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Register a new userExotic photonic molecules via Lennard-Jones-like potentials
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Ultracold systems offer an unprecedented level of control of interactions between atoms. An important challenge is to achieve a similar level of control of the interactions between photons. Towards this goal, we propose a realization of a novel Lennard-Jones-like potential between photons coupled to the Rydberg states via electromagnetically induced transparency (EIT). This potential is achieved by tuning Rydberg states to a F{o}rster resonance with other Rydberg states. We consider few-body problems in 1D and 2D geometries and show the existence of self-bound clusters (molecules) of photons. We demonstrate that for a few-body problem, the multi-body interactions have a significant impact on the geometry of the molecular ground state. This leads to phenomena without counterparts in conventional systems: For example, three photons in 2D preferentially arrange themselves in a line-configuration rather than in an equilateral-triangle configuration. Our result opens a new avenue for studies of many-body phenomena with strongly interacting photons.
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In the field of ultracold atoms in optical lattices a plethora of phenomena governed by the hopping energy $J$ and the interaction energy $U$ have been studied in recent years. However, the trapping potential typically present in these systems sets another energy scale and the effects of the corresponding time scale on the quantum dynamics have rarely been considered. Here we study the quantum collapse and revival of a lattice Bose-Einstein condensate (BEC) in an arbitrary spatial potential, focusing on the special case of harmonic confinement. Analyzing the time evolution of the single-particle density matrix, we show that the physics arising at the (temporally) recurrent quantum phase revivals is essentially captured by an effective single particle theory. This opens the possibility to prepare exotic non-equilibrium condensate states with a large degree of freedom by engineering the underlying spatial lattice potential.
Liquid crystals (LCs) composed of mesogens play important roles in various scientific and engineering problems. How a system with many mesogens can enter a LC state is an interesting and important problem. Using stiff and free-joint Lennard-Jones chain molecules as mesogens, we study the conditions under which the mesogens can enter various LC phases. The guideline is to eliminate the unwanted translational orders under a controlled fine-tuning procedure across a sequence of systems. Instead of monitoring the growth of order out of the disorder, we prepare a configuration of high orientation ordering and find out where it relaxes to. Such a procedure begins with a reference system, consisting of short chains of homogeneous soft spheres, in a liquid-vapor coexistence situation, at which the thermodynamic instability triggers a fast spontaneous growing process. By applying a short pulse of auxiliary field to align the dispersedly oriented clusters, followed by reducing the volume and, finally, changing the homogeneous molecules into heterogeneous chains, we are able to obtain a range of systems, including nematic and smectic LCs, at their stable ordered states. The model can be extended to study the influence of nanoparticles or external field on the LC structure.
The homogeneous and heterogeneous nucleation of a Lennard-Jones liquid is investigated using the umbrella sampling method. The free energy cost of forming a nucleating droplet is determined as a function of the quench depth, and the saddle point nature of the droplets is verified using an intervention technique. The structure and symmetry of the nucleating droplets is found for a range of temperatures. We find that for deep quenches the nucleating droplets become more anisotropic and diffuse with no well defined core or surface. The environment of the nucleating droplets form randomly stacked hexagonal planes. This behavior is consistent with a spinodal nucleation interpretation. We also find that the free energy barrier for heterogeneous nucleation is a minimum when the lattice spacing of the impurity equals the lattice spacing of the equilibrium crystalline phase. If the lattice spacing of the impurity is different, the crystal grows into the bulk instead of wetting the impurity.
The definitions of breaks and clusters in a one-dimensional chain in equilibrium are discussed. Analytical expressions are obtained for the expected cluster length, $langle K rangle$, as a function of temperature and pressure in a one-dimensional Lennard-Jones chain. These expressions are compared with results from molecular dynamics simulations. It is found that $langle K rangle$ increases exponentially with $beta = 1/k_BT$ and with pressure, $P$ in agreement with previous results in the literature. A method is illustrated for using $langle K rangle (beta, P)$ to generate a phase diagram for the Lennard-Jones chain. Some implications for the study of heat transport in Lennard-Jones chains are discussed.
We report on numerical procedures for, and preliminary results on the search for, tunnelling centres in Lennard-Jones clusters, seen as simple model systems of glasses. Several of the double-well potentials identified are good candidates to give rise to two-level systems. The role of boundary effects, and the application of the semiclassical WKB approximation in multidimensional spaces for the calculation of the ground state splitting are discussed.
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