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Thermoelectric current in a graphene Cooper pair splitter

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 Added by Nikita Kirsanov
 Publication date 2020
  fields Physics
and research's language is English




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Thermoelectric effect generating electricity from thermal gradient and vice versa appears in numerous generic applications. Recently, an original prospect of thermoelectricity arising from the nonlocal Cooper pair splitting (CPS) and the elastic co-tunneling (EC) in hybrid normal metal-superconductor-normal metal (NSN) structures was foreseen. Here we demonstrate experimentally the existence of non-local Seebeck effect in a graphene-based CPS device comprising two quantum dots connected to an aluminum superconductor and theoretically validate the observations. This non-local Seebeck effect offers an efficient tool for producing entangled electrons.



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We report an experimental study of Cooper pair splitting in an encapsulated graphene based multiterminal junction in the ballistic transport regime. Our device consists of two transverse junctions, namely the superconductor/graphene/superconductor and the normal metal/graphene/normal metal junctions. In this case, the electronic transport through one junction can be tuned by an applied bias along the other. We observe clear signatures of Cooper pair splitting in the local as well as nonlocal electronic transport measurements. Our experimental data can be very well described by using a modified Octavio-Tinkham-Blonder-Klapwijk model and a three-terminal beam splitter model.
We propose an approach allowing the computation of currents and their correlations in interacting multiterminal mesoscopic systems involving quantum dots coupled to normal and/or superconducting leads. The formalism relies on the expression of branching currents and noise crossed correlations in terms of one- and two-particle Greens functions for the dots electrons, which are then evaluated self-consistently within a conserving approximation. We then apply this to the Cooper-pair beam-splitter setup recently proposed [L. Hofstetter et al. Nature (London) 461 960 (2009); Phys. Rev. Lett. 107 136801 (2011); L. G. Herrmann et al. Phys. Rev. Lett. 104 026801 (2010)], which we model as a double quantum dot with weak interactions, connected to a superconducting lead and two normal ones. Our method not only enables us to take into account a local repulsive interaction on the dots, but also to study its competition with the direct tunneling between dots. Our results suggest that even a weak Coulomb repulsion tends to favor positive current cross correlations in the antisymmetric regime (where the dots have opposite energies with respect to the superconducting chemical potential).
Cooper pair splitters are promising candidates for generating spin-entangled electrons. However, the splitting of Cooper pairs is a random and noisy process, which hinders further synchronized operations on the entangled electrons. To circumvent this problem, we here propose and analyze a dynamic Cooper pair splitter that produces a noiseless and regular flow of spin-entangled electrons. The Cooper pair splitter is based on a superconductor coupled to quantum dots, whose energy levels are tuned in and out of resonance to control the splitting process. We identify the optimal operating conditions for which exactly one Cooper pair is split per period of the external drive and the flow of entangled electrons becomes noiseless. To characterize the regularity of the Cooper pair splitter in the time domain, we analyze the $g^{(2)}$-function of the output currents and the distribution of waiting times between split Cooper pairs. Our proposal is feasible using current technology, and it paves the way for dynamic quantum information processing with spin-entangled electrons.
We investigate the nonlocal thermoelectric transport in a Cooper-pair splitter based on a double-quantum-dot-superconductor three-terminal hybrid structure. We find that the nonlocal coupling between the superconductor and the quantum dots gives rise to nonlocal thermoelectric effects which originate from the nonlocal particle-hole breaking of the system. We show that Cooper-pair splitting induces the generation of a thermo-current in the superconducting lead without any transfer of charge between the two normal metal leads. Conversely, we show that a nonlocal heat exchange between the normal leads is mediated by non-local Andreev reflection. We discuss the influence of finite Coulomb interaction and study under which conditions nonlocal power generation becomes possible, and when the Cooper-pair splitter can be employed as a cooling device.
We consider a double quantum dot coupled to two normal leads and one superconducting lead, modeling the Cooper pair beam splitter studied in two recent experiments. Starting from a microscopic Hamiltonian we derive a general expression for the branching current and the noise crossed correlations in terms of single and two-particle Greens function of the dot electrons. We then study numerically how these quantities depend on the energy configuration of the dots and the presence of direct tunneling between them, isolating the various processes which come into play. In absence of direct tunneling, the antisymmetric case (the two levels have opposite energies with respect to the superconducting chemical potential) optimizes the Crossed Andreev Reflection (CAR) process while the symmetric case (the two levels have the same energies) favors the Elastic Cotunneling (EC) process. Switching on the direct tunneling tends to suppress the CAR process, leading to negative noise crossed correlations over the whole voltage range for large enough direct tunneling.
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