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Register a new userNoise in stimulated Raman scattering measurement: From basics to practice
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Xavier Audier
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We revisit laser intensity noise in the context of stimulated Raman scattering (SRS), which has recently proved to be a key technique to provide label free images of chemical bonds in biological and medical samples. Contrary to most microscopy techniques, which detect a weak photon flux resulting from light matter interactions, SRS is a pump-probe scheme that works in the high flux regime and happens as a weak modulation ($10^{-4}-10^{-6}$) in a strong laser field. As a result, laser noise is a key issue in SRS detection. This practical tutorial provides the experimentalists with the tools required to assess the amount of noise and the ultimate SRS detection limit in a conventional lock-in-based SRS system. We first define the quantities that are relevant when discussing intensity noise, and illustrate them through a conventional model of light detection by a photodiode. Stimulated Raman Scattering is then introduced in its lock-in-based implementation, and the model presented is adapted in this particular case. The power spectral density (PSD), relative intensity noise (RIN), signal to noise ratio (SNR), and sensitivity of the system are derived and discussed. Two complementary methods are presented that allow measurement of the RIN and assessment of the performance of a SRS system. Such measurements are illustrated on two commercial laser systems. Finally, the consequences of noise in SRS are discussed, and future developments are suggested. The presentation is made simple enough for under-graduated, graduated students, and newcomers in the field of stimulated Raman, and more generally in pump-probe based schemes.
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Stimulated Raman scattering (SRS) in plasma in a non-eigenmode regime is studied theoretically and numerically. Different from normal SRS with the eigen electrostatic mode excited, the non-eigenmode SRS is developed at plasma density $n_e>0.25n_c$ when the laser amplitude is larger than a certain threshold. To satisfy the phase-matching conditions of frequency and wavenumber, the excited electrostatic mode has a constant frequency around half of the incident light frequency $omega_0/2$, which is no longer the eigenmode of electron plasma wave $omega_{pe}$. Both the scattered light and the electrostatic wave are trapped in plasma with their group velocities being zero. Super hot electrons are produced by the non-eigen electrostatic wave. Our theoretical model is validated by particle-in-cell simulations. The SRS driven in this non-eigenmode regime may play a considerable role in the experiments of laser plasma interactions as long as the laser intensity is higher than $10^{15}$W/cm$^2$.
A simple physical mechanism of stimulated light scattering on nanoscale objects in water suspension similar to Langmuir waves mechanism in plasma is proposed. The proposed mechanism is based on a dipole interaction between the light wave and the non-compensated electrical charge that inevitably exists on a nanoscale object (a virus or a nanoparticle) in water environment. The experimental data for tobacco mosaic virus and polystyrene nanospheres are presented to support the suggested physical mechanism. It has been demonstrated that stimulated amplification spectral line frequencies observed experimentally are well explained by the suggested mechanism. In particular, the absence of lower frequency lines and the generation lines shift when changing the pH are due to ion friction appearing in the ionic solution environment. The selection rules observed experimentally also confirm the dipole interaction type. It has been shown that microwave radiation on nanoscale object acoustic vibrations frequency should appear under such scattering conditions. We demonstrate that such conditions also allow for local selective heating of nanoscale objects by dozens to hundreds degrees K. This effect is controlled by the optical irradiation parameters and can be used for affecting selectively certain types of viruses.
It is known that photon pairs generated from pulse-pumped spontaneous parametric processes can be described by independent temporal modes and form a multi-temporal mode entangled state. However, the exact form of the temporal modes is not known even though the joint spectral intensity of photon pairs can be measured by the method of stimulated emission tomography. In this paper, we describe a feedback-iteration method which, combined with the stimulated emission method, can give rise to the exact forms of the independent temporal modes for the temporally entangled photon pairs.
Stimulated low-frequency Raman scattering can give essential information about the elastic properties of different nanoparticles systems, in particular, biological nanostructures. In the present study, low-frequency vibrational modes in human and bovine serum albumin were for the first time investigated using stimulated low-frequency Raman scattering. Stimulated low-frequency Raman scattering frequency shifts, corresponding to acoustic eigenfrequencies of the sample, were registered by Fabri-Perot interferometers. Conversion efficiency, threshold and set of eigenfrequencies were also measured. Stimulated low-frequency Raman scattering can be applied for biological objects identification and impact on them.
We introduce a scattering-type scanning near-field infrared microscope (s-SNIM) for the local scale near- field sample analysis and spectroscopy from room (RT) down to liquid helium (LHe) temperatures. The extension of s-SNIM down to T = 5K is in particular crucial for low-temperature phase transitions, e.g. for the examination of superconductors, as well as low energy excitations. The LT s-SNIM performance is tested with CO2-IR excitation at T = 7K using a bare Au reference and a structured Si/SiO$_2$-sample. Furthermore, we quantify the impact of local laser heating under the s-SNIM tip apex by monitoring the light-induced ferroelectric-to-paraelectric phase transition of the skyrmion-hosting multiferroic material GaV4S8 at T$_c$ = 42K. We apply LT s-SNIM to study the spectral response of GaV$_4$S$_8$ and its lateral domain structure in the ferroelectric phase by the mid-IR to THz free-electron laser-light source FELBE at the Helmholtz-Zentrum Dresden-Rossendorf, Germany. Notably, our s-SNIM is based on a non-contact atomic force microscope(AFM), and thus can be complemented in-situ by various other AFM techniques, such as topography profiling, piezo-response force microscopy (PFM) and/or Kelvin-probe force microscopy (KPFM). The combination of these methods support the comprehensive study of the mutual interplay in the topographic, electronic and optical properties of surfaces from room temperature down to 5K.
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