No Arabic abstract
International nuclear safeguards inspectors do not have a method to verify the contents of sealed storage casks containing spent reactor fuel. The heavy shielding that is used to limit radiation emission attenuates and scatters photons and neutrons emitted by the fuel, and thereby hinders inspection with these probes. This problem is especially pressing given the policy decisions of several nations to begin permanent disposal of spent fuel in deep geological repositories. Radiography with cosmic-ray muons provides a potential solution, as muons are able to penetrate the cask and fuel and provide information on the cask contents. Here we show in simulation that muon scattering radiography can be used to inspect the contents of sealed geological storage casks, and can discern between a variety of plausible diversion scenarios. This technique can be applied immediately prior to permanent interment in a geological repository, giving inspectors a final opportunity to verify State declarations of spent fuel disposal.
Radiography with cosmic ray muon scattering has proven to be a successful method of imaging nuclear material through heavy shielding. Of particular interest is monitoring dry storage casks for diversion of plutonium contained in spent reactor fuel. Using muon tracking detectors that surround a cylindrical cask, cosmic ray muon scattering can be simultaneously measured from all azimuthal angles, giving complete tomographic coverage of the cask interior. This paper describes the first application of filtered back projection algorithms, typically used in medical imaging, to cosmic ray muon imaging. The specific application to monitoring spent nuclear fuel in dry storage casks is investigated via GEANT4 simulations. With a cylindrical muon tracking detector surrounding a typical spent fuel cask, the cask contents can be confirmed with high confidence in less than two days exposure. Similar results can be obtained by moving a smaller detector to view the cask from multiple angles.
Muon radiography is a fast growing field in applied scientific research. In recent years, many detector technologies and imaging techniques using the Coulomb scattering and absorption properties of cosmic-ray muons have been developed for the non-destructive assay of various structures across a wide range of applications. This work presents the first results that assess the feasibility of using muons to interrogate waste silos within the UK Nuclear Industry. Two such approaches, using different techniques that exploit each of these properties, have previously been published, and show promising results from both simulation and experimental data for the detection of shielded high-Z materials and density variations from volcanic assay. Both detector systems are based on scintillator and photomultiplier technologies. Results from dedicated simulation studies using both these technologies and image reconstruction techniques are presented for an intermediate-sized nuclear waste storage facility filled with concrete and an array of uranium samples. Both results highlight the potential to identify uranium objects of varying thicknesses greater than 5cm within real-time durations of several weeks. Increased contributions from Coulomb scattering within the concrete of the structure hinder the ability of both approaches to resolve objects of 2cm dimensions even with increased statistics. These results are all dependent on both the position of the objects within the facility and the locations of the detectors. Results for differing thicknesses of concrete, which reflect the unknown composition of the structures under interrogation, are also presented alongside studies performed for a series of data collection durations. It is anticipated that with further research, muon radiography in one, or both of these forms, will play a key role in future industrial applications within the UK Nuclear Industry.
Most of the plutonium in the world resides inside spent nuclear reactor fuel rods. This high-level radioactive waste is commonly held in long-term storage within large, heavily shielded casks. Currently, international nuclear safeguards inspectors have no stand-alone method of verifying the amount of reactor fuel stored within a sealed cask. Here we demonstrate experimentally that measurements of the scattering angles of cosmic ray muons which pass through a storage cask can be used to determine if spent fuel assemblies are missing without opening the cask. This application of technology and methods commonly used in high-energy particle physics provides a potential solution to this long-standing problem in international nuclear safeguards.
Muon radiography is a promising technique to image the internal density structures upto a few hundred meters scale, such as tunnels, pyramids and volcanos, by measuring the flux attenuation of cosmic ray muons after trvaling through these targets. In this study, we conducted an experimantal cosmic ray muon radiography of the Wudalianchi volcano in northeast China for imaging its internal density structures. The muon detector used in this study is made of plastic scintillator and silicon photomultiplier. After about one and a half month observation for the Laoheishan volcano cone in the Wudalianchi volcano, from September 23rd to November 10th, 2019, more than 3 million muon tracks passing the data selection criteria are obtained. Based on the muon observations and the high-resoluiton topography from aerial photogrammetry by unmanned aerial vehicle, the relative density image of the Laoheishan volcano cone is obtained. The experiment in this study is the first muon radiography of volcano performed in China, and the results suggest the feasibility of radiography technique based on plastic scintillator muon detector. As a new passive geophysical imaging method, cosmic ray muon radiography could become a promising method to obtain the high-resoution 2-D and 3-D density structures for shallow geological targets.
Spent nuclear fuel (SNF) antineutrino flux is an important source of uncertainties for a reactor neutrino flux prediction. However, if one want to determine the contribution of spent fuel, many data are needed, such as the amount of spent fuel in the pool, the time after discharged from the reactor core, the burnup of each assembly, and the antineutrino spectrum of the isotopes in the spend fuel. A method to calculate the contribution of SNF is proposed in this study. In this method, reactor simulation code verified by experiment have been used to simulate the fuel depletion by taking into account more than 2000 isotopes and fission products, the quantity of SNF in each six spend fuel pool, and the antineutrino spectrum of SNF varying with time after SNF discharged from core. Results show that the contribution of SNF to the total antineutrino flux is about 0.26%~0.34%, and the shutdown impact is about 20%. The SNF spectrum would distort the softer part of antineutrino spectra, and the maximum contribution from SNF is about 3.0%, but there is 18% difference between line evaluate method and under evaluate method. In addition, non-equilibrium effects are also discussed, and the results are compatible with theirs considering the uncertainties.