No Arabic abstract
In a recent experiment [A. Donarini et al., Nat Comms 10, 381 (2019)], electronic transport through a carbon nanotube quantum dot was observed to be suppressed by the formation of a quantum-coherent ``dark state. In this paper we consider theoretically the counting statistics and waiting-time distribution of this dark-state-limited transport. We show that the statistics are characterised by giant super-Poissonian Fano factors and long-tailed waiting-time distributions, both of which are signatures of the bistability and extreme electron bunching caused by the dark state.
Illumination of atoms by resonant lasers can pump electrons into a coherent superposition of hyperfine levels which can no longer absorb the light. Such superposition is known as dark state, because fluorescent light emission is then suppressed. Here we report an all-electric analogue of this destructive interference effect in a carbon nanotube quantum dot. The dark states are a coherent superposition of valley (angular momentum) states which are decoupled from either the drain or the source leads. Their emergence is visible in asymmetric current-voltage characteristics, with missing current steps and current suppression which depend on the polarity of the applied source-drain bias. Our results demonstrate for the first time coherent-population trapping by all-electric means in an artificial atom.
We theoretically study the conditional counting statistics of electron transport through a system consisting of a single quantum dot (SQD) or coherently coupled double quantum dots (DQDs) monitored by a nearby quantum point contact (QPC) using the generating functional approach with the maximum eigenvalue of the evolution equation matrix method, the quantum trajectory theory method (Monte Carlo method), and an efficient method we develop. The conditional current cumulants that are significantly different from their unconditional counterparts can provide additional information and insight into the electron transport properties of mesoscopic nanostructure systems. The efficient method we develop for calculating the conditional counting statistics is numerically stable, and is capable of calculating the conditional counting statistics for a more complex system than the maximum eigenvalue method and for a wider range of parameters than the quantum trajectory method. We apply our method to investigate how the QPC shot noise affects the conditional counting statistics of the SQD system, going beyond the treatment and parameter regime studied in the literature. We also investigate the case when the interdot coherent coupling is comparable to the dephasing rate caused by the back action of the QPC in the DQD system, in which there is considerable discrepancy in the calculated conditional current cumulants between the population rate (master-) equation approach of sequential tunneling and the full quantum master-equation approach of coherent tunneling.
We demonstrate single-electron pumping in a gate-defined carbon nanotube double quantum dot. By periodic modulation of the potentials of the two quantum dots we move the system around charge triple points and transport exactly one electron or hole per cycle. We investigate the pumping as a function of the modulation frequency and amplitude and observe good current quantization up to frequencies of 18 MHz where rectification effects cause the mechanism to break down.
Quantum sensing exploits fundamental features of quantum mechanics and quantum control to realise sensing devices with potential applications in a broad range of scientific fields ranging from basic science to applied technology. The ultimate goal are devices that combine unprecedented sensitivity with excellent spatial resolution. Here, we propose a new platform for all-electric nanoscale quantum sensing based on a carbon nanotube double quantum dot. Our analysis demonstrates that the platform can achieve sensitivities that allow for the implementation of single-molecule magnetic resonance spectroscopy and therefore opens a promising route towards integrated on-chip quantum sensing devices.
We systematically study the coupling of longitudinal modes (shells) in a carbon nanotube quantum dot. Inelastic cotunneling spectroscopy is used to probe the excitation spectrum in parallel, perpendicular and rotating magnetic fields. The data is compared to a theoretical model including coupling between shells, induced by atomically sharp disorder in the nanotube. The calculated excitation spectra show good correspondence with experimental data.