Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userAnomalous thermoelectric effects of ZrTe$_{5}$ in and beyond the quantum limit
70
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
Thermoelectric effects are more sensitive and promising probes to topological properties of emergent materials, but much less addressed compared to other physical properties. Zirconium pentatelluride (ZrTe$_{5}$) has inspired active investigations recently because of its multiple topological nature. We study the thermoelectric effects of ZrTe$_{5}$ in a magnetic field and find several anomalous behaviors. The Nernst response has a steplike profile near zero field when the charge carriers are electrons only, suggesting the anomalous Nernst effect arising from a nontrivial profile of Berry curvature. Both the thermopower and Nernst signal exhibit exotic peaks in the strong-field quantum limit. At higher magnetic fields, the Nernst signal has a sign reversal at a critical field where the thermopower approaches to zero. We propose that these anomalous behaviors can be attributed to the Landau index inversion, which is resulted from the competition of the $sqrt{B}$ dependence of the Dirac-type Landau bands and linear-$B$ dependence of the Zeeman energy ($B$ is the magnetic field). Our understanding to the anomalous thermoelectric properties in ZrTe$_{5}$ opens a new avenue for exploring Dirac physics in topological materials.
rate research
Read More
The thermoelectric Hall effect is the generation of a transverse heat current upon applying an electric field in the presence of a magnetic field. Here we demonstrate that the thermoelectric Hall conductivity $alpha_{xy}$ in the three-dimensional Dirac semimetal ZrTe$_5$ acquires a robust plateau in the extreme quantum limit of magnetic field. The plateau value is independent of the field strength, disorder strength, carrier concentration, or carrier sign. We explain this plateau theoretically and show that it is a unique signature of three-dimensional Dirac or Weyl electrons in the extreme quantum limit. We further find that other thermoelectric coefficients, such as the thermopower and Nernst coefficient, are greatly enhanced over their zero-field values even at relatively low fields.
Arising from the interplay between charge, spin and orbital of electrons, spin-orbit torque (SOT) has attracted immense interest in the past decade. Despite vast progress, the existing quantification methods of SOT still have their respective restrictions on the magnetic anisotropy, the entanglement between SOT effective fields, and the artifacts from the thermal gradient and the planar Hall effect, etc. Thus, accurately characterizing SOT across diverse samples remains as a critical need. In this work, with the aim of removing the afore-mentioned restrictions, thus enabling the universal SOT quantification, we report the characterization of the sign and amplitude of SOT by angular measurements. We first validate the applicability of our angular characterization in a perpendicularly magnetized Pt/Co-Ni heterostructure by showing excellent agreements to the results of conventional quantification methods. Remarkably, the thermoelectric effects, i.e., the anomalous Nernst effect (ANE) arising from the temperature gradient can be self-consistently disentangled and quantified from the field dependence of the angular characterization. The superiority of this angular characterization has been further demonstrated in a Cu/CoTb/Cu sample with large ANE but negligible SOT, and in a Pt/Co-Ni sample with weak perpendicular magnetic anisotropy (PMA), for which the conventional quantification methods are not applicable and even yield fatal error. By providing a comprehensive and versatile way to characterize SOT and thermoelectric effects in diverse heterostructures, our results pave the important foundation for the spin-orbitronic study as well as the interdisciplinary research of thermal spintronic.
Using first-principles calculations combined with Boltzmann transport theory, we investigate the effects of topological edge states on the thermoelectric properties of Bi nanoribbons. It is found that there is a competition between the edge and bulk contributions to the Seebeck coefficients. However, the electronic transport of the system is dominated by the edge states because of its much larger electrical conductivity. As a consequence, a room temperature value exceeding 3.0 could be achieved for both p- and n-type systems when the relaxation time ratio between the edge and the bulk states is tuned to be 1000. Our theoretical study suggests that the utilization of topological edge states might be a promising approach to cross the threshold of the industrial application of thermoelectricity.
We use first-principles methods to reveal that in ZrTe$_5$, a layered van der Waals material like graphite, atomic displacements corresponding to five of the six zone-center A$_g$ (symmetry-preserving) phonon modes can drive a topological phase transition from strong to weak topological insulator with a Dirac semimetal state emerging at the transition, giving rise to a Dirac topology surface in the multi-dimensional space formed by the A$_g$ phonon modes. This implies that the topological phase transition in ZrTe$_5$ can be realized with many different settings of external stimuli that are capable of penetrating through the phonon-space Dirac surface without breaking the crystallographic symmetry. Furthermore, we predict that domains with effective mass of opposite signs can be created by laser pumping and will host Weyl modes of opposite chirality propagating along the domain boundaries. Studying phonon-space topology surfaces provides a new route to understanding and utilizing the exotic physical properties of ZrTe$_5$ and related quantum materials.
We present magneto transport experiments of quasi 3D PbTe wide quantum wells. A plateau-like structure in the Hall resistance is observed, which corresponds to the Shubnikov de Haas oscillations in the same manner as known from the quantum Hall effect. The onsets of plateaux in Rxy do not correspond to 2D filling factors but coincide with the occupation of 3D (bulk-) Landau levels. At the same time a non-local signal is observed which corresponds to the structure in Rxx and Rxy and fulfils exactly the Onsager-Casimir relation (Rij,kl(B) = Rkl,ij(-B)). We explain the behaviour in terms of edge channel transport which is controlled by a permanent backscattering across a system of percolative EC - loops in the bulk region. Long range potential fluctuations with an amplitude of the order of the subband splitting are explained to play an essential role in this electron system.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
