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Predictions of $alpha$ decay half-lives for even-even superheavy nuclei with $104 leqslant Z leqslant 128$ based on two-potential approach within cluster-formation model

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 Added by Xiao-Hua Li
 Publication date 2020
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and research's language is English




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In present work, we systematically study the $alpha$ decay half-lives of 170 even-even nuclei with $60 leqslant Z leqslant 118$ within the two-potential approach while the $alpha$ decay preformation factor $P_alpha$ is obtained by the cluster-formation model. The calculated results can well reproduce the experimental data. In addition, we extend this model to predict the $alpha$ decay half-lives of 64 even-even nuclei with $104 leqslant Z leqslant 128$ whose $alpha$ decay is energetically allowed or observed but not yet quantified. For comparing, the two famous models i.e. SemFIS proposed by D. Poenaru ${et al.}$ [href {https://doi.org/10.1209/0295-5075/77/62001}{Europhys. Lett. textbf{77} (2007) 62001}] and UDL proposed by C. Qi ${et al.}$ [href {https://doi.org/10.1103/PhysRevLett.103.072501}{Phys. Rev. Lett. textbf{103} (2009) 072501}] are used. The predicted results of these models are basically consistent. At the same time, through analyzing the changing trend of $alpha$ decay energy $Q_{alpha}$ of emph{Z} = 118, 120, 122, 124, 126 and 128 isotopes nuclei with the increasing of neutron number emph{N} and that of $alpha$ decay preformation factor $P_alpha$ of those isotopes even-even nuclei with the increasing of neutron number emph{N}, emph{N} = 178 may be a new neutron magic number.



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252 - G. Royer , H.F. Zhang 2008
New recent experimental $alpha$ decay half-lives have been compared with the results obtained from previously proposed formulas depending only on the mass and charge numbers of the $alpha$ emitter and the Q$alpha$ value. For the heaviest nuclei they are also compared with calculations using the Density-Dependent M3Y (DDM3Y) effective interaction and the Viola-Seaborg-Sobiczewski (VSS) formulas. The correct agreement allows us to make predictions for the $alpha$ decay half-lives of other still unknown superheavy nuclei from these analytic formulas using the extrapolated Q$alpha$ of G. Audi, A. H. Wapstra, and C. Thibault [Nucl. Phys. A729, 337 (2003)].
The Quark-Meson-Coupling (QMC) model has been applied to the study of the properties of even-even super-heavy nuclei with 96 < Z < 110, over a wide range of neutron numbers. The aim is to identify the deformed shell gaps at N = 152 and N = 162 predicted in macroscopic-microscopic (macro-micro) models, in a model based on the mean-field Hartree-Fock+BCS approximation. The predictive power of the model has been tested on proton and neutron spherical shell gaps in light doubly closed (sub)shell nuclei. In the super-heavy region, the ground state binding energies of 98 < Z < 110 and 146 < N < 160 differ, in the majority of cases, from the measured values by less than 2.5 MeV, with the deviation decreasing with increasing Z and N. The axial quadrupole deformation parameter, calculated over the range of neutron numbers 138 < N < 184, revealed a prolate-oblate coexistence and shape transition around N = 168, followed by an oblate-spherical transition towards the expected N = 184 shell closure in Cm, Cf, Fm and No. The closure is not predicted in Rf, Sg, Hs and Ds as another shape transition to a highly deformed shape in Sg, Hs and Ds for N > 178 appears, while 288Rf (N = 184) remains oblate. The bulk properties predicted by QMC are found to have a limited sensitivity to the deformed shell gaps at N = 152 and 162. However, the evolution of the neutron single-particle spectra with 0 < beta2 < 0.55 gives unambiguous evidence for the location and size of the N = 152 and 162 gaps as a function of Z and N. In addition, the neutron number dependence of neutron pairing energies provides supporting evidence for existence of the energy gaps.
Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in the macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential. A standard flooding technique has been used to determine the barrier heights. It was shown the Fourier shape parametrization containing only three deformation parameters reproduces well the nuclear shapes of nuclei on their way to fission. In addition, the non-axial degree of freedom is taken into account to describe better the form of nuclei around the ground state and in the saddles region. Apart from the symmetric fission valley, a new very asymmetric fission mode is predicted in most superheavy nuclei. The fission fragment mass distributions of considered nuclei are obtained by solving the 3D Langevin equations.
$alpha$ decay is usually associated with both ground and low-lying isomeric states of heavy and superheavy nuclei, and the unpaired nucleon plays a key role on $alpha$ decay. In this work, we systematically studied the $alpha$ decay half-lives of odd-$A$ nuclei, including both favored and unfavored $alpha$ decay within the two-potential approach based on the isospin dependent nuclear potential. The $alpha$ preformation probabilities are estimated by using an analytic formula taking into account the shell structure and proton-neutron correlation, and the parameters are obtained through the $alpha$ decay half-lives data. The results indicate that in general the $alpha$ preformation probabilities of even-$Z$, odd-$N$ nuclei are slightly smaller than the odd-$Z$, even-$N$ ones. We found that the odd-even staggering effect may play a more important role on spontaneous fission than $alpha$ decay. The calculated half-lives can well reproduce the experimental data.
In this work, we systematically study the two-proton($2p$) radioactivity half-lives using the two-potential approach while the nuclear potential is obtained by using Skyrme-Hartree-Fock approach with the Skyrme effective interaction of {SLy8}. For true $2p$ radioactivity($Q_{2p}$ $>$ 0 and $Q_p$ $< $0, where the $Q_p$ and $Q_{2p}$ are the released energy of the one-proton and two-proton radioactivity), the standard deviation between the experimental half-lives and our theoretical calculations is {0.701}. In addition, we extend this model to predict the half-lives of 15 possible $2p$ radioactivity candidates with $Q_{2p}$ $>$ 0 taken from the evaluated atomic mass table AME2016. The calculated results indicate that a clear linear relationship between the logarithmic $2p$ radioactivity half-lives $rm{log}_{10}T_{1/2}$ and coulomb parameters [ ($Z_{d}^{0.8}$+$l^{0.25}$)$Q_{2p}^{-1/2}$] considered the effect of orbital angular momentum proposed by Liu $et$ $al$ [Chin. Phys. C textbf{45}, 024108 (2021)] is also existed. For comparison, the generalized liquid drop model(GLDM), the effective liquid drop model(ELDM) and Gamow-like model are also used. Our predicted results are consistent with the ones obtained by the other models.
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