No Arabic abstract
Despite the several novel features arising from the dissipative optomechanical coupling, such effect remains vastly unexplored due to the lack of a simple formalism that captures non-Hermiticity in optomechanical systems. In this Letter, we show that quasinormal-mode-based perturbation theory is capable of correctly predicting both dispersive and dissipative optomechanical couplings. We validate our model through simulations and also by comparison with experimental results reported in the literature. Finally, we apply this formalism to plasmonic systems, used for molecular optomechanics, where strong dissipative coupling signatures in the amplification of vibrational modes are observed.
Coupled mode theory (CMT) is a powerful framework for decomposing interactions between electromagnetic waves and scattering bodies into resonances and their couplings with power-carrying channels. It has widespread use in few-resonance, weakly coupled resonator systems across nanophotonics, but cannot be applied to the complex scatterers of emerging importance. We use quasinormal modes to develop an exact, ab initio generalized coupled mode theory from Maxwells equations. This quasinormal coupled mode theory, which we denote QCMT, enables a direct, mode-based construction of scattering matrices without resorting to external solvers or data. We consider canonical scattering bodies, for which we show that a CMT model will necessarily be highly inaccurate, whereas QCMT exhibits near-perfect accuracy.
Optical resonators are widely used in modern photonics. Their spectral response and temporal dynamics are fundamentally driven by their natural resonances, the so-called quasinormal modes (QNMs), with complex frequencies. For optical resonators made of dispersive materials, the QNM computation requires solving a nonlinear eigenvalue problem. This rises a difficulty that is only scarcely documented in the literature. We review our recent efforts for implementing efficient and accurate QNM-solvers for computing and normalizing the QNMs of micro- and nano-resonators made of highly-dispersive materials. We benchmark several methods for three geometries, a two-dimensional plasmonic crystal, a two-dimensional metal grating, and a three-dimensional nanopatch antenna on a metal substrate, in the perspective to elaborate standards for the computation of resonance modes.
Dissipative and dispersive optomechanical couplings are experimentally observed in a photonic crystal split-beam nanocavity optimized for detecting nanoscale sources of torque. Dissipative coupling of up to approximately $500$ MHz/nm and dispersive coupling of $2$ GHz/nm enable measurements of sub-pg torsional and cantilever-like mechanical resonances with a thermally-limited torque detection sensitivity of 1.2$times 10^{-20} text{N} , text{m}/sqrt{text{Hz}}$ in ambient conditions and 1.3$times 10^{-21} text{N} , text{m}/sqrt{text{Hz}}$ in low vacuum. Interference between optomechanical coupling mechanisms is observed to enhance detection sensitivity and generate a mechanical-mode-dependent optomechanical wavelength response.
We report a self-consistent quasinormal mode theory for nanometer scale electromagnetism where the possible nonlocal and quantum effects are treated through quantum surface responses. With Feibelmans frequency-dependent textit{d} parameters to describe the quantum surface responses, we formulate the source-free Maxwells equations into a generalized linear eigenvalue problem to define the quasinormal modes. We then construct an orthonormal relation for the modes and consequently unlock the powerful toolbox of modal analysis. The orthonormal relation is validated by the reconstruction of the full numerical results through modal contributions. Significant changes in the landscape of the modes are observed due to the incorporation of the quantum surface responses for a number of nanostructures. Our semi-analytical modal analysis enables transparent physical interpretation of the spontaneous emission enhancement of a dipolar emitter as well as the near-field and far-field responses of planewave excitations in the nanostructures.
We present a theoretical study of optomechanical systems in which the mechanical resonator modulates both the resonant frequency (dispersive coupling) and the decay rates (dissipative coupling) of the optical cavity. We extend the generic dispersive framework to a more general case in which the dissipative coupling is split between its external and intrinsic contribution. We report a complete analysis of the influence of each kind of optical losses (intrinsic and external) on the three coupling mechanisms and highlight the interest of each external decay rate regime. The basic tools to experimentally identify the three couplings and their relative influence on the optical response are presented. We demonstrate the general expression of the optical spring effect and optomechanical damping. Comparison between experimental measurements in photonic crystal systems from the literature and our theoretical modal yields good agreement.