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Register a new userStatistical properties of thermally expandable particles in soft Rayleigh-Benard convection
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The dynamics of inertial particles in Rayleigh-B{e}nard convection, where both particles and fluid exhibit thermal expansion, is studied using direct numerical simulations (DNS). We consider the effect of particles with a thermal expansion coefficient larger than that of the fluid, causing particles to become lighter than the fluid near the hot bottom plate and heavier than the fluid near the cold top plate. Because of the opposite directions of the net Archimedes force on particles and fluid, particles deposited at the plate now experience a relative force towards the bulk. The characteristic time for this motion towards the bulk to happen, quantified as the time particles spend inside the thermal boundary layers (BLs) at the plates, is shown to depend on the thermal response time, $tau_T$, and the thermal expansion coefficient of particles relative to that of the fluid, $K = alpha_p / alpha_f$. In particular, the residence time is constant for small thermal response times, $tau_T lesssim 1$, and increasing with $tau_T$ for larger thermal response times, $tau_T gtrsim 1$. Also, the thermal BL residence time is increasing with decreasing $K$. A one-dimensional (1D) model is developed, where particles experience thermal inertia and their motion is purely dependent on the buoyancy force. Although the values do not match one-to-one, this highly simplified 1D model does predict a regime of a constant thermal BL residence time for smaller thermal response times and a regime of increasing residence time with $tau_T$ for larger response times, thus explaining the trends in the DNS data well.
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The ordering of particles in the drying process of a colloidal suspension is crucial in determining the properties of the resulting film. For example, microscopic inhomogeneities can lead to the formation of cracks and defects that can deteriorate the quality of the film considerably. This type of problem is inherently multiscale and here we study it numerically, using our recently developed method for the simulation of soft polymeric capsules in multicomponent fluids. We focus on the effect of the particle softness on the film microstructure during the drying phase and how it relates to the formation of defects. We quantify the order of the particles by measuring both the Voronoi entropy and the isotropic order parameter. Surprisingly, both observables exhibit a non-monotonic behaviour when the softness of the particles is increased. We further investigate the correlation between the interparticle interaction and the change in the microstructure during the evaporation phase. We observe that the rigid particles form chain-like structures that tend to scatter into small clusters when the particle softness is increased.
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