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Broadband Ultrahigh-Resolution chip-scale Scanning Soliton Dual-Comb Spectroscopy

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 Added by Tong Lin
 Publication date 2020
  fields Physics
and research's language is English




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We present a chip-scale scanning dual-comb spectroscopy (SDCS) approach for broadband ultrahigh-resolution spectral acquisition. SDCS uses Si3N4 microring resonators that generate two single soliton micro-combs spanning 37 THz (300 nm) on the same chip from a single 1550-nm laser, forming a high-mutual-coherence dual-comb. We realize continuous tuning of the dual-comb system over the entire optical span of 37.5 THz with high precision using integrated microheater-based wavelength trackers. This continuous wavelength tuning is enabled by simultaneous tuning of the laser frequency and the two single soliton micro-combs over a full free spectral range of the microrings. We measure the SDCS resolution to be 319+-4.6 kHz. Using this SDCS system, we perform the molecular absorption spectroscopy of H13C14N over its 2.3 THz (18 nm)-wide overtone band, and show that the massively parallel heterodyning offered by the dual-comb expands the effective spectroscopic tuning speed of the laser by one order of magnitude. Our chip-scale SDCS opens the door to broadband spectrometry and massively parallel sensing with ultrahigh spectral resolution.



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Dissipative Kerr-microresonator soliton combs (hereafter called soliton combs) are promising to realize chip scale integration of full soliton comb systems providing high precision, broad spectral coverage and a coherent link to the micro/mm/THz domain with diverse applications coming on line all the time. However, the large soliton comb spacing hampers some applications. For example, for spectroscopic applications, there are simply not enough comb lines available to sufficiently cover almost any relevant absorption features. Here, we overcome this limitation by scanning the comb mode spacing by employing PDH locking and a microheater on the microresonator, showing continuous scanning of the soliton comb modes across nearly the full FSR of the microresonator without losing soliton operation, while spectral features with a bandwidth of as small of 5 MHz are resolved. Thus, comb mode scanning allows to cover the whole comb mode spectrum of tens of THz bandwidth with only one chip-scale comb.
We demonstrate fiber mode-locked dual frequency comb spectroscopy for broadband, high resolution measurements in a rapid compression machine (RCM). We apply an apodization technique to improve the short-term signal-to-noise-ratio (SNR), which enables broadband spectroscopy at combustion-relevant timescales. We measure the absorption on 24345 individual wavelength elements (comb teeth) between 5967 and 6133 cm-1 at 704 microsecond time resolution during a 12-ms compression of a CH4-N2 mixture. We discuss the effect of the apodization technique on the absorption spectra, and apply an identical effect to the spectral model during fitting to recover the mixture temperature. The fitted temperature is compared against an adiabatic model, and found to be in good agreement with expected trends. This work demonstrates the potential of DCS to be used as an in situ diagnostic tool for broadband, high resolution, measurements in engine-like environments.
We demonstrate seamless channel multiplexing and high bitrate superchannel transmission of coherent optical orthogonal-frequency-division-multiplexing (CO-OFDM) data signals utilizing a dissipative Kerr soliton (DKS) frequency comb generated in an on-chip microcavity. Aided by comb line multiplication through Nyquist pulse modulation, the high stability and mutual coherence among mode-locked Kerr comb lines are exploited for the first time to eliminate the guard intervals between communication channels and achieve full spectral density bandwidth utilization. Spectral efficiency as high as 2.625 bit/Hz/s is obtained for 180 CO-OFDM bands encoded with 12.75 Gbaud 8-QAM data, adding up to total bitrate of 6.885 Tb/s within 2.295 THz frequency comb bandwidth. Our study confirms that high coherence is the key superiority of Kerr soliton frequency combs over independent laser diodes, as a multi-spectral coherent laser source for high-bandwidth high-spectral-density transmission networks.
We present a novel compact dual-comb source based on a monolithic optical crystalline MgF$_2$ multi-resonator stack. The coherent soliton combs generated in two microresonators of the stack with the repetition rate of 12.1 GHz and difference of 1.62 MHz provided after heterodyning a 300 MHz wide radio-frequency comb. Analogous system can be used for dual-comb spectroscopy, coherent LIDAR applications and massively parallel optical communications.
Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the chip scale. However, the need to precisely match the resonance wavelengths of distinct high-quality-factor microcavities has hindered the development of an on-chip dual comb source. Here, we report the first simultaneous generation of two microresonator combs on the same chip from a single laser. The combs span a broad bandwidth of 51 THz around a wavelength of 1.56 $mu$m. We demonstrate low-noise operation of both frequency combs by deterministically tuning into soliton mode-locked states using integrated microheaters, resulting in narrow ($<$ 10 kHz) microwave beatnotes. We further use one mode-locked comb as a reference to probe the formation dynamics of the other comb, thus introducing a technique to investigate comb evolution without auxiliary lasers or microwave oscillators. We demonstrate broadband high-SNR absorption spectroscopy of dichloromethane spanning 170 nm using the dual comb source over a 20 $mu$s acquisition time. Our device paves the way for compact and robust dual-comb spectrometers at nanosecond timescales.
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