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Register a new userOrbital-selective Kondo-lattice and enigmatic f-electrons emerging from inside the antiferromagnetic phase of a heavy fermion
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Novel electronic phenomena frequently form in heavy fermions as a consequence of the mutual nature of localization and itineracy of f electrons. On the magnetically ordered side of the heavy fermion phase diagram, f moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whether a Kondo lattice can develop inside the magnetically ordered phase. Using spectroscopic imaging with the scanning tunneling microscope, complemented by neutron scattering, x ray absorption spectroscopy, and dynamical mean field theory, we probe the electronic states in the antiferromagnetic USb2 as a function of temperature. We visualize a large gap in the antiferromagnetic phase at high temperatures, T lower than TN 200 K, within which Kondo hybridization gradually develops below Tcoh 80 K. Our dynamical mean field theory calculations indicate the antiferromagnetism and Kondo lattice to reside predominantly on different f orbitals, promoting orbital selectivity as a new conception into how these two phenomena coexist in heavy fermions. Finally, at Tstar 45 K we discover a novel 1st order like electronic transition through the abrupt emergence of non trivial 5f electronic states that may share some resemblance to the hidden order phase of URu2Si2.
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In heavy-fermion compounds, the dual character of $f$ electrons underlies their rich and often exotic properties like fragile heavy quasipartilces, variety of magnetic orders and unconventional superconductivity. 5$f$-electron actinide materials provide a rich setting to elucidate the larger and outstanding issue of the competition between magnetic order and Kondo entanglement and, more generally, the interplay among different channels of interactions in correlated electron systems. Here, by using angle-resolved photoemission spectroscopy, we present detailed electronic structure of USb$_2$ and observed two different kinds of nearly flat bands in the antiferromagnetic state of USb$_2$. Polarization-dependent measurements show that these electronic states are derived from 5$f$ orbitals with different characters; in addition, further temperature-dependent measurements reveal that one of them is driven by the Kondo correlations between the 5$f$ electrons and conduction electrons, while the other reflects the dominant role of the magnetic order. Our results on the low-energy electronic excitations of USb$_2$ implicate orbital selectivity as an important new ingredient for the competition between Kondo correlations and magnetic order and, by extension, in the rich landscape of quantum phases for strongly correlated $f$ electron systems.
In solids containing elements with f orbitals, the interaction between f-electron spins and those of itinerant electrons leads to the development of low-energy fermionic excitations with a heavy effective mass. These excitations are fundamental to the appearance of unconventional superconductivity and non-Fermi-liquid behaviour observed in actinide- and lanthanide-based compounds. Here we use spectroscopic mapping with the scanning tunnelling microscope to detect the emergence of heavy excitations with lowering of temperature in a prototypical family of cerium-based heavy-fermion compounds. We demonstrate the sensitivity of the tunnelling process to the composite nature of these heavy quasiparticles, which arises from quantum entanglement of itinerant conduction and f electrons. Scattering and interference of the composite quasiparticles is used to resolve their energy-momentum structure and to extract their mass enhancement, which develops with decreasing temperature. The lifetime of the emergent heavy quasiparticles reveals signatures of enhanced scattering and their spectral lineshape shows evidence of energy-temperature scaling. These findings demonstrate that proximity to a quantum critical point results in critical damping of the emergent heavy excitation of our Kondo lattice system.
Physical properties of polycrystalline CeCrGe$_{3}$ and LaCrGe$_{3}$ have been investigated by x-ray absorption spectroscopy, magnetic susceptibility $chi(T)$, isothermal magnetization M(H), electrical resistivity $rho(T)$, specific heat C($T$) and thermoelectric power S($T$) measurements. These compounds are found to crystallize in the hexagonal perovskite structure (space group textit{P6$_{3}$/mmc}), as previously reported. The $rho(T)$, $chi(T)$ and C($T$) data confirm the bulk ferromagnetic ordering of itinerant Cr moments in LaCrGe$_{3}$ and CeCrGe$_{3}$ with $T_{C}$ = 90 K and 70 K respectively. In addition a weak anomaly is also observed near 3 K in the C($T$) data of CeCrGe$_{3}$. The T dependences of $rho$ and finite values of Sommerfeld coefficient $gamma$ obtained from the specific heat measurements confirm that both the compounds are of metallic character. Further, the $T$ dependence of $rho$ of CeCrGe$_{3}$ reflects a Kondo lattice behavior. An enhanced $gamma$ of 130 mJ/mol,K$^{2}$ together with the Kondo lattice behavior inferred from the $rho(T)$ establish CeCrGe$_{3}$ as a moderate heavy fermion compound with a quasi-particle mass renormalization factor of $sim$ 45.
Strong electron correlations can give rise to extraordinary properties of metals with renormalized quasiparticles which are at the basis of Landaus Fermi liquid theory. Near a quantum critical point, these quasiparticles can be destroyed and non-Fermi liquid behavior ensues. YbRh$_2$Si$_2$ is a prototypical correlated metal as it exhibits quasiparticles formation, formation of Kondo lattice coherence and quasiparticle destruction at a field-induced quantum critical point. Here we show how, upon lowering the temperature, the Kondo lattice coherence develops and finally gives way to non-Fermi liquid electronic excitations. By measuring the single-particle excitations through scanning tunneling spectroscopy down to 0.3 K, we find the Kondo lattice peak emerging below the Kondo temperature $T_{rm K} sim$ 25 K, yet this peak displays a non-trivial temperature dependence with a strong increase around 3.3 K. At the lowest temperature and as a function of an external magnetic field, the width of this peak is minimized in the quantum critical regime. Our results provide a striking demonstration of the non-Fermi liquid electronic excitations in quantum critical metals, thereby elucidating the strange-metal phenomena that have been ubiquitously observed in strongly correlated electron materials.
Dimensionality plays an essential role in determining the anomalous non-Fermi liquid properties in heavy fermion systems. So far most heavy fermion compounds are quasi-two-dimensional or three-dimensional. Here we report the synthesis and systematic investigations of the single crystals of the quasi-one-dimensional Kondo lattice CeCo$_2$Ga$_8$. Resistivity measurements at ambient pressure reveal the onset of coherence at $T^*approx 20,$K and non-Fermi liquid behavior with linear temperature dependence over a decade in temperature from 2 K to 0.1 K. The specific heat increases logarithmically with lowering temperature between 10 K and 2 K and reaches 800 mJ/mol K$^2$ at 1 K, suggesting that CeCo$_2$Ga$_8$ is a heavy fermion compound in the close vicinity of a quantum critical point. Resistivity measurements under pressure further confirm the non-Fermi liquid behavior in a large temperature-pressure range. The magnetic susceptibility is found to follow the typical behavior for a one-dimensional (1D) spin chain from 300 K down to $T^*$, and first-principles calculations predict flat Fermi surfaces for the itinerant $f$-electron bands. These suggest that CeCo$_2$Ga$_8$ is a rare example of the quasi-1D Kondo lattice, but its non-Fermi liquid behaviors resemble those of the quasi-two-dimensional YbRh$_2$Si$_2$ family. The study of the quasi-one-dimensional CeCo$_2$Ga$_8$ family may therefore help us to understand the role of dimensionality on heavy fermion physics and quantum criticality.
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