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Register a new userConfined nano-NMR spectroscopy using NV centers
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Nano-NMR spectroscopy with nitrogen-vacancy centers holds the potential to provide high resolution spectra of minute samples. This is likely to have important implications for chemistry, medicine and pharmaceutical engineering. One of the main hurdles facing the technology is that diffusion of unpolarized liquid samples broadens the spectral lines thus limiting resolution. Experiments in the field are therefore impeded by the efforts involved in achieving high polarization of the sample which is a challenging endeavor. Here we examine a scenario where the liquid is confined to a small volume. We show that the confinement counteracts the effect of diffusion, thus overcoming a major obstacle to the resolving abilities of the NV-NMR spectrometer.
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Over the years, an enormous effort has been made to establish nitrogen vacancy (NV) centers in diamond as easily accessible and precise magnetic field sensors. However, most of their sensing protocols rely on the application of bias magnetic fields, preventing their usage in zero- or low-field experiments. We overcome this limitation by exploiting the full spin $S=1$ nature of the NV center, allowing us to detect nuclear spin signals at zero- and low-field with a linearly polarized microwave field. As conventional dynamical decoupling protocols fail in this regime, we develop new robust pulse sequences and optimized pulse pairs, which allow us to sense temperature and weak AC magnetic fields and achieve an efficient decoupling from environmental noise. The sensing scheme is applicable to common NV center based setups and opens new frontiers for the application of NV centers as magnetic field sensors in the zero- and low-field regime.
We present a scheme to generate entangled photons using the NV centers in diamond. We show how the long-lived nuclear spin in diamond can mediate entanglement between multiple photons thereby increasing the length of entangled photon string. With the proposed scheme one could generate both n-photon GHZ and cluster states. We present an experimental scheme realizing the same and estimating the rate of entanglement generation both in the presence and absence of a cavity.
In this article we present a simple repeater scheme based on the negatively-charged nitrogen vacancy centre in diamond (NV-). Each repeater node is built from simple modules comprising an optical cavity containing a single NV-, with one nuclear spin from 15N as quantum memory. The operation in the module only uses deterministic processes and interactions and achieves high fidelity (>99%) operation, and modules are connected by optical fiber. In the repeater node architecture, the processes between modules by photons can be in principle deterministic, however current limitations on optical components lead to the processes to be probabilistic but heralded. The most resource modest repeater architecture contains at least two modules at each node, and the repeater nodes are than connected by telecom wavelength entangled photon pairs. We discuss the performance of quantum repeaters starting from the minimum-resource strategy with several modules (~10) and then incorporating more resource-intense strategies step by step. Our architecture enables large-scale quantum information networks with existing technology.
Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose and demonstrate a magnetic-field-independent, deterministic and highly efficient polarization scheme by introducing chopped laser pulses into the double-resonance initialization method. With this method, we demonstrate initialization of single-nuclear-spin approaching $98.1%$ and a $^{14}N$-$^{13}C$ double-nuclear-spin system approaching $96.8%$ at room temperature. The initialization is limited by a nuclear-spin depolarization effect due to chopped laser excitation. Our approach could be extended to NV systems with more nuclear spins and would be a useful tool in future applications such as nano-MRI and single-cell NMR.
Microfludic channels are now a well established platform for many purposes, including bio-medical research and Lab on a Chip applications. However, the nature of flow within these channels is still unclear. There is evidence that the mean drift velocity in these channels deviates from the regular Navier-Stokes solution with `no slip boundary conditions. Understanding these effects, is not only of value for fundamental fluid mechanics interest, but it also has practical importance for the future development of microfluidic and nanofludic infrastructures. We propose a nano-NMR based setup for measuring the drift velocity near the surface of a microfludic channel in a non-intrusive fashion. We discuss different possible protocols, and provide a detailed analysis of the measurements sensitivity in each case. We show that the nano-NMR scheme outperforms current fluorescence based techniques.
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