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TRITIUM - A Real-Time Tritium Monitor System for Water Quality Surveillance

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 Added by Carlos Azevedo
 Publication date 2019
  fields Physics
and research's language is English




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In this work the development results of the TRITIUM project is presented. The main objective of the project is the construction of a near real-time monitor for low activity tritium in water, aimed at in-situ surveillance and radiological protection of river water in the vicinity of nuclear power plants. The European Council Directive 2013/51/Euratom requires that the maximum level of tritium in water for human consumption to be lower than 100 Bq/L. Tritium levels in the cooling water of nuclear power plants in normal operation are much higher than the levels caused by the natural and cosmogenic components, and may easily surmount the limit required by the Directive. The current liquid-scintillation measuring systems in environmental radioactivity laboratories are sensitive to such low levels, but they are not suitable for real-time monitoring. Moreover, there is no currently available device with enough sensitivity and monitoring capabilities that could be used for surveillance of the cooling water of nuclear power plants. A detector system based on scintillation fibers read out by photomultiplier tubes (PMTs) or silicon photomultiplier (SiPM) arrays is under development for in-water tritium measurement. This detector will be installed in the vicinity of Almaraz nuclear power plant (Spain) in Spring 2019. An overview of the project development and the results of first prototypes are presented.

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In this work we present simulation results for a modular tritium in-water real-time monitor. The system allows for scalability in order to achieve the required sensitivity. The modules are composed by 340 uncladed scintillating fibers immersed in water and 2 photosensors for light readout. Light yield and Birks coefficient uncertainties for low energy beta particles is discussed. A study of the detection efficiency according to the fiber length is presented. Discussion on the system requirements and background mitigation for a device with sensitivity of 100,Bq/L, required to comply with the European directive 2013/51/Euratom, is presented. Due to the low energetic beta emission from tritium a detection efficiency close to 3.3% was calculated for a single 2,mm round fiber.
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We present measurements of the electron-recoil (ER) response of the LUX dark matter detector based upon 170,000 highly pure and spatially-uniform tritium decays. We reconstruct the tritium energy spectrum using the combined energy model and find good agreement with expectations. We report the average charge and light yields of ER events in liquid xenon at 180 V/cm and 105 V/cm and compare the results to the NEST model. We also measure the mean charge recombination fraction and its fluctuations, and we investigate the location and width of the LUX ER band. These results provide input to a re-analysis of the LUX Run3 WIMP search.
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The direct detection of dark matter particles requires ultra-low background conditions at energies below a few tens of keV. Radioactive isotopes are produced via cosmogenic activation in detectors and other materials and those isotopes constitute a background source which has to be under control. In particular, tritium is specially relevant due to its decay properties (very low endpoint energy and long half-life) when induced in the detector medium, and because it can be generated in any material as a spallation product. Quantification of cosmogenic production of tritium is not straightforward, neither experimentally nor by calculations. In this work, a method for the calculation of production rates at sea level has been developed and applied to some of the materials typically used as targets in dark matter detectors (germanium, sodium iodide, argon and neon); it is based on a selected description of tritium production cross sections over the entire energy range of cosmic nucleons. Results have been compared to available data in the literature, either based on other calculations or from measurements. The obtained tritium production rates, ranging from a few tens to a few hundreds of nuclei per kg and per day at sea level, point to a significant contribution to the background in dark matter experiments, requiring the application of specific protocols for target material purification, material storing underground and limiting the time the detector is on surface during the building process in order to minimize the exposure to the most dangerous cosmic ray components.
128 - Walter C. Pettus 2017
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