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Register a new userDoping evolution of the charge excitations and electron correlations in electron-doped superconducting La$_{2-x}$Ce$_{x}$CuO$_{4}$
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Electron correlations play a dominant role in the charge dynamics of the cuprates. We use resonant inelastic x-ray scattering (RIXS) to track the doping dependence of the collective charge excitations in electron doped La$_{2-x}$Ce$_{x}$CuO$_{4}$(LCCO). From the resonant energy dependence and the out-of-plane momentum dependence, the charge excitations are identified as three-dimensional (3D) plasmons, which reflect the nature of the electronic structure and Coulomb repulsion on both short and long length scales. With increasing electron doping, the plasmon excitations show monotonic hardening in energy, a consequence of the electron correlation effect on electron structure near the Fermi surface (FS). Importantly, the plasmon excitations evolve from a broad feature into a well defined peak with much increased life time, revealing the evolution of the electrons from incoherent states to coherent quasi-particles near the FS. Such evolution marks the reduction of the short-range electronic correlation, and thus the softening of the Mottness of the system with increasing electron doping.
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High-transition-temperature (high-Tc) superconductivity develops near antiferromagnetic phases, and it is possible that magnetic excitations contribute to the superconducting pairing mechanism. To assess the role of antiferromagnetism, it is essential to understand the doping and temperature dependence of the two-dimensional antiferromagnetic spin correlations. The phase diagram is asymmetric with respect to electron and hole doping, and for the comparatively less-studied electron-doped materials, the antiferromagnetic phase extends much further with doping [1, 2] and appears to overlap with the superconducting phase. The archetypical electron-doped compound Nd{2-x}Ce{x}CuO{4pmdelta} (NCCO) shows bulk superconductivity above x approx 0.13 [3, 4], while evidence for antiferromagnetic order has been found up to x approx 0.17 [2, 5, 6]. Here we report inelastic magnetic neutron-scattering measurements that point to the distinct possibility that genuine long-range antiferromagnetism and superconductivity do not coexist. The data reveal a magnetic quantum critical point where superconductivity first appears, consistent with an exotic quantum phase transition between the two phases [7]. We also demonstrate that the pseudogap phenomenon in the electron-doped materials, which is associated with pronounced charge anomalies [8-11], arises from a build-up of spin correlations, in agreement with recent theoretical proposals [12, 13].
We used femtosecond optical pump-probe spectroscopy to study the photoinduced change in reflectivity of thin films of the electron-doped cuprate La$_{2-x}$Ce$_x$CuO$_4$ (LCCO) with dopings of x$=$0.08 (underdoped) and x$=$0.11 (optimally doped). Above T$_c$, we observe fluence-dependent relaxation rates which onset at a similar temperature that transport measurements first see signatures of antiferromagnetic correlations. Upon suppressing superconductivity with a magnetic field, it is found that the fluence and temperature dependence of relaxation rates is consistent with bimolecular recombination of electrons and holes across a gap (2$Delta_{AF}$) originating from antiferromagnetic correlations which comprise the pseudogap in electron-doped cuprates. This can be used to learn about coupling between electrons and high-energy ($omega>2Delta_{AF}$) excitations in these compounds and set limits on the timescales on which antiferromagnetic correlations are static.
The London penetration depth, lambda{ab}(T), is reported for thin films of the electron-doped superconductor Pr{2-x}Ce{x}CuO{4-y} at three doping levels (x = 0.13, 0.15 and 0.17). Measurements down to 0.35 K were carried out using a tunnel diode oscillator with excitation fields applied both perpendicular and parallel to the conducting planes. For all samples and both field orientations lambda{ab}(T) showed power law behavior implying a superconducting gap with nodes.
For electron-doped cuprates, the strong suppression of antiferromagnetic spin correlation by efficient reduction annealing by the protect-annealing method leads to superconductivity not only with lower Ce concentrations but also with higher transition temperatures. To reveal the nature of this superconducting state, we have performed angle-resolved photoemission spectroscopy measurements of protect-annealed electron-doped superconductors Pr$_{1.3-x}$La$_{0.7}$Ce$_{x}$CuO$_{4}$ and directly investigated the superconducting gap. The gap was found to be consistent with $d$-wave symmetry, suggesting that strong electron correlation persists and hence antiferromagnetic spin fluctuations remain a candidate that mediates Copper pairing in the protect-annealed electron-doped cuprates.
Magnetic excitations in the energy range up to 100 meV are studied for over-doped La$_{2-x}$Sr$_{x}$CuO$_{4}$ with $x=0.25$ and 0.30, using time-of-flight neutron spectroscopy. Comparison of spectra integrated over the width of an antiferromagnetic Brillouin zone demonstrates that the magnetic scattering at intermediate energies, $20 lesssim omega lesssim 100$ meV, progressively decreases with over-doping. This strongly suggests that the magnetism is not related to Fermi surface nesting, but rather is associated with a decreasing volume fraction of (probably fluctuating) antiferromagnetic bubbles.
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