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Developments and improvements of radiopure ZnWO$_{4}$ anisotropic scintillators

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 Added by Riccardo Cerulli
 Publication date 2020
  fields Physics
and research's language is English




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The ZnWO$_4$ is an anisotropic crystal scintillator; for its peculiar characteristics, it is a very promising detector to exploit the so-called directionality approach in the investigation of those Dark Matter (DM) candidates inducing nuclear recoils. Recently, in the framework of the ADAMO project, an R&D to develop high quality and ultra-radiopure ZnWO$_4$ crystal scintillators has been carried out. In the present paper the measurements to study the anisotropic response of a ZnWO$_4$ to $alpha$ particles and to nuclear recoils induced by neutron scattering are reported. Monochromatic neutrons have been produced by a neutron generator at ENEA-CASACCIA. The quenching factor values for nuclear recoils along different crystallographic axes have been determined for three different nuclear recoils energies. These results open the possibility to realize a pioneer experiment to investigate the above mentioned DM candidates by means of the directionality.



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As low as possible radioactive contamination of a detector plays a crucial role to improve sensitivity of a double beta decay experiment. The radioactive contamination of a sample of $^{116}$CdWO$_4$ crystal scintillator by thorium was reduced by a factor $approx 10$, down to the level 0.01 mBq/kg ($^{228}$Th), by exploiting the recrystallization procedure. The total alpha activity of uranium and thorium daughters was reduced by a factor $approx 3$, down to 1.6 mBq/kg. No change in the specific activity (the total $alpha$ activity and $^{228}$Th) was observed in a sample of ZnWO$_4$ crystal produced by recrystallization after removing $approx 0.4$ mm surface layer of the crystal.
Anisotropic scintillators can offer a unique possibility to exploit the so-called directionality approach in order to investigate the presence of those Dark Matter (DM) candidates inducing nuclear recoils. In fact, their use can overcome the difficulty of detecting extremely short nuclear recoil traces. In this paper we present recent measurements performed on the anisotropic response of a ZnWO$_4$ crystal scintillator to nuclear recoils, in the framework of the ADAMO project. The anisotropic features of the ZnWO$_4$ crystal scintillators were initially measured with $alpha$ particles; those results have been also confirmed by the additional measurements presented here. The experimental nuclear recoil data were obtained by using a neutron generator at ENEA-CASACCIA and neutron detectors to tag the scattered neutrons; in particular, the quenching factor values for nuclear recoils along different crystallographic axes have been determined for three different neutron scattering angles (i.e. nuclear recoils energies). From these measurements, the anisotropy of the light response for nuclear recoils in the ZnWO$_4$ crystal scintillator has been determined at 5.4 standard deviations.
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