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Register a new userMultiple photodetachment of carbon anions via single and double core-hole creation
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We report on new measurements of m-fold photodetachment (m=2-5) of carbon anions via K-shell excitation and ionization. The experiments were carried out employing the photon-ion merged-beams technique at a synchrotron light source. While previous measurements were restricted to double detachment (m=2) and to just the lowest-energy K-shell resonance at about 282 eV, our absolute experimental $m$-fold detachment cross sections at photon energies of up to 1000 eV exhibit a wealth of new thresholds and resonances. We tentatively identify these features with the aid of detailed atomic-structure calculations. In particular, we find unambiguous evidence for fivefold detachment via double K-hole production.
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Photodetachment thermometry on a beam of OH$^-$ in a cryogenic storage ring cooled to below 10 K is carried out using two-dimensional, frequency and time dependent photodetachment spectroscopy over 20 minutes of ion storage. In equilibrium with the low-level blackbody field, we find an effective radiative temperature near 15 K with about 90% of all ions in the rotational ground state. We measure the J = 1 natural lifetime (about 193 s) and determine the OH$^-$ rotational transition dipole moment with 1.5% uncertainty. We also measure rotationally dependent relative near-threshold photodetachment cross sections for photodetachment thermometry.
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This article studies the photodetachment of a single electron anion near an attractive center. Both the differential and total photodetachment cross section are analysed. We obtain the electron flux crossing through a spherical detector centered at the force center using the semiclassical approximation. The closed-orbit theory gives the total cross section which contains a smooth background and an oscillatory part. Concrete calculations and discussions are carried out for two types of wave source: the $s$- and $p_z$-wave source. Photodetachment processes for three conditions are compared: an anion near an attractive center, near a repulsive center and in a homogeneous electric field.
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We propose to use the near-threshold electron scattering data for atoms to guide the reliable experimental determination of their electron affinities (EAs), extracted using the Wigner Threshold Law, from laser photodetachment threshold spectroscopy measurements. Data from the near-threshold electron elastic scattering from W, Te, Rh, Sb and Sn atoms calculated using our complex angular momentum method, wherein is embedded the electron-electron correlations and core polarization interaction, are used as illustrations. We conclude with a remark on the relativistic effects on the EA calculation for the heavy At atom.
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