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An extended Hubbard model on a honeycomb lattice with two orbitals per site at charge neutrality is investigated with unbiased large-scale quantum Monte Carlo simulations. The Fermi velocity of the Dirac fermions is renormalized as the cluster charge interaction increases, until a mass term emerges and a quantum phase transition from Dirac semi-metal to valence bond solid (VBS) insulator is established. The quantum critical point is discovered to belong to 3D $N=4$ Gross-Neveu chiral XY universality with the critical exponents obtained at high precision. Further enhancement of the interaction drives the system into two different VBS phases, the properties and transition between them are also revealed. Since the model is related to magic-angle twisted bilayer graphene, our results may have relevance towards the symmetry breaking order at the charge neutrality point of the material, and associate the wide range of universal strange metal behavior around it with quantum critical fluctuations.
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The flat bands of magic-angle twisted bilayer graphene (MATBG) host strongly-correlated electronic phases such as correlated insulators, superconductors and a strange metal state. The latter state, believed to hold the key to a deeper understanding of the electronic properties of MATBG, is obscured by the abundance of phase transitions; so far, this state could not be unequivocally differentiated from a metal undergoing frequent electron-phonon collisions. We report on transport measurements in superconducting (SC) MATBG in which the correlated insulator states were suppressed by screening. The uninterrupted metallic ground state features a T-linear resistivity extending over three decades in temperature, from 40 mK to 20 K, spanning a broad range of dopings including those where a correlation-driven Fermi surface reconstruction occurs. This strange-metal behavior is distinguished by Planckian scattering rates and a linear magneto-resistivity $rho propto B$. To the contrary, near charge neutrality or a fully-filled flat band, as well as for devices twisted away from the magic angle, the archetypal Fermi liquid behavior is recovered. Our measurements demonstrate the existence of a quantum-critical phase whose fluctuations dominate the metallic ground state. Further, a transition to the strange metal is observed upon suppression of the SC order, which suggests an intimate relationship between quantum fluctuations and superconductivity in MATBG.
We present a systematic study of the low-energy collective modes for different insulating states at integer fillings in twisted bilayer graphene. In particular, we provide a simple counting rule for the total number of soft modes, and analyze their energies and symmetry quantum numbers in detail. To study the soft mode spectra, we employ time dependent Hartree-Fock whose results are reproduced analytically via an effective sigma model description. We find two different types of low-energy modes - (i) approximate Goldstone modes associated with breaking an enlarged U(4)$times$U(4) symmetry and, surprisingly, a set of (ii) nematic modes with non-zero angular momentum under three-fold rotation. The modes of type (i) include true gapless Goldstone modes associated with exact symmetries in addition to gapped pseudo-Goldstone modes associated with approximate symmetries. While the modes of type (ii) are always gapped, we show that their gap decreases as the Berry curvature grows more concentrated. For realistic parameter values, the gapped soft modes of both types have comparable gaps of only a few meV, and lie completely inside the mean-field bandgap. The entire set of soft modes emerge as Goldstone modes of a different idealized model in which Berry flux is limited to a solenoid, which enjoys an enlarged U(8) symmetry. Furthermore, we discuss the number of Goldstone modes for each symmetry-broken state, distinguishing the linearly vs quadratically dispersing modes. Finally, we present a general symmetry analysis of the soft modes for all possible insulating Slater determinant states at integer fillings that preserve translation symmetry, independent of the energetic details. The resulting soft mode degeneracies and symmetry quantum numbers provide a fingerprint of the different insulting states enabling their experimental identification from a measurement of their soft modes.
The electronic properties of twisted bilayer graphene (TBG) can be dramatically different from those of a single graphene layer, in particular when the two layers are rotated relative to each other by a small angle. TBG has recently attracted a great deal of interest, sparked by the discovery of correlated insulating and superconducting states, for twist angle $theta$ close to a so-called magic angle $approx 1.1{deg}$. In this work, we unveil, via near-field optical microscopy, a collective plasmon mode in charge-neutral TBG near the magic angle, which is dramatically different from the ordinary single-layer graphene intraband plasmon. In selected regions of our samples, we find a gapped collective mode with linear dispersion, akin to the bulk magnetoplasmons of a two-dimensional (2D) electron gas. We interpret these as interband plasmons and associate those with the optical transitions between quasi-localized states originating from the moire superlattice. Surprisingly, we find a higher plasmon group velocity than expected, which implies an enhanced strength of the corresponding optical transition. This points to a weaker interlayer coupling in the AA regions. These intriguing optical properties offer new insights, complementary to other techniques, on the carrier dynamics in this novel quantum electron system.
Magic-angle twisted bilayer graphene (MATBG) exhibits a range of correlated phenomena that originate from strong electron-electron interactions. These interactions make the Fermi surface highly susceptible to reconstruction when $ pm 1, pm 2, pm 3$ electrons occupy each moir e unit cell and lead to the formation of correlated insulating, superconducting and ferromagnetic phases. While some phases have been shown to carry a non-zero Chern number, the local microscopic properties and topological character of many other phases remain elusive. Here we introduce a set of novel techniques hinging on scanning tunneling microscopy (STM) to map out topological phases in MATBG that emerge in finite magnetic field. By following the evolution of the local density of states (LDOS) at the Fermi level with electrostatic doping and magnetic field, we visualize a local Landau fan diagram that enables us to directly assign Chern numbers to all observed phases. We uncover the existence of six topological phases emanating from integer fillings in finite fields and whose origin relates to a cascade of symmetry-breaking transitions driven by correlations. The spatially resolved and electron-density-tuned LDOS maps further reveal that these topological phases can form only in a small range of twist angles around the magic-angle value. Both the microscopic origin and extreme sensitivity to twist angle differentiate these topological phases from the Landau levels observed near charge neutrality. Moreover, we observe that even the charge-neutrality Landau spectrum taken at low fields is considerably modified by interactions and exhibits an unexpected splitting between zero Landau levels that can be as large as ${sim },3-5$ meV. Our results show how strong electronic interactions affect the band structure of MATBG and lead to the formation of correlation-enabled topological phases.
We show that the insulating states of magic-angle twisted bilayer graphene support a series of collective modes corresponding to local particle-hole excitations on triangular lattice sites. Our theory is based on a continuum model of the magic angle flat bands. When the system is insulating at moire band filling $ u=-3$, our calculations show that the ground state supports seven low-energy modes that lie well below the charge gap throughout the moire Brillouin zone, one of which couples strongly to THz photons. The low-energy collective modes are faithfully described by a model with a local $SU(8)$ degree of freedom in each moire unit cell that we identify as the direct product of spin, valley, and an orbital pseudospin. Apart from spin and valley-wave modes, the collective mode spectrum includes a low-energy intra-flavor exciton mode associated with transitions between flat valence and conduction band orbitals.
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