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Register a new userThe pressure-enhanced superconducting phase of Sr$_x$-Bi$_2$Se$_3$ probed by hard point contact spectroscopy
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The superconducting systems emerging from topological insulators upon metal ion intercalation or application of high pressure are ideal for investigation of possible topological superconductivity. In this context, Sr-intercalated Bi$_2$Se$_3$ is specially interesting because it displays pressure induced re-entrant superconductivity where the high pressure phase shows almost two times higher $T_c$ than the ambient superconducting phase ( $T_Csim$ 2.9 K). Interestingly, unlike the ambient phase, the pressure-induced superconducting phase shows strong indication of unconventional superconductivity. However, since the pressure-induced phase remains inaccessible to spectroscopic techniques, the detailed study of the phase remained an unattained goal. Here we show that the high-pressure phase can be realized under a mesoscopic point contact, where transport spectroscopy can be used to probe the spectroscopic properties of the pressure-induced phase. We find that the point contact junctions on the high-pressure phase show unusual response to magnetic field supporting the possibility of unconventional superconductivity.
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Recently it was demonstrated that Sr intercalation provides a new route to induce superconductivity in the topological insulator Bi$_2$Se$_3$. Topological superconductors are predicted to be unconventional, with mixed even and odd parity Cooper pairs states. An adequate probe to test for unconventional superconductivity is the upper critical field, $B_{c2}$. For a standard BCS layered superconductor $B_{c2}$ shows an anisotropy when the magnetic field is applied parallel and perpendicular to the layers, but is isotropic when the field is rotated in the plane of the layers. Here we report measurements of the upper critical field of superconducting Sr$_x$Bi$_2$Se$_3$ crystals ($T_c = 3.0$~K). Surprisingly, field-angle dependent magnetotransport measurements reveal a large anisotropy of $B_{c2}$ when the magnet field is rotated in the basal plane. The large two-fold anisotropy, while six-fold is anticipated, cannot be explained with the Ginzburg-Landau anisotropic effective mass model or flux flow induced by the Lorentz force. The rotational symmetry breaking of $B_{c2}$ indicates unconventional superconductivity with an odd-parity polarized triplet Cooper pair state ($Delta_4$-pairing) recently proposed for rhombohedral topological superconductors, or might have a structural nature, such as self-organized stripe ordering of Sr atoms.
The discovery of topological superconductivity in doped Bi$_2$Se$_3$ made this class of materials highly important for the field of condensed matter physics. However, the structural origin of the superconducting state remained elusive, despite being investigated intensively in recent years. We use scanning tunneling microscopy and the normal incidence x-ray standing wave (NIXSW) technique in order to determine the vertical position of the dopants -- one of the key parameters for understanding topological superconductivity in this material -- for the case of Sr$_{x}$Bi$_2$Se$_3$. In a novel approach we analyze the NIXSW data in consideration of the inelastic mean free path of the photoemitted electrons, which allows us to distinguish between symmetry equivalent sites. We find that Sr-atoms are not situated inside the van der Waals gap between the Bi$_2$Se$_3$ quintuple layers but rather in the quintuple layer close to the outer Se planes.
An archetypical layered topological insulator Bi$_2$Se$_3$ becomes superconductive upon doping with Sr, Nb or Cu. Superconducting properties of these materials in the presence of in-plane magnetic field demonstrate spontaneous symmetry breaking: 180$^circ$-rotation symmetry of superconductivity versus 120$^circ$-rotation symmetry of the crystal. Such behavior brilliantly confirms nematic topological superconductivity. To what extent this nematicity is due to superconducting pairing in these materials, rather than due to crystal structure distortions? This question remained unanswered, because so far no visible deviations from the 3-fold crystal symmetry were resolved in these materials. To address this question we grow high quality single crystals of Sr$_x$Bi$_2$Se$_3$, perform detailed X-ray diffraction and magnetotransport studies and reveal that the observed superconducting nematicity direction correlates with the direction of small structural distortions in these samples( $sim 0.02$% elongation in one crystallographic direction). Additional anisotropy comes from orientation of the crystallite axes. 2-fold symmetry of magnetoresistance observed in the most uniform crystals well above critical temperature demonstrates that these structural distortions are nevertheless strong enough. Our data in combination with strong sample-to-sample variation of the superconductive anisotropy parameter are indicative for significance of the structural factor in the apparent nematic superconductivity in Sr$_x$Bi$_2$Se$_3$.
A state of matter with a multi-component order parameter can give rise to vestigial order. In the vestigial phase, the primary order is only partially melted, leaving a remaining symmetry breaking behind, an effect driven by strong classical or quantum fluctuations. Vestigial states due to primary spin and charge-density-wave order have been discussed in the context of iron-based and cuprate materials. Here we present the observation of a partially melted superconductor in which pairing fluctuations condense at a separate phase transition and form a nematic state with broken Z3, i.e. three-state Potts-model symmetry. High-resolution thermal expansion, specific heat and magnetization measurements of the doped topological insulator NbxBi2Se3 reveal that this symmetry breaking occurs at Tnem=3.8 K above Tc=3.25 K, along with an onset of superconducting fluctuations. Thus, before Cooper pairs establish long-range coherence at Tc, they fluctuate in a way that breaks the rotational invariance at Tnem and induces a distortion of the crystalline lattice. Similar results are found for CuxBi2Se3.
We present a novel experimental evidence for the odd-parity nematic superconductivity in high-quality single crystals of doped topological insulator Sr$_x$Bi$_2$Se$_3$. The X-ray diffraction shows that the grown single crystals are either weakly stretched or compressed uniaxially in the basal plane along one of the crystal axis. We show that in the superconducting state, the upper critical magnetic field $H_{c2}$ has a two-fold rotational symmetry and depends on the sign of the strain: in the stretched samples, the maximum of $H_{c2}$ is achieved when the in-plane magnetic field is transverse to the strain axis, while in the compressed samples this maximum is observed when the field is along the strain direction. This result is naturally explained within a framework of the odd-parity nematic superconductivity coupled to the strain. Magnetoresistance in the normal state is independent of the current direction and also has a two-fold rotational symmetry that demonstrates the nematicity of the electronic system in the normal state.
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