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Register a new userA new approach to monitor 13C-targets degradation in situ for 13C(alpha,n)16O cross-section measurements at LUNA
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Giovanni Francesco Ciani Dr
Publication date
2020
fields
Physics
and research's language is
English
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Direct measurements of reaction cross-sections at astrophysical energies often require the use of solid targets able to withstand high ion beam currents for extended periods of time. Thus, monitoring target thickness, isotopic composition, and target stoichiometry during data taking is critical to account for possible target modifications and to reduce uncertainties in the final cross-section results. A common technique used for these purposes is the Nuclear Resonant Reaction Analysis (NRRA), which however requires that a narrow resonance be available inside the dynamic range of the accelerator used. In cases when this is not possible, as for example the 13C(alpha,n)16O reaction recently studied at low energies at the Laboratory for Underground Nuclear Astrophysics (LUNA) in Italy, alternative approaches must be found. Here, we present a new application of the shape analysis of primary gamma rays emitted by the 13C(p,g)14N radiative capture reaction. This approach was used to monitor 13C target degradation {em in situ} during the 13C(alpha,n)16O data taking campaign. The results obtained are in agreement with evaluations subsequently performed at Atomki (Hungary) using the NRRA method. A preliminary application for the extraction of the 13C(alpha,n)16O reaction cross-section at one beam energy is also reported.
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At the n_TOF experiment at CERN a dedicated single-crystal chemical vapor deposition (sCVD) Diamond Mosaic-Detector has been developed for (n,$alpha$) cross-section measurements. The detector, characterized by an excellent time and energy resolution, consists of an array of 9 sCVD diamond diodes. The detector has been characterized and a cross-section measurement has been performed for the $^{59}$Ni(n,$alpha$)$^{56}$Fe reaction in 2012. The characteristics of the detector, its performance and the promising preliminary results of the experiment are presented.
The absolute cross section of the $^{13}$C($alpha$,n)$^{16}$O reaction has been measured at E$_{alpha}$ = 0.8 to 8.0 MeV with an overall accuracy of 4%. The precision is needed to subtract reliably a background in the observation of geo-neutrinos, e.g. in the KamLAND detector.
We present a new measurement of the $alpha$-spectroscopic factor ($S_alpha$) and the asymptotic normalization coefficient (ANC) for the 6.356 MeV 1/2$^+$ subthreshold state of $^{17}$O through the $^{13}$C($^{11}$B, $^{7}$Li)$^{17}$O transfer reaction and we determine the $alpha$-width of this state. This is believed to have a strong effect on the rate of the $^{13}$C($alpha$, $n$)$^{16}$O reaction, the main neutron source for {it slow} neutron captures (the $s$-process) in asymptotic giant branch (AGB) stars. Based on the new width we derive the astrophysical S-factor and the stellar rate of the $^{13}$C($alpha$, $n$)$^{16}$O reaction. At a temperature of 100 MK our rate is roughly two times larger than that by citet{cau88} and two times smaller than that recommended by the NACRE compilation. We use the new rate and different rates available in the literature as input in simulations of AGB stars to study their influence on the abundances of selected $s$-process elements and isotopic ratios. There are no changes in the final results using the different rates for the $^{13}$C($alpha$, $n$)$^{16}$O reaction when the $^{13}$C burns completely in radiative conditions. When the $^{13}$C burns in convective conditions, as in stars of initial mass lower than $sim$2 $M_sun$ and in post-AGB stars, some changes are to be expected, e.g., of up to 25% for Pb in our models. These variations will have to be carefully analyzed when more accurate stellar mixing models and more precise observational constraints are available.
Low mass Asymptotic Giant Branch stars are among the most important polluters of the interstellar medium. In their interiors, the main component (A>90) of the slow neutron capture process (the s-process) is synthesized, the most important neutron source being the 13C(alpha,n)16O reaction. In this paper we review its current experimental status discussing possible future synergies between some experiments currently focused on the determination of its rate. Moreover, in order to determine the level of precision needed to fully characterize this reaction, we present a theoretical sensitivity study, carried out with the FUNS evolutionary stellar code and the NEWTON post-process code. We modify the rate up to a factor of two with respect to a reference case. We find that variations of the 13C(alpha,n)16O rate do not appreciably affect s-process distributions for masses above 3 Msun at any metallicity. Apart from a few isotopes, in fact, the differences are always below 5%. The situation is completely different if some 13C burns in a convective environment: this occurs in FUNS models with M<3 Msun at solar-like metallicities. In this case, a change of the 13C(alpha,n)16O reaction rate leads to non-negligible variations of the elements Surface distribution (10% on average), with larger peaks for some elements (as rubidium) and for neutron-rich isotopes (as 86Kr and 96Zr). Larger variations are found in low-mass low-metallicity models, if protons are mixed and burnt at very high temperatures. In this case, the surface abundances of the heavier elements may vary by more than a factor 50.
The general properties needed in targets (sources) for high precision, high accuracy measurements are reviewed. The application of these principles to the problem of developing targets for the Fission TPC is described. Longer term issues, such as the availability of actinide materials, improved knowledge of energy losses and straggling and the stability of targets during irradiation are also discussed.
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