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Register a new userStudy of cosmogenic radionuclides in the COSINE-100 NaI(Tl) detectors
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COSINE-100 is a direct detection dark matter search experiment that uses a 106 kg array of eight NaI(Tl) crystals that are kept underground at the Yangyang Underground Laboratory to avoid cosmogenic activation of radioisotopes by cosmic rays. Even though the cosmogenic activity is declining with time, there are still significant background rates from the remnant nuclides. In this paper, we report measurements of cosmogenic isotope contaminations with less than one year half-lives that are based on extrapolations of the time dependent activities of their characteristic energy peaks to activity rates at the time the crystals were deployed underground. For longer-lived $^{109}$Cd ($T_{1/2}=1.6$ y) and $^{22}$Na ($T_{1/2}=2.6$ y), we investigate time correlations of characteristic $gamma$/X-ray peaks. The inferred sea-level production rates are compared with caluclations based on the ACTIVIA and MENDL-2 model calculations and experimental data. For $^{3}$H, which has a long, 12.3 year half-life, we evaluated the activity levels from the exposure times and determined a cosmogenic activation rate that is consistent with other measurements.
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The COSINE-100 dark matter search experiment is an array of NaI(Tl) crystal detectors located in the Yangyang Underground Laboratory (Y2L). To understand measured backgrounds in the NaI(Tl) crystals we have performed Monte Carlo simulations using the Geant4 toolkit and developed background models for each crystal that consider contributions from both internal and external sources, including cosmogenic nuclides. The background models are based on comparisons of measurement data with Monte Carlo simulations that are guided by a campaign of material assays and are used to evaluate backgrounds and identify their sources. The average background level for the six crystals (70 kg total mass) that are studied is 3.5 counts/day/keV/kg in the (2-6) keV energy interval. The dominant contributors in this energy region are found to be $^{210}$Pb and $^3$H.
We present new constraints on the dark matter-induced annual modulation signal using 1.7 years, of COSINE-100 data with a total exposure of 97.7 kg$cdot$years. The COSINE-100 experiment, consisting of 106 kg of NaI(Tl) target material, is designed to carry out a model-independent test of DAMA/LIBRAs claim of WIMP discovery by searching for the same annual modulation signal using the same NaI(Tl) target. The crystal data show a 2.7 cpd/kg/keV background rate on average in the 2--6 keV energy region of interest. Using a $chi$-squared minimization method we observe best fit values for modulation amplitude and phase of 0.0092$pm$0.0067 cpd/kg/keV and 127.2$pm$45 d, respectively.
The annual modulation signal observed by the DAMA experiment is a long-standing question in the community of dark matter direct detection. This necessitates an independent verification of its existence using the same detection technique. The COSINE-100 experiment has been operating with 106~kg of low-background NaI(Tl) detectors providing interesting checks on the DAMA signal. However, due to higher backgrounds in the NaI(Tl) crystals used in COSINE-100 relative to those used for DAMA, it was difficult to reach final conclusions. Since the start of COSINE-100 data taking in 2016, we also have initiated a program to develop ultra-pure NaI(Tl) crystals for COSINE-200, the next phase of the experiment. The program includes efforts of raw powder purification, ultra-pure NaI(Tl) crystal growth, and detector assembly techniques. After extensive research and development of NaI(Tl) crystal growth, we have successfully grown a few small-size (0.61$-$0.78 kg) thallium-doped crystals with high radio-purity. A high light yield has been achieved by improvements of our detector assembly technique. Here we report the ultra-pure NaI(Tl) detector developments at the Institute for Basic Science, Korea. The technique developed here will be applied to the production of NaI(Tl) detectors for the COSINE-200 experiment.
Using a narrow band positron beam, the response of a large high-resolution NaI(Tl) crystal to an incident positron beam was measured. It was found that nuclear interactions cause the appearance of additional peaks in the low energy tail of the deposited energy spectrum.
A high purity and large volume NaI(Tl) scintillator was developed to search for cosmic dark matter. The required densities of radioactive impurities (RIs) such as U-chain, Th-chain are less than a few ppt to establish high sensitivity to dark matter. The impurity of RIs were effectively reduced by selecting raw materials of crucible and by performing chemical reduction of lead ion in NaI raw powder. The impurity of $^{226}$Ra was reduced less than 100 $mu$Bq/kg in NaI(Tl) crystal. It should be remarked that the impurity of $^{210}$Pb, which is difficult to reduce, is effectively reduced by chemical processing of NaI raw powder down to less than 30 $mu$Bq/kg. The expected sensitivity to cosmic dark matter by using 250 kg of the high purity and large volume NaI(Tl) scintillator (PICO-LON; Pure Inorganic Crystal Observatory for LOw-background Neutr(al)ino) is 7$times$10$^{-45}$ cm$^{2}$ for 50 GeV$/c^{2}$ WIMPs.
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