Metamagnetic transitions and anomalous magnetoresistance in EuAg$_4$As$_2$ single crystal


Abstract in English

In this paper, the magnetic and transport properties were systematically studied for EuAg$_4$As$_2$ single crystals, crystallizing in a centrosymmetric trigonal CaCu$_4$P$_2$ type structure. It was confirmed that two magnetic transitions occur at $textit{T}$$_{N1}$ = 10 K and $textit{T}$$_{N2}$ = 15 K, respectively. With the increasing field, the two transitions are noticeably driven to lower temperature. At low temperatures, applying a magnetic field in the $textit{ab}$ plane induces two successive metamagnetic transitions. For both $textit{H}$ $parallel$ $textit{ab}$ and $textit{H}$ $parallel$ $textit{c}$, EuAg$_4$As$_2$ shows a positive, unexpected large magnetoresistance (up to 202%) at low fields below 10 K, and a large negative magnetoresistance (up to -78%) at high fields/intermediate temperatures. Such anomalous field dependence of magnetoresistance may have potential application in the future magnetic sensors. Finally, the magnetic phase diagrams of EuAg$_{4}$As$_{2}$ were constructed for both $textit{H}$ $parallel$ $textit{ab}$ and $textit{H}$ $parallel$ $textit{c}$.

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