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When two lasers are applied to a non-centrosymmetric material, light can be generated at the difference of the incoming frequencies $Deltaomega$, a phenomenon known as difference frequency generation (DFG), well characterized in semiconductors. In this work, we derive a general expression for DFG in metals, which we use to show that the DFG in chiral topological semimetals under circular polarized light is quantized in units of $e^3/h^2$ and independent of material parameters, including the scattering time $tau$, when $Deltaomega gg tau^{-1}$. In this regime, DFG provides a simpler alternative to measure a quantized response in metals compared to previous proposals based on single frequency experiments. Our general derivation unmasks, in addition, a free-carrier contribution to the circular DFG beyond the semiclassical one. This contribution can be written as a Fermi surface integral, features strong frequency dependence, and oscillates with a $pi/2$ shift with respect to the quantized contribution. We make predictions for the circular DFG of chiral and non-chiral materials using generic effective models, and ab-initio calculations for TaAs and RhSi. Our work provides a complete picture of the DFG in the length gauge approach, in the clean, non-interacting limit, and highlights a plausible experiment to measure topologically quantizated photocurrents in metals.
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Topological semimetals, such as Dirac, Weyl, or line-node semimetals, are gapless states of matter characterized by their nodal band structures and surface states. In this work, we consider layered (topologically trivial) insulating systems in $D$ dimensions that are composed of coupled multi-layers of $d$-dimensional topological semimetals. Despite being nominal bulk insulators, we show that crystal defects having co-dimension $(D-d)$ can harbor robust lower dimensional topological semimetals embedded in a trivial insulating background. As an example we show that defect-bound topological semimetals can be localized on stacking faults and partial dislocations. Finally, we propose how an embedded topological Dirac semimetal can be identified in experiment by introducing a magnetic field and resolving the relativistic massless Dirac Landau level spectrum at low energies in an otherwise gapped system.
We review the recent, mainly theoretical, progress in the study of topological nodal line semimetals in three dimensions. In these semimetals, the conduction and the valence bands cross each other along a one-dimensional curve in the three-dimensional Brillouin zone, and any perturbation that preserves a certain symmetry group (generated by either spatial symmetries or time-reversal symmetry) cannot remove this crossing line and open a full direct gap between the two bands. The nodal line(s) is hence topologically protected by the symmetry group, and can be associated with a topological invariant. In this Review, (i) we enumerate the symmetry groups that may protect a topological nodal line; (ii) we write down the explicit form of the topological invariant for each of these symmetry groups in terms of the wave functions on the Fermi surface, establishing a topological classification; (iii) for certain classes, we review the proposals for the realization of these semimetals in real materials and (iv) we discuss different scenarios that when the protecting symmetry is broken, how a topological nodal line semimetal becomes Weyl semimetals, Dirac semimetals and other topological phases and (v) we discuss the possible physical effects accessible to experimental probes in these materials.
Dirac and Weyl semimetals, materials where electrons behave as relativistic fermions, react to position- and time-dependent perturbations, such as strain, as if emergent electromagnetic fields were applied. Since they differ from external electromagnetic fields in their symmetries and phenomenology they are called pseudo-electromagnetic fields, and enable a simple and unified description of a variety of inhomogeneous systems involving topological semimetals. We review the different physical ways to create effective pseudo-fields, their observable consequences as well as their similarities and differences compared to electromagnetic fields. Among these difference is their effect on quantum anomalies, the absence of a classical symmetry in the quantum theory, which we revisit from a quantum field theory and a semiclassical viewpoint. We conclude with predicted observable signatures of the pseudo-fields and the nascent experimental status.
We use first principles calculations to study the electronic properties of rock salt rare earth monopnictides La$X$ ($X=$N, P, As, Sb, Bi). A new type of topological band crossing termed `linked nodal rings is found in LaN when the small spin-orbital coupling (SOC) on nitrogen orbitals is neglected. Turning on SOC gaps the nodal rings at all but two points, which remain gapless due to $C_4$-symmetry and leads to a 3D Dirac semimetal. Interestingly, unlike LaN, compounds with other elements in the pnictogen group are found to be topological insulators (TIs), as a result of band reordering due to the increased lattice constant as well as the enhanced SOC on the pnictogen atom. These TI compounds exhibit multi-valley surface Dirac cones at three $bar{M}$-points on the $(111)$-surface.
Topological nodal line semimetals host stable chained, linked, or knotted line degeneracies in momentum space protected by symmetries. In this paper, we use the Jones polynomial as a general topological invariant to capture the global knot topology of the nodal lines. We show that every possible change in Jones polynomial is attributed to the local evolutions around every point where two nodal lines touch. As an application of our theory, we show that nodal chain semimetals with four touching points can evolve to a Hopf-link. We extend our theory to 3D non-Hermitian multi-band exceptional line semimetals.
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