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Register a new userMagnetic properties and domain structure of ultrathin yttrium iron garnet/Pt bilayers
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Johannes Mendil
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We report on the structure, magnetization, magnetic anisotropy, and domain morphology of ultrathin yttrium iron garnet (YIG)/Pt films with thickness ranging from 3 to 90 nm. We find that the saturation magnetization is close to the bulk value in the thickest films and decreases towards low thickness with a strong reduction below 10 nm. We characterize the magnetic anisotropy by measuring the transverse spin Hall magnetoresistance as a function of applied field. Our results reveal strong easy plane anisotropy fields of the order of 50-100 mT, which add to the demagnetizing field, as well as weaker in-plane uniaxial anisotropy ranging from 10 to 100 $mu$T. The in-plane easy axis direction changes with thickness, but presents also significant fluctuations among samples with the same thickness grown on the same substrate. X-ray photoelectron emission microscopy reveals the formation of zigzag magnetic domains in YIG films thicker than 10 nm, which have dimensions larger than several 100 $mu$m and are separated by achiral N{e}el-type domain walls. Smaller domains characterized by interspersed elongated features are found in YIG films thinner than 10 nm.
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Yttrium iron garnet is a complex ferrimagnetic insulator with 20 magnon modes which is used extensively in fundamental experimental studies of magnetisation dynamics. As a transition metal oxide with moderate gap (2.8 eV), yttrium iron garnet requires a careful treatment of electronic correlation. We have applied quasiparticle self-consistent GW to provide a fully ab initio description of the electronic structure and resulting magnetic properties, including the parameterisation of a Heisenberg model for magnetic exchange interactions. Subsequent spin dynamical modelling with quantum statistics extends our description to the magnon spectrum and thermodynamic properties such as the Curie temperature, finding favourable agreement with experimental measurements. This work provides a snapshot of the state-of-the art in modelling of complex magnetic insulators.
The dynamic observation of domain wall motion induced by electric field in magnetoelectric iron garnet film is reported. Measurements in 800 kV/cm electric field pulses gave the domain wall velocity ~45 m/s. Similar velocity was achieved in magnetic field pulse about 50 Oe. Reversible and irreversible micromagnetic structure transformation is demonstrated. These effects are promising for applications in spintronics and magnetic memory.
We investigate the temperature dependent microwave absorption spectrum of an yttrium iron garnet sphere as a function of temperature (5 K to 300 K) and frequency (3 GHz to 43.5 GHz). At temperatures above 100 K, the magnetic resonance linewidth increases linearly with temperature and shows a Gilbert-like linear frequency dependence. At lower temperatures, the temperature dependence of the resonance linewidth at constant external magnetic fields exhibits a characteristic peak which coincides with a non-Gilbert-like frequency dependence. The complete temperature and frequency evolution of the linewidth can be modeled by the phenomenology of slowly relaxing rare-earth impurities and either the Kasuya-LeCraw mechanism or the scattering with optical magnons. Furthermore, we extract the temperature dependence of the saturation magnetization, the magnetic anisotropy and the g-factor.
Spin waves can probe the Dzyaloshinskii-Moriya interaction (DMI) which gives rise to topological spin textures, such as skyrmions. However, the DMI has not yet been reported in yttrium iron garnet (YIG) with arguably the lowest damping for spin waves. In this work, we experimentally evidence the interfacial DMI in a 7~nm-thick YIG film by measuring the nonreciprocal spin wave propagation in terms of frequency, amplitude and most importantly group velocities using all electrical spin-wave spectroscopy. The velocities of propagating spin waves show chirality among three vectors, i.e. the film normal direction, applied field and spin-wave wavevector. By measuring the asymmetric group velocities, we extract a DMI constant of 16~$mu$J/m$^{2}$ which we independently confirm by Brillouin light scattering. Thickness-dependent measurements reveal that the DMI originates from the oxide interface between the YIG and garnet substrate. The interfacial DMI discovered in the ultrathin YIG films is of key importance for functional chiral magnonics as ultra-low spin-wave damping can be achieved.
For longitudinal spin Seebeck effect (LSSE) devices, a multilayer structure comprising ferromagnetic and nonmagnetic layers is expected to improve their thermoelectric power. In this study, we developed the fabrication method for alternately stacked yttrium-iron-garnet (YIG)/Pt multilayer films on a gadolinium gallium garnet (GGG) (110) substrate, GGG/[YIG(49 nm)/Pt(4 nm)]$_n$ ($n =$ 1 - 5) based on room-temperature sputtering and $ex$-$situ$ post-annealing method and we evaluated their structural and LSSE properties. The fabricated [YIG/Pt]$_n$ samples show flat YIG/Pt interfaces and almost identical saturation magnetization $M_{rm s}$, although they contain polycrystalline YIG layers on Pt layers as well as single-crystalline YIG layers on GGG. In the samples, we observed clear LSSE signals and found that the LSSE thermoelectric power factor (PF) increases monotonically with increasing $n$; the PF of the [YIG/Pt]$_5$ sample is enhanced by a factor of $sim 28$ compared to that of [YIG/Pt]$_1$. This work may provide a guideline for developing future multilayerbased LSSE devices.
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