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Register a new userSuperconducting phase diagrams of LuB$_{12}$ and Lu$_{1-x}$Zr$_x$B$_{12}$ ($x le 0.45$) down to 50 mK
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Lutetium dodecaboride LuB12 is a simple weak-coupling BCS superconductor with critical temperature Tc = 0.42 K, whilst ZrB12 is a strong-coupling BCS superconductor with the highest critical temperature Tc = 6.0 K among this group of materials. In case of lutetium substitution by zirconium ions in LuB12 the crossover from weak- to strong-coupling superconductor can be studied. We have investigated the evolution of critical temperature Tc and critical field Hc in high-quality single crystalline superconducting samples of Lu(1-x)Zr(x)B12 (0 =< x =< 0.45) by measuring magnetic ac susceptibility between 1 K and 50 mK. To obtain this kind of experimental data, a new susceptometer was designed, constructed and tested, which can work in a wide temperature range of 0.05 K - 3 K in 3He-4He dilution refrigerator. The measurements with this new susceptometer revealed how Tc(x) and Hc(x) increases with increasing concentration of zirconium in Lu(1-x)Zr(x)B12 solid solutions as well as how their superconducting phase diagram develops.
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We have determined the superconducting and magnetic properties of four samples of Lu$_x$Zr$_{1-x}$B$_{12}$ ($x=0.04$, $0.07$, $0.17$, and $0.8$) using muon spin rotation ($mu$SR) and magnetometry measurements. We observed a strong magnetic signal in both the $mu$SR and magnetometry data in one sample ($x=0.07$), likely caused by the formation of static moments of size $approx 1,mu_{rm B}$ due to a clustering effect of the Lu$^{3+}$ ions. In all other samples, we find only a small magnetic signal in the $mu$SR data thought to originate from boron nuclei in the B$_{12}$ cages. The superconductivity is found to evolve with $x$, with a decrease in $x$ resulting in an increase in critical temperature and a decrease of the penetration depth. Most remarkably, we find the formation of nodes in the superconducting gap for $x leq 0.17$, providing a new example of an $s$-to-$d$-wave crossover in a superconductor.
We report measurements of the magnetic penetration depth $lambda$ in single crystals of Pr(Os$_{1-x}$Ru$_{x}$)$_{4}$Sb$_{12}$ down to 0.1 K. Both $lambda$ and superfluid density $rho_{s}$ exhibit an exponential behavior for the $x$$geq$0.4 samples, going from weak ($x$=0.4,0.6), to moderate, coupling ($x$=0.8). For the $x$$leq$0.2 samples, both $lambda$ and $rho_{s}$ vary as $T^{2}$ at low temperatures, but $rho_{s}$ is s-wave-like at intermediate to high temperatures. Our data are consistent with a three-phase scenario, where a fully-gapped phase at $T_{c1}$ undergoes two transitions: first to an unconventional phase at $T_{c2}$$lesssim$$T_{c1}$, then to a nodal low-$T$ phase at $T_{c3}$$<$$T_{c2}$, for small values of $x$.
Based on low temperature resistivity, heat capacity and magnetization investigations we show that the unusually strong suppression of superconductivity in Lu$_x$Zr$_{1-x}$B$_{12}$ BSC-type superconductors in the range $x$$<$0.08 is caused by the emergence of static spin polarization in the vicinity of non-magnetic lutetium impurities. The analysis of received results points to a formation of static magnetic moments with $mu_{eff}$$approx$$3mu_B$ per Lu-ion. The size of these spin polarized nanodomains was estimated to be about 5 ${AA}$.
The effects of pressure up to $sim 20$ kbar, on the structural phase transition of SrFe$_2$As$_2$ and lightly Sn-doped BaFe$_2$As$_2$, as well as on the superconducting transition temperature and upper critical field of (Ba$_{0.55}$K$_{0.45}$)Fe$_2$As$_2$ single crystals have been studied. All the transition temperatures decrease with pressure in an almost linear fashion. Under pressure, the upper critical field curve, $H_{c2}(T)$, for (Ba$_{0.55}$K$_{0.45}$)Fe$_2$As$_2$ shifts down in temperature to follow the zero field $T_c$ with very little change in slope. Composite $P - T$ phase diagrams for three parent compounds, AFe$_2$As$_2$ (A = Ba, Sr, Ca), are constructed and appear to be remarkably similar: (i) having a structural (antiferromagnetic) phase transition line with a negative slope and (ii) showing signs of the emerging superconducting state at intermediate pressures.
Resistivity measurements were performed on Pr$_{1-x}$La$_x$Os$_4$Sb$_{12}$ single crystals at temperatures down to 20 mK and in fields up to 18 T. The results for dilute-Pr samples ($x=0.3$ and 0.67) are consistent with model calculations performed assuming a singlet crystalline-electric-field (CEF) ground state. The residual resistivity of these crystals features a smeared step centered around 9 T, the predicted crossing field for the lowest CEF levels. The CEF contribution to the magnetoresistance has a weaker-than-calculated dependence on the field direction, suggesting that interactions omitted from the CEF model lead to avoided crossing in the effective levels of the Pr$^{3+}$ ion. The dome-shaped magnetoresistance observed for $x = 0$ and 0.05 cannot be reproduced by the CEF model, and likely results from fluctuations in the field-induced antiferroquadrupolar phase.
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