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Register a new userRealization of Ordered Magnetic Skyrmions in Thin Films at Ambient Conditions
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Added by
Lisa DeBeer-Schmitt
Publication date
2019
fields
Physics
and research's language is
English
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Magnetic skyrmions present interesting physics due to their topological nature and hold significant promise for future information technologies. A key barrier to realizing skyrmion devices has been stabilizing these spin structures under ambient conditions. In this manuscript, we exploit the tunable magnetic properties of amorphous Fe/Gd mulitlayers to realize skyrmion lattices which are stable over a large temperature and magnetic field parameter space, including room temperature and zero magnetic field. These hybrid skyrmions have both Bloch-type and Neel-type character and are stabilized by dipolar interactions rather than Dzyaloshinskii-Moriya interactions, which are typically considered required for the generation of skyrmions. Small angle neutron scattering (SANS) was used in combination with soft X-ray microscopy to provide a unique, multi-scale probe of the local and long-range order of these structures. These results identify a pathway to engineer controllable skyrmion phases in thin film geometries which are stable at ambient conditions.
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The magnetic structure of the in-plane skyrmions in epitaxial MnSi/Si(111) thin films is probed in three dimensions by the combination of polarized neutron reflectometry (PNR) and small angle neutron scattering (SANS). We demonstrate that skyrmions exist in a region of the phase diagram above at temperature of 10 K. PNR shows the skyrmions are confined to the middle of the film due to the potential well formed by the surface twists. However, SANS shows that there is considerable disorder within the plane indicating that the magnetic structure is a 2D skyrmion glass.
Facing the ever-growing demand for data storage will most probably require a new paradigm. Magnetic skyrmions are anticipated to solve this issue as they are arguably the smallest spin textures in magnetic thin films in nature. We designed cobalt-based multilayered thin films where the cobalt layer is sandwiched between two heavy metals providing additive interfacial Dzyaloshinskii-Moriya interactions, which reach about 2 mJ/m2 in the case of the Ir/Co/Pt multilayers. Using a magnetization-sensitive scanning x-ray transmission microscopy technique, we imaged magnetic bubble-like domains in these multilayers. The study of their behavir in magnetic field allows us to conclude that they are actually magnetic skyrmions stabilized by the Dzyaloshinsskii-Moriya interaction. This discoevry of stable skyrmions at room temperature in a technologically relevant material opens the way for device applications in a near future.
Non-collinear magnets exhibit a rich array of dynamic properties at microwave frequencies. They can host nanometre-scale topological textures known as skyrmions, whose spin resonances are expected to be highly sensitive to their local magnetic environment. Here, we report a magnetic resonance study of an [Ir/Fe/Co/Pt] multilayer hosting Neel skyrmions at room temperature. Experiments reveal two distinct resonances of the skyrmion phase during in-plane ac excitation, with frequencies between 6-12 GHz. Complementary micromagnetic simulations indicate that the net magnetic dipole moment rotates counterclockwise (CCW) during both resonances. The magnon probability distribution for the lower-frequency resonance is localised within isolated skyrmions, unlike the higher-frequency mode which principally originates from areas between skyrmions. However, the properties of both modes depend sensitively on the out-of-plane dipolar coupling, which is controlled via the ferromagnetic layer spacing in our heterostructures. The gyrations of stable isolated skyrmions reported in this room temperature study encourage the development of new material platforms and applications based on skyrmion resonances. Moreover, our material architecture enables the resonance spectra to be tuned, thus extending the functionality of such applications over a broadband frequency range.
The detection of ensembles of spins under ambient conditions has revolutionized the biological, chemical, and physical sciences through magnetic resonance imaging and nuclear magnetic resonance. Pushing sensing capabilities to the individual-spin level would enable unprecedented applications such as single molecule structural imaging; however, the weak magnetic fields from single spins are undetectable by conventional far-field resonance techniques. In recent years, there has been a considerable effort to develop nanoscale scanning magnetometers, which are able to measure fewer spins by bringing the sensor in close proximity to its target. The most sensitive of these magnetometers generally require low temperatures for operation, but measuring under ambient conditions (standard temperature and pressure) is critical for many imaging applications, particularly in biological systems. Here we demonstrate detection and nanoscale imaging of the magnetic field from a single electron spin under ambient conditions using a scanning nitrogen-vacancy (NV) magnetometer. Real-space, quantitative magnetic-field images are obtained by deterministically scanning our NV magnetometer 50 nanometers above a target electron spin, while measuring the local magnetic field using dynamically decoupled magnetometry protocols. This single-spin detection capability could enable single-spin magnetic resonance imaging of electron spins on the nano- and atomic scales and opens the door for unique applications such as mechanical quantum state transfer.
Measuring spins is the corner stone of a variety of analytical techniques including modern magnetic resonance imaging (MRI). The full potential of spin imaging and sensing across length scales is hindered by the achievable signal-to-noise in inductive detection schemes. Here we show that a proximal Nitrogen-Vacancy (NV) ensemble serves as a precision sensing array. Monitoring its quantum relaxation enables sensing of freely diffusing and unperturbed magnetic ions in a microfluidic device. Multiplexed CCD acquisition and an optimized detection scheme enable direct spin noise imaging under ambient conditions with experimental sensitivities down to 1000 statistically polarized spins, of which only 35 ions contribute to a net magnetization, and 20 s acquisition time. We also demonstrate imaging of spin labeled cellular structures with spatial resolutions below 500 nm. Our study marks a major step towards sub-{mu}m imaging magnetometry and applications in microanalytics, material and life sciences.
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