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Giant supercurrent drag effect between graphene and LaAlO3/SrTiO3 interface

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 Added by Ran Tao
 Publication date 2020
  fields Physics
and research's language is English




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Double-layer electronic systems enable the investigation of interlayer quasiparticle interactions and the discovery of intriguing interlayer correlated states. Here we report interlayer drag measurements between graphene and superconducting LaAlO3/SrTiO3 (LAO/STO) heterointerface separated by a natural insulating barrier of LAO (as thin as 2 nm). Applying a drive current (Idrive) in the graphene layer induces a negative drag voltage at the LAO/STO interface in the vicinity of the superconducting transition, which is attributed to the supercurrent drag effect, arising from the interlayer interactions involving the superconducting carriers. Benefiting from the high tunability of both layers and the ultra-small interlayer spacing, an extremely large interlayer current coupling ratio (r = |Idrag/Idrive|, Idrag: the equivalent drag current at LAO/STO interface) is eventually achieved, surpassing conventional systems consisting of normal metal and superconducting films by two orders of magnitude. More strikingly, this ratio is estimated to be up to 10^5 at the zero-temperature limit. The unique temperature- and carrier density/polarity-dependent behaviors suggest a brand-new microscopic interaction mechanism accounting for the observed giant supercurrent drag effect. Our study is anticipated to inspire further exploration of hybrid interlayer coupling via utilization of newly-emerging two-dimensional electronic systems, in particular those exhibiting long-range electronic and magnetic orders.



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Heterostructures made of transition metal oxides are new tailor-made materials which are attracting much attention. We have constructed a 6-band k.p Hamiltonian and used it within the envelope function method to calculate the subband structure of a variety of LaAlO3/SrTiO3 heterostructures. By use of density functional calculations, we determine the k.p parameters describing the conduction band edge of SrTiO3: the three effective mass parameters, L=0.6104 eV AA^2, M=9.73 eV AA^2, N=-1.616 eV AA^2, the spin orbit splitting Delta_SO=28.5 meV and the low temperature tetragonal distortion energy splitting Delta_T=2.1 meV. For confined systems we find strongly anisotropic non-parabolic subbands. As an application we calculate bands, density of states and magnetic energy levels and compare the results to Shubnikov-de Haas quantum oscillations observed in high magnetic fields. For typical heterostructures we find that electric field strength at the interface of F = 0.1 meV/AA for a carrier density of 7.2 10^{12} cm^-2 results in a subband structure that is similar to experimental results.
691 - Y. Lei , Y. Z. Chen , Y. W. Xie 2014
Electrical field and light-illumination have been two most widely used stimuli in tuning the conductivity of semiconductor devices. Via capacitive effect electrical field modifies the carrier density of the devices, while light-illumination generates extra carriers by exciting trapped electrons into conduction band1. Here, we report on an unexpected light illumination enhanced field effect in a quasi-two-dimensional electron gas (q2DEG) confined at the LaAlO3/SrTiO3 (LAO/STO) interface which has been the focus of emergent phenomenon exploration2-14. We found that light illumination greatly accelerates and amplifies the field effect, driving the field-induced resistance growth which originally lasts for thousands of seconds into an abrupt resistance jump more than two orders of magnitude. Also, the field-induced change in carrier density is much larger than that expected from the capacitive effect, and can even be opposite to the conventional photoelectric effect. This work expands the space for novel effect exploration and multifunctional device design at complex oxide interfaces.
Reports of emergent conductivity, superconductivity, and magnetism at oxide interfaces have helped to fuel intense interest in their rich physics and technological potential. Here we employ magnetic force microscopy to search for room-temperature magnetism in the well-studied LaAlO3/SrTiO3 system. Using electrical top gating to deplete electrons from the oxide interface, we directly observe an in-plane ferromagnetic phase with sharply defined domain walls. Itinerant electrons, introduced by a top gate, align antiferromagnetically with the magnetization, at first screening and then destabilizing it as the conductive state is reached. Subsequent depletion of electrons results in a new, uncorrelated magnetic pattern. This newfound control over emergent magnetism at the interface between two non-magnetic oxides portends a number of important technological applications.
The oxide heterostructure LaAlO3/SrTiO3 supports a two-dimensional electron liquid with a variety of competing phases including magnetism, superconductivity and weak antilocalization due to Rashba spin-orbit coupling. Further confinement of this 2D electron liquid to the quasi-one-dimensional regime can provide insight into the underlying physics of this system and reveal new behavior. Here we describe magnetotransport experiments on narrow LaAlO3/SrTiO3 structures created by a conductive atomic force microscope lithography technique. Four-terminal local transport measurements on ~10-nm-wide Hall bar structures yield longitudinal resistances that are comparable to the resistance quantum h/e2 and independent of the channel length. Large nonlocal resistances (as large as 10^4 ohms) are observed in some but not all structures with separations between current and voltage that are large compared to the 2D mean-free path. The nonlocal transport is strongly suppressed by the onset of superconductivity below ~200 mK. The origin of these anomalous transport signatures is not understood, but may arise from coherent transport defined by strong spin-orbit coupling and/or magnetic interactions.
The magnetoresistance as a function of temperature and field for atomically flat interfaces between 8 unit cells of LaAlO3 and SrTiO3 is reported. Anomalous anisotropic behavior of the magnetoresistance is observed below 30 K for superconducting samples with carrier concentration of 3.5times10^13 cm^-2 . We associate this behavior to a magnetic order formed at the interface.
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