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Third order parametric downconversion: a stimulated approach

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 Publication date 2020
  fields Physics
and research's language is English




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We study the process of seeded, or stimulated, third-order parametric down-conversion, as an extension of our previous work on spontaneous parametric downconversion (TOSPDC). We present general expressions for the spectra and throughputs expected for the cases where the seed field or fields overlap either only one or two of the TOSPDC modes, and also allow for both pump and seed to be either monochromatic or pulsed. We present a numerical study for a particular source design, showing that doubly-overlapped seeding can lead to a considerably greater generated flux as compared with singly-overlapped seeding. We furthermore show that doubly-overlapped seeding permits stimulated emission tomography for the reconstruction of the three-photon TOSPDC joint spectral intensity. We hope that our work will guide future experimental efforts based on the process of third-order parametric downconversion.



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We introduce a theoretical framework based on Fanos theory of discrete-continuum interactions to analyze the quantum dynamics of broadband parametric downconversion (PDC) in the few-pump-photon regime of nonlinear quantum nanophotonics. Applying this unified analytic approach to 1D $chi^{(2)}$-nonlinear waveguides, we find a host of remarkable dynamical features due to the coupling of a discrete pump state to the signal continuum, from unit-efficiency (i.e., complete) downconversion when the coupling is dissipative, to Rabi-like oscillations with sub-exponential decay when it is dispersive. The theory provides a straightforward way to analytically compute a full characterization of the PDC dynamics, including the complete eigensystem of the continuum Hamiltonian and expressions for the signal biphoton correlation function. We also apply the theory to study a pair of linearly coupled $chi^{(2)}$ waveguides, where two discrete pump states simultaneously downconvert into a common-mode signal continuum, resulting in Fano interference that critically affects the PDC rate. Under appropriate conditions, the theory predicts characteristic Fano lineshapes and even complete destructive interference resulting in the full suppression of PDC, due to the formation of a bound pump state in the continuum. Generalizing further, we show that the framework can also be applied to higher-order parametric processes such as parametric three-photon generation, and we also find numerical signatures that Fano-type interactions occur even for multi-photon PDC under stronger pumping. Our results establish broadband PDC as yet another physical system natively exhibiting Fano-type interactions and advance a theoretical framework in which to understand the complicated quantum dynamics of strongly nonlinear broadband quantum optics.
Optical fibers have been considered an optimal platform for third-order parametric down-conversion since they can potentially overcome the weak third-order nonlinearity by their long interaction length. Here we present, in the first part, a theoretical derivation for the conversion rate both in the case of spontaneous generation and in the presence of a seed beam. Then we review three types of optical fibers and we examine their properties in terms of conversion efficiency and practical feasibility.
The advanced-wave picture is ... an intuitive treatment of two-photon correlation with the help of the concept of an effective field acting upon one of the two detectors and formed by parametric conversion of the advanced wave emitted by the second detector ... [A. V. Belinskii and D. N. Klyshko, JETP 78, 259 (1994)]. This quote from Belinskii and Klyshko nicely describes the concept of the advanced-wave picture; an intuitive tool for designing and predicting results from coincidence-based two-photon experiments. Up to now, the advanced-wave picture has been considered primarily for the case of an ideal plane-wave pump beam and only for design purposes. Here we study the advanced wave picture for a structured pump beam and in the context of stimulated emission provoked by an auxiliary input laser beam. This suggests stimulated parametric down-conversion as a useful experimental tool for testing the experimental sets designed with the advanced-wave picture. We present experimental results demonstrating the strategy of designing the experiment with advanced-wave picture and testing with stimulated emission.
We address the pair of conjugated field modes obtained from parametric-downconversion as a convenient system to analyze the quantum-classical transition in the continuous variable regime. We explicitly evaluate intensity correlations, negativity and entanglement for the system in a thermal state and show that a hierarchy of nonclassicality thresholds naturally emerges in terms of thermal and downconversion photon number. We show that the transition from quantum to classical regime may be tuned by controlling the intensities of the seeds and detected by intensity measurements. Besides, we show that the thresholds are not affected by losses, which only modify the amount of nonclassicality. The multimode case is also analyzed in some detail.
Parametric downconversion (PDC) is a technique of ubiquitous experimental significance in the production of non-classical, photon-number correlated twin beams. Standard theory of PDC as a two-mode squeezing process predicts and homodyne measurements observe a thermal photon number distribution per beam. Recent experiments have obtained conflicting distributions. In this paper, we explain the observation by an a-priori theoretical model solely based on directly accessible physical quantities. We compare our predictions with experimental data and find excellent agreement.
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