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Register a new userTwo Neutron Correlation Study in Photofission of Actinides
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Roman V. Shapovalov
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It is well known that two fission fragments (FFs) are emitted essentially back to back in the laboratory frame. That can be used widely in many applications as a unique signature of fissionable materials. However, such fission fragments are difficult to detect. The energy and angular distributions of neutrons, on the other hand, are easy to measure, and that distribution will carry information about the fission fragments energy and angular spectra, as well as the neutron spectra in the fission fragment rest frame. We propose to investigate the two neutron correlation yield resulting from two FFs as a function of different targets, the angle between the two neutrons and the neutron energies. The preliminary calculation of the two neutron correlation shows a huge asymmetry effect: many more neutrons are emitted anti-parallel to each other than parallel to each other. That asymmetry becomes even more if the energy cut on each neutron is done. This study will potentially permit a new technique for actinide detection for homeland security and safeguards applications as well as improve our knowledge of correlated neutron emission.
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We have calculated the fission probabilities for 237-Np, 233,235,238-U, 232-Th, and nat-Pb following the absorption of photons with energies from 68 MeV to 3.77 GeV using the RELDIS Monte-Carlo code. This code implements the cascade-evaporation-fission model of intermediate-energy photonuclear reactions. It includes multiparticle production in photoreactions on intranuclear nucleons, pre-equilibrium emission, and the statistical decay of excited residual nuclei via competition of evaporation, fission, and multifragmentation processes. The calculations show that in the GeV energy region the fission process is not solely responsible for the entire total photoabsorption cross section, even for the actinides: ~55-70% for 232-Th, ~70-80% for 238-U, and ~80-95% for 233-U, 235-U, and 237-Np. This is because certain residual nuclei that are created by deep photospallation at GeV photon energies have relatively low fission probabilities. Using the recent experimental data on photofission cross sections for 237-Np and 233,235,238-U from the Saskatchewan and Jefferson Laboratories and our calculated fission probabilities, we infer the total photoabsorption cross sections for these four nuclei. The resulting cross sections per nucleon agree in shape and in magnitude with each other. However, disagreement in magnitude with total-photoabsorption cross-section data from previous measurements for nuclei from C to Pb calls into question the concept of a ``Universal Curve for the photoabsorption cross section per nucleon for all nuclei.
A new technique was developed to measure the lifetimes of neutron unbound nuclei in the picosecond range. The decay of 26O -> 24O+n+n was examined as it had been predicted to have an appreciable lifetime due to the unique structure of the neutron-rich oxygen isotopes. The half-life of 26O was extracted as 4.5^{+1.1}_{-1.5}(stat.) +/- 3 (sys.) ps. This corresponds to 26O having a finite lifetime at an 82% confidence level and, thus, suggests the possibility of two-neutron radioactivity.
The photofission cross-section of 238U was measured at sub-barrier energies as a function of the gamma-ray energy using, for the first time, a monochromatic, high-brilliance, Compton-backscattered gamma-ray beam. The experiment was performed at the High Intensity gamma-ray Source (HIgS) facility at beam energies between E=4.7 MeV and 6.0 MeV and with ~3% energy resolution. Indications of transmission resonances have been observed at gamma-ray beam energies of E=5.1 MeV and 5.6 MeV with moderate amplitudes. The triple-humped fission barrier parameters of 238U have been determined by fitting EMPIRE-3.1 nuclear reaction code calculations to the experimental photofission cross section.
The aCORN experiment uses a novel asymmetry method to measure the electron-antineutrino correlation (a-coefficient) in free neutron decay that does not require precision proton spectroscopy. aCORN completed two physics runs at the NIST Center for Neutron Research. The first run on the NG-6 beam line in 2013--2014 obtained the result a = 0.1090 +/- 0.0030 (stat) +/- 0.0028 (sys), a total uncertainty of 3.8%. The second run on the new NG-C high flux beam line promises an improvement in precision to <2%.
We have investigated experimentally the pressure dependence of the production of ultracold neutrons (UCN) in superfluid helium in the range from saturated vapor pressure to 20bar. A neutron velocity selector allowed the separation of underlying single-phonon and multiphonon pro- cesses by varying the incident cold neutron (CN) wavelength in the range from 3.5 to 10{AA}. The predicted pressure dependence of UCN production derived from inelastic neutron scattering data was confirmed for the single-phonon excitation. For multiphonon based UCN production we found no significant dependence on pressure whereas calculations from inelastic neutron scattering data predict an increase of 43(6)% at 20bar relative to saturated vapor pressure. From our data we conclude that applying pressure to superfluid helium does not increase the overall UCN production rate at a typical CN guide.
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