No Arabic abstract
A theoretical study is performed for the excitation of a single atom localized in the center of twisted light modes. Here we present the explicit dependence of excitation rates on critical parameters, such as the polarization of light, its orbital angular momentum projection, and the orientation of its propagation axis with respect to the atomic quantization axis. The effect of a spatial spread of the atom is also considered in detail. The expressions for transition rates obtained in this work can be used for any atom of arbitrary electronic configuration. For definiteness we apply them to the specific case of $^{2}S_{1/2} (F=0) rightarrow; ^{2}F_{7/2} (F=3, M=0)$ electric octupole (E3) transition in $^{171}$Yb$^{+}$ ion. Our analytical and numerical results are suitable for the analysis and planning of future experiments on the excitation of electric-dipole-forbidden transitions by twisted light modes in optical atomic clocks.
Modern intense ultrafast pulsed lasers generate an electric field of sufficient strength to permit tunnel ionization of the valence electrons in atoms. This process is usually treated as a rapid succession of isolated events, in which the states of the remaining electrons are neglected. Such electronic interactions are predicted to be weak, the exception being recollision excitation and ionization caused by linearly-polarized radiation. In contrast, it has recently been suggested that intense field ionization may be accompanied by a two-stage `shake-up reaction. Here we report a unique combination of experimental techniques that enables us to accurately measure the tunnel ionization probability for argon exposed to 50 femtosecond laser pulses. Most significantly for the current study, this measurement is independent of the optical focal geometry, equivalent to a homogenous electric field. Furthermore, circularly-polarized radiation negates recollision. The present measurements indicate that tunnel ionization results in simultaneous excitation of one or more remaining electrons through shake-up. From an atomic physics standpoint, it may be possible to induce ionization from specific states, and will influence the development of coherent attosecond XUV radiation sources. Such pulses have vital scientific and economic potential in areas such as high-resolution imaging of in-vivo cells and nanoscale XUV lithography.
We analyze a similar scheme for producing light-mediated entanglement between atomic ensembles, as first realized by Julsgaard, Kozhekin and Polzik [Nature {bf 413}, 400 (2001)]. In the standard approach to modeling the scheme, a Holstein-Primakoff approximation is made, where the atomic ensembles are treated as bosonic modes, and is only valid for short interaction times. In this paper, we solve the time evolution without this approximation, which extends the region of validity of the interaction time. For short entangling times, we find this produces a state with similar characteristics as a two-mode squeezed state, in agreement with standard predictions. For long entangling times, the state evolves into a non-Gaussian form, and the two-mode squeezed state characteristics start to diminish. This is attributed to more exotic types of entangled states being generated. We characterize the states by examining the Fock state probability distributions, Husimi $Q$ distributions, and non-local entanglement between the ensembles. We compare and connect several quantities obtained using the Holstein-Primakoff approach and our exact time evolution methods.
We experimentally investigate a recently proposed optical excitation scheme [V.I. Yudin et al., Phys. Rev. A 82, 011804(R)(2010)] that is a generalization of Ramseys method of separated oscillatory fields and consists of a sequence of three excitation pulses. The pulse sequence is tailored to produce a resonance signal which is immune to the light shift and other shifts of the transition frequency that are correlated with the interaction with the probe field. We investigate the scheme using a single trapped 171Yb+ ion and excite the highly forbidden 2S1/2-2F7/2 electric-octupole transition under conditions where the light shift is much larger than the excitation linewidth, which is in the Hertz range. The experiments demonstrate a suppression of the light shift by four orders of magnitude and an immunity against its fluctuations.
We present experimental evidence that light storage, i.e. the controlled release of a light pulse by an atomic sample dependent on the past presence of a writing pulse, is not restricted to small group velocity media but can also occur in a negative group velocity medium. A simple physical picture applicable to both cases and previous light storage experiments is discussed.
The elastic Rayleigh scattering of twisted light and, in particular, the polarization (transfer) of the scattered photons have been analyzed within the framework of second-order perturbation theory and Diracs relativistic equation. Special attention was paid hereby to the scattering on three different atomic targets: single atoms, a mesoscopic (small) target, and a macroscopic (large) target, which are all centered with regard to the beam axis. Detailed calculations of the polarization Stokes parameters were performed for C^{5+} ions and for twisted Bessel beams. It is shown that the polarization of scattered photons is sensitive to the size of an atomic target and to the helicity, the opening angle, and the projection of the total angular momentum of the incident Bessel beam. These computations indicate more that the Stokes parameters of the (Rayleigh) scattered twisted light may significantly differ from their behaviour for an incident plane-wave radiation.