Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userDistribution of the magnetic environment in charge ordered La$_{1.885}$Sr$_{0.115}$CuO$_{4}$
149
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
We report the inverse Laplace transform (ILT) analysis of the $^{139}$La nuclear spin-lattice relaxation rate $1/T_1$ in charge ordered La$_{1.885}$Sr$_{0.115}$CuO$_4$ ($T_{charge} sim 80$K, $T_{c} simeq T_{spin}^{neutron}=30$K), and shed new light on its magnetic inhomogeneity. We deduce the probability density function $P(1/T_{1})$ of the distributed $1/T_1$ (i.e. the histogram of distributed $1/T_1$) by taking the inverse Laplace transform of the experimentally observed nuclear magnetization recovery curve $M(t)$. We demonstrate that spin freezing sets in in some domains precisely below the onset of charge order at $T_{charge}$, but their volume fraction grows only gradually toward $T_{c}$. Nearly a half of the sample volume exhibits properties expected for canonical high $T_c$ cuprates without charge order even near $T_c$. Our findings explain why charge order does not suppress $T_c$ of La$_{1.885}$Sr$_{0.115}$CuO$_4$ as significantly as in La$_{1.875}$Ba$_{0.125}$CuO$_4$.
rate research
Read More
The presence of charge and spin stripe order in the La2CuO4-based family of superconductors continues to lead to new insight on the unusual ground state properties of high Tc cuprates. Soon after the discovery of charge stripe order at T(charge)=65K in Nd3+ co-doped LSCO ($T_{c}simeq6$~K) [Tranquada et al., Nature {bf 375} (1995) 561], Hunt et al. demonstrated that La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$ and superconducting LSCO with x~1/8 (Tc ~ 30K) share nearly identical NMR anomalies near $T_{charge}$ of the former [Phys. Rev. Lett. {bf 82} (1999) 4300]. Their inevitable conclusion that LSCO also undergoes charge order at a comparable temperature became controversial, because diffraction measurements at the time were unable to detect Bragg peaks associated with charge order. Recent advances in x-ray diffraction techniques finally led to definitive confirmations of the charge order Bragg peaks in LSCO with an onset at as high as T(charge)=80K. Meanwhile, improved instrumental technology has enabled routine NMR measurements that were not feasible two decades ago. Motivated by these new developments, we revisit the charge order transition of a LSCO single crystal based on 63Cu NMR techniques. We demonstrate that 63Cu NMR properties of the nuclear spin $I_{z}$ = -1/2 to +1/2 central transition below T(charge) exhibit unprecedentedly strong dependence on the measurement time scale set by the NMR pulse separation time $tau$; a new kind of anomalous, very broad wing-like 63Cu NMR signals gradually emerge below T(charge) only for extremely short $tau lesssim 4~mu$s, while the spectral weight of the normal NMR signals is progressively wiped out. The NMR linewidth and relaxation rates depend strongly on $tau$ below T(charge), and their enhancement in the charge ordered state indicates that charge order turns on strong but inhomogeneous growth of Cu spin-spin correlations.
We present results of magnetic neutron diffraction experiments on the co-doped super-oxygenated La(2-x)Sr(x)CuO(4+y) (LSCO+O) system with x=0.09. The spin-density wave has been studied and we find long-range incommensurate antiferromagnetic order below T_N coinciding with the superconducting ordering temperature T_c=40 K. The incommensurability value is consistent with a hole-doping of n_h~1/8, but in contrast to non-superoxygenated La(2-x)Sr(x)CuO(4) with hole-doping close to n_h ~ 1/8 the magnetic order parameter is not field-dependent. We attribute this to the magnetic order being fully developed in LSCO+O as in the other striped lanthanum-cuprate systems.
By using new and previous measurements of the $ab$-plane conductivity $sigma_1^{ab} (omega,T)$ of La$_{2-x}$Sr$_x$CuO$_{4}$ (LSCO) it is shown that the spectral weight $W = int_0^Omega {sigma_1^{ab} (omega,T) domega}$ obeys the same law $W = W_0 - B(Omega) T^2$ which holds for a conventional metal like gold, for $Omega$s below the plasma frequency. However $B(Omega)$, which measures the thermal response of the charge system, in LSCO exhibits a peculiar behavior which points towards correlation effects. In terms of hopping models, $B(Omega)$ is directly related to an energy scale $t_T$, smaller by one order of magnitude than the full bandwidth $t_0 sim W_0$.
We show that disruption of charge-density-wave (stripe) order by charge transfer excitation, enhances the superconducting phase rigidity in La_{1.885}Ba_{0.115}CuO_4 (LBCO). Time-Resolved Resonant Soft X-Ray Diffraction demonstrates that charge order melting is prompt following near-infrared photoexcitation whereas the crystal structure remains intact for moderate fluences. THz time-domain spectroscopy reveals that, for the first 2 ps following photoexcitation, a new Josephson Plasma Resonance edge, at higher frequency with respect to the equilibrium edge, is induced indicating enhanced superconducting interlayer coupling. The fluence dependence of the charge-order melting and the enhanced superconducting interlayer coupling are correlated with a saturation limit of about 0.5 mJ/cm2. Using a combination of x-ray and optical spectroscopies we establish a hierarchy of timescales between enhanced superconductivity, melting of charge order and rearrangement of the crystal structure.
We investigate the hole and lattice dynamics in a prototypical high temperature superconducting system La{2-x}Sr{x}CuO{4} using infrared spectroscopy. By exploring the anisotropy in the electronic response of CuO2 planes we show that our results support the notion of stripes. Nevertheless, charge ordering effects are not apparent in the phonon spectra. All crystals show only the expected infrared active modes for orthorhombic phases without evidence for additional peaks that may be indicative of static charge ordering. Strong electron-phonon interaction manifests itself through the Fano lineshape of several phonon modes. This analysis reveals anisotropic electron-phonon coupling across the phase diagram, including superconducting crystals. Due to the ubiquity of the CuO2 plane, these results may have implications for other high Tc superconductors.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
