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Targeted evolution of pinning landscapes for large superconducting critical currents

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 Added by Ivan Sadovskyy
 Publication date 2019
  fields Physics
and research's language is English




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The ability of type-II superconductors to carry large amounts of current at high magnetic fields is a key requirement for future design innovations in high-field magnets for accelerators and compact fusion reactors and largely depends on the vortex pinning landscape comprised of material defects. The complex interaction of vortices with defects that can be grown chemically, e.g., self-assembled nanoparticles and nanorods, or introduced by post-synthesis particle irradiation precludes a priori prediction of the critical current and can result in highly non-trivial effects on the critical current. Here, we borrow concepts from biological evolution to create a genetic algorithm evolving pinning landscapes to accommodate vortex pinning and determine the best possible configuration of inclusions for two different scenarios: an evolution process starting from a pristine system and one with pre-existing defects to demonstrate the potential for a post-processing approach to enhance critical currents. Furthermore, the presented approach is even more general and can be adapted to address various other targeted material optimization problems.



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We present the new paradigm of critical current by design. Analogous to materials by design, it aims at predicting the optimal defect landscape in a superconductor for targeted applications by elucidating the vortex dynamics responsible for the bulk critical current. To highlight this approach, we demonstrate the synergistic combination of critical current measurements on commercial high-temperature superconductors containing self-assembled and irradiation tailored correlated defects by using large-scale time-dependent Ginzburg-Landau simulations for vortex dynamics.
434 - I. Swiecicki , C. Ulysse , T. Wolf 2011
We have developed a masked ion irradiation technique to engineer the energy landscape for vortices in oxide superconductors. This approach associates the possibility to design the landscape geometry at the nanoscale with the unique capability to adjust depth of the energy wells for vortices. This enabled us to unveil the key role of vortex channeling in modulating the amplitude of the field matching effects with the artificial energy landscape, and to make the latter govern flux dynamics over an usually wide range of temperatures and applied fields.
Understanding the effect of pinning on the vortex dynamics in superconductors is a key factor towards controlling critical current values. Large-scale simulations of vortex dynamics can provide a rational approach to achieve this goal. Here, we use the time-dependent Ginzburg-Landau equations to study thin superconducting films with artificially created pinning centers arranged periodically in hexagonal lattices. We calculate the critical current density for various geometries of the pinning centers --- varying their size, strength, and density. Furthermore, we shed light upon the influence of pattern distortion on the magnetic-field-dependent critical current. We compare our result directly with available experimental measurements on patterned molybdenum-germanium films, obtaining good agreement. Our results give important systematic insights into the mechanisms of pinning in these artificial pinning landscapes and open a path for tailoring superconducting films with desired critical current behavior.
The current-carrying capacity of type-II superconductors is decisively determined by how well material defect structures can immobilize vortex lines. In order to gain deeper insights into the fundamental pinning mechanisms, we have explored the case of vortex trapping by randomly distributed spherical inclusions using large-scale simulations of the time-dependent Ginzburg-Landau equations. We find that for a small density of particles having diameters of two coherence lengths, the vortex lattice preserves its structure and the critical current $j_c$ decays with the magnetic field following a power-law $B^{-alpha}$ with $alpha approx 0.66$, which is consistent with predictions of strong-pinning theory. For a higher density of particles and/or larger inclusions, the lattice becomes progressively more disordered and the exponent smoothly decreases down to $alpha approx 0.3$. At high magnetic fields, all inclusions capture a vortex and the critical current decays faster than $B^{-1}$ as would be expected by theory. In the case of larger inclusions with a diameter of four coherence length, the magnetic-field dependence of the critical current is strongly affected by the ability of inclusions to capture multiple vortex lines. We found that at small densities, the fraction of inclusions trapping two vortex lines rapidly grows within narrow field range leading to a peak in $j_c(B)$-dependence within this range. With increasing inclusion density, this peak transforms into a plateau, which then smooths out. Using the insights gained from simulations, we determine the limits of applicability of strong-pinning theory and provide different routes to describe vortex pinning beyond those bounds.
We have theoretically studied the supercurrent profiles in three-dimensional normal metal and ferromagnetic Josephson configurations, where the magnitude of the superconducting gaps in the superconducting leads are unequal, i.e., $Delta_1 eq Delta_2$, creating asymmetric $S_1NS_2$ and $S_1FS_2$ systems. Our results reveal that by increasing the ratio of the superconducting gaps $Delta_2/Delta_1$, the critical supercurrent in a ballistic $S_1NS_2$ system can be enhanced by more than $100%$, and reaches a saturation point, or decays away, depending on the junction thickness, magnetization strength, and chemical potential. The total critical current in a diffusive $S_1NS_2$ system was found to be enhanced by more than $50%$ parabolically, and reaches saturation by increasing one of the superconducting gaps. In a uniform ferromagnetic junction, the supercurrent undergoes reversal by increasing $Delta_2/Delta_1>1$. Through decomposing the total supercurrent into its supergap and subgap components, our results illustrate their crucial relative contributions to the Josephson current flow. It was found that the competition of subgap and supergap currents in a $S_1FS_2$ junction results in the emergence of second harmonics in the current-phase relation. In contrast to a diffusive asymmetric Josephson configuration, the behavior of the supercurrent in a ballistic system with $Delta_2/Delta_1=1$ can be properly described by the subgap current component only, in a wide range of parameter sets, including Fermi level mismatch, magnetization strength, and junction thickness. Interestingly, when $Delta_2/Delta_1>1$, our results have found multiple parameter sets where the total supercurrent is driven by the supergap component. Therefore, our comprehensive study highlights the importance of subgap and supergap supercurrent components in both the ballistic and diffusive regimes.
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