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Superconductivity under pressure in the Dirac semimetal PdTe2

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 Added by A. de Visser
 Publication date 2019
  fields Physics
and research's language is English




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The Dirac semimetal PdTe$_2$ was recently reported to be a type-I superconductor ($T_c = $1.64 K, $mu_0 H_c (0) = 13.6$ mT) with unusual superconductivity of the surface sheath. We here report a high-pressure study, $p leq 2.5$ GPa, of the superconducting phase diagram extracted from ac-susceptibility and transport measurements on single crystalline samples. $T_c (p)$ shows a pronounced non-monotonous variation with a maximum $T_c = $1.91 K around 0.91 GPa, followed by a gradual decrease to 1.27 K at 2.5 GPa. The critical field of bulk superconductivity in the limit $T rightarrow 0$, $H_c(0,p)$, follows a similar trend and consequently the $H_c(T,p)$-curves under pressure collapse on a single curve: $H_c(T,p)=H_c(0,p)[1-(T/T_c(p))^2]$. Surface superconductivity is robust under pressure as demonstrated by the large superconducting screening signal that persists for applied dc-fields $H_a > H_c$. Surprisingly, for $p geq 1.41$ GPa the superconducting transition temperature at the surface $T_c^S$ is larger than $T_c$ of the bulk. Therefore surface superconductivity may possibly have a non-trivial nature and is connected to the topological surface states detected by ARPES. We compare the measured pressure variation of $T_c$ with recent results from band structure calculations and discuss the importance of a Van Hove singularity.

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The superconductor PdTe$_2$ was recently classified as a Type II Dirac semimetal, and advocated to be an improved platform for topological superconductivity. Here we report magnetic and transport measurements conducted to determine the nature of the superconducting phase. Surprisingly, we find that PdTe$_2$ is a Type I superconductor with $T_c = 1.64$ K and a critical field $mu_0 H_c (0) = 13.6$ mT. Our crystals also exhibit the intermediate state as demonstrated by the differential paramagnetic effect. For $H > H_c$ we observe superconductivity of the surface sheath. This calls for a close examination of superconductivity in PdTe$_2$ in view of the presence of topological surface states.
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