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Register a new userStability of Big Surface Bubbles: Impact of Evaporation and Bubbles Size
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Surface bubbles have attracted much interest in the past decades. In this article, we propose to explore the lifetime and thinning dynamics of centimetric surface bubbles. We study the impact of the bubbles size as well as that of the atmospheric humidity through a careful control and systematic variation of the relative humidity in the measuring chamber. We first adress the question of the drainage under saturated water vapor conditions and show that a model including both capillary and gravity driven drainage provides the best prediction for this process. Additionally, unprecedented statistics on the bubbles lifetimes confirm experimentally that this parameter is set by evaporation to leading order. We make use of a model based on the overall thinning dynamics of the thin film and assume a rupture thickness of the order 10-100 nm to obtain a good representation of these data. For experiments conducted far from saturation, the convective evaporation of the bath is shown to dominate the overall mass loss in the cap film due to evaporation.
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The addition of sweeteners in fizzy beverages not only affects the sugar content but also the bubbles stability. In this article, we propose a model experiment, in which the lifetime of hundreds of single bubbles is measured, to assess the stability of bubbles in solutions containing either sucrose or sweeteners. We show that the bubbles are indeed more stable in presence of sweeteners, which are surface active molecules and adsorb at the interface. Additionally, we test an antifoam at different concentrations and show that our experiment allows to identify the best concentration to reproduce the stability obtained in sucrose when we replace this latter by a sweetener.
Soap bubbles are by essence fragile and ephemeral. Depending on their composition and environment, bubble bursting can be triggered by gravity-induced drainage and/or the evaporation of the liquid and/or the presence of nuclei. In this paper, we design bubbles made of a composite liquid shell able to neutralize all these effects and keep their integrity in a standard atmosphere. This composite material is obtained in a simple way by replacing surfactants by partially-wetting microparticles and water by a water/glycerol mixture. A nonlinear model able to predict the evolution of these composite bubbles toward an equilibrium state is proposed and quantitatively compared to experimental data. This work unveils a composite liquid film with unique robustness, which can easily be manufactured to design complex objects.
We study the excess free energy due to phase coexistence of fluids by Monte Carlo simulations using successive umbrella sampling in finite LxLxL boxes with periodic boundary conditions. Both the vapor-liquid phase coexistence of a simple Lennard-Jones fluid and the coexistence between A-rich and B-rich phases of a symmetric binary (AB) Lennard-Jones mixture are studied, varying the density rho in the simple fluid or the relative concentration x_A of A in the binary mixture, respectively. The character of phase coexistence changes from a spherical droplet (or bubble) of the minority phase (near the coexistence curve) to a cylindrical droplet (or bubble) and finally (in the center of the miscibility gap) to a slab-like configuration of two parallel flat interfaces. Extending the analysis of M. Schrader, P. Virnau, and K. Binder [Phys. Rev. E 79, 061104 (2009)], we extract the surface free energy gamma (R) of both spherical and cylindrical droplets and bubbles in the vapor-liquid case, and present evidence that for R -> Infinity the leading order (Tolman) correction for droplets has sign opposite to the case of bubbles, consistent with the Tolman length being independent on the sign of curvature. For the symmetric binary mixture the expected non-existence of the Tolman length is confirmed. In all cases {and for a range of radii} R relevant for nucleation theory, gamma(R) deviates strongly from gamma (Infinity) which can be accounted for by a term of order gamma(Infinity)/gamma(R)-1 ~ 1/R^2. Our results for the simple Lennard-Jones fluid are also compared to results from density functional theory and we find qualitative agreement in the behavior of gamma(R) as well as in the sign and magnitude of the Tolman length.
We study multielectron bubble phases in the $N=2$ and $N=3$ Landau levels in a high mobility GaAs/AlGaAs sample. We found that the longitudinal magnetoresistance versus temperature curves in the multielectron bubble region exhibit sharp peaks, irrespective of the Landau level index. We associate these peaks with an enhanced scattering caused by thermally fluctuating domains of a bubble phase and a uniform uncorrelated electron liquid at the onset of the bubble phases. Within the $N=3$ Landau level, onset temperatures of three-electron and two-electron bubbles exhibit linear trends with respect to the filling factor; the onset temperatures of three-electron bubbles are systematically higher than those of two-electron bubbles. Furthermore, onset temperatures of the two-electron bubble phases across $N=2$ and $N=3$ Landau levels are similar, but exhibit an offset. This offset and the dominant nature of the three-electron bubbles in the $N=3$ Landau level reveals the role of the short-range part of the electron-electron interaction in the formation of the bubbles.
The prediction of the lifetime of surface bubbles necessitates a better understanding of the thinning dynamics of the bubble cap. In 1959, Mysel textit{et al.} cite{mysels1959soap}, proposed that textit{marginal regeneration} i.e. the rise of patches, thinner than the film should be taken into account to describe the film drainage. Nevertheless, an accurate description of these buoyant patches and of their dynamics as well as a quantification of their contribution to the thinning dynamics is still lacking. In this paper, we visualize the patches, and show that their rising velocities and sizes are in good agreement with models respectively based on the balance of gravitational and surface viscous forces and on a Rayleigh-Taylor like instability cite{Seiwert2017,Shabalina2019}. Our results suggest that, in an environment saturated in humidity, the drainage induced by their dynamics correctly describes the film drainage at the apex of the bubble within the experimental error bars. We conclude that the film thinning of soap bubbles is indeed controlled, to a large extent, by textit{marginal regeneration} in the absence of evaporation.
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