider transport in a fluid flow of arbitrary complexity but with a dominant flow direction. This is the situation encountered, for example, when analyzing the dynamics of sufficiently small particles immersed in a turbulent fluid and vertically sinking because of their weight. We develop a formalism characterizing the dynamics of particles released from one layer of fluid and arriving in a second one after traveling along the dominant direction. The main ingredient in our study is the definition of a two-layer map that describes the Lagrangian transport between both layers. We combine geometric approaches and probabilistic network descriptions to analyze the two-layer map. From the geometric point of view, we express the properties of lines, surfaces and densities transported by the flow in terms of singular values related to Lyapunov exponents, and define a new quantifier, the Finite Depth Lyapunov Exponent. Within the network approach, degrees and an entropy are introduced to characterize transport. We also provide relationships between both methodologies. The formalism is illustrated with numerical results for a modification of the ABC flow, a model commonly studied to characterize three-dimensional chaotic advection.
Natural convection in porous media is a fundamental process for the long-term storage of CO2 in deep saline aquifers. Typically, details of mass transfer in porous media are inferred from the numerical solution of the volume-averaged Darcy-Oberbeck-Boussinesq (DOB) equations, even though these equations do not account for the microscopic properties of a porous medium. According to the DOB equations, natural convection in a porous medium is uniquely determined by the Rayleigh number. However, in contrast with experiments, DOB simulations yield a linear scaling of the Sherwood number with the Rayleigh number (Ra) for high values of Ra (Ra>>1,300). Here, we perform Direct Numerical Simulations (DNS), fully resolving the flow field within the pores. We show that the boundary layer thickness is determined by the pore size instead of the Rayleigh number, as previously assumed. The mega- and proto- plume sizes increase with the pore size. Our DNS results exhibit a nonlinear scaling of the Sherwood number at high porosity, and for the same Rayleigh number, higher Sherwood numbers are predicted by DNS at lower porosities. It can be concluded that the scaling of the Sherwood number depends on the porosity and the pore-scale parameters, which is consistent with experimental studies.
In this paper, a numerical study on the melting behavior of phase change material (PCM) with gradient porous media has been carried out at the pore scales. In order to solve the governing equations, a pore-scale lattice Boltzmann method with the double distribution functions is used, in which a volumetric LB scheme is employed to handle the boundary. The Monte Carlo random sampling is adopted to generate a microstructure of two-dimensional gradient foam metal which are then used to simulate the solid-liquid phase transition in the cavity. The effect of several factors, such as gradient porosity structure, gradient direction, Rayleigh number and particle diameters on the liquid fraction of PCM are systematically investigated. It is observed that the presence of gradient media affect significantly the melting rate and shortens full melting time compared to that for constant porosity by enhancing natural convection. The melting time of positive and negative gradients will change with Rayleigh number, and there is a critical value for Rayleigh number. Specifically, when Rayleigh number is below the critical value, the positive gradient is more advantageous, and when Rayleigh number exceeds the critical value, the negative gradient is more advantageous. Moreover, smaller particle diameters would lead to lower permeability and larger internal surfaces for heat transfer.
Imbibition, the displacement of a nonwetting fluid by a wetting fluid, plays a central role in diverse energy, environmental, and industrial processes. While this process is typically studied in homogeneous porous media with uniform permeabilities, in many cases, the media have multiple parallel strata of different permeabilities. How such stratification impacts the fluid dynamics of imbibition, as well as the fluid saturation after the wetting fluid breaks through to the end of a given medium, is poorly understood. We address this gap in knowledge by developing an analytical model of imbibition in a porous medium with two parallel strata, combined with a pore network model that explicitly describes fluid crossflow between the strata. By numerically solving these models, we examine the fluid dynamics and fluid saturation left after breakthrough. We find that the breakthrough saturation of nonwetting fluid is minimized when the imposed capillary number Ca is tuned to a value Ca$^*$ that depends on both the structure of the medium and the viscosity ratio between the two fluids. Our results thus provide quantitative guidelines for predicting and controlling flow in stratified porous media, with implications for water remediation, oil/gas recovery, and applications requiring moisture management in diverse materials.
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