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Register a new userCharacterization of $^{233}$U alpha recoil sources for $^{229(m)}$Th beam production
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Radioactive $^{233}$U alpha recoil sources are being considered for the production of a thorium ion source to study the low-energy isomer in $^{229}$Th with high-resolution collinear laser spectroscopy at the IGISOL facility of the University of Jyvaskyla. In this work two different $^{233}$U sources have been characterized via alpha and gamma spectroscopy of the decay radiation obtained directly from the sources and from alpha-recoils embedded in implantation foils. These measurements revealed rather low $^{229}$Th recoil efficiencies of only a few percent. Although the low efficiency of one of the two sources can be attributed to its inherent thickness, the low recoil efficiency of the second, thinner source, was unexpected. Rutherford backscattering spectrometry (RBS) was performed to investigate the elemental composition as a function of depth revealing a contamination layer on top of the thin source. The combination of spectroscopic methods proves to be a useful approach in the assessment of alpha recoil source performance in general.
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Four different techniques were applied for the production of $^{233}$U alpha recoil ion sources, providing $^{229}$Th ions. They were compared with respect to a minimum energy spread of the $^{229}$Th recoil ions, using the emitted alpha particles as an indicator. The techniques of Molecular Plating, Drop-on-Demand inkjet printing, chelation from dilute nitric acid solution on chemically functionalized silicon surfaces, and self-adsorption on passivated titanium surfaces were used. All fabricated sources were characterized by using alpha spectrometry, radiographic imaging, and scanning electron microscopy. A direct validation for the estimated recoil ion rate was obtained by collecting $^{228}$Th recoil ions from $^{232}$U recoil ion sources prepared by self-adsorption and Molecular Plating. The chelation and the self-adsorption based approaches appear most promising for the preparation of recoil ion sources delivering monochromatic recoil ions.
Thorium-229 is a unique case in nuclear physics: it presents a metastable first excited state Th-229m, just a few electronvolts above the nuclear ground state. This so-called isomer is accessible by VUV lasers, which allows transferring the amazing precision of atomic laser spectroscopy to nuclear physics. Being able to manipulate the Th-229 nuclear states at will opens up a multitude of prospects, from studies of the fundamental interactions in physics to applications as a compact and robust nuclear clock. However, direct optical excitation of the isomer or its radiative decay back to the ground state has not yet been observed, and a series of key nuclear structure parameters such as the exact energies and half-lives of the low-lying nuclear levels of Th-229 are yet unknown. Here we present the first active optical pumping into Th-229m. Our scheme employs narrow-band 29 keV synchrotron radiation to resonantly excite the second excited state, which then predominantly decays into the isomer. We determine the resonance energy with 0.07 eV accuracy, measure a half-life of 82.2 ps, an excitation linewidth of 1.70 neV, and extract the branching ratio of the second excited state into the ground and isomeric state respectively. These measurements allow us to re-evaluate gamma spectroscopy data that have been collected over 40~years.
Electromagnetic properties of the deformed neutron-odd nucleus $^{229}$Th are investigated in the framework of the unified model, with primary emphasis upon the properties of the low-lying isomeric state.
We perform coincidence measurements between $alpha$ particles and $gamma$ rays from a $^{233}$U source to determine the half-lives of the excited state in a $^{229}$Th nucleus. We first prove that the half-lives of 42.43- and 164.53-keV states are consistent with literature values, whereas that of the 97.14-keV state (93(7) ps) deviates from a previously measured value (147(12) ps). The half-lives of 71.83- and 163.25-keV states are determined for the first time. Based on the obtained half-lives and the Alaga rule, we estimate the radiative half-life of the low-energy isomeric state ($^{229m}$Th) to be $5.0(11)times10^{3}$ s, which is one of the key parameters for the frequency standard based on $^{229}$Th.
Understanding of $gamma$-ray production via neutron interactions on oxygen is essential for the study of neutrino neutral-current quasielastic interactions in water Cherenkov detectors. A measurement of $gamma$-ray production from such reactions was performed using a 77~MeV quasi-monoenergetic neutron beam. Several $gamma$-ray peaks, which are expected to come from neutron-${rm ^{16}O}$ reactions, are observed and production cross sections are measured for nine $gamma$-ray components of energies between 2 and 8~MeV. These are the first measurements at this neutron energy using a nearly monoenergitic beam.
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