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Register a new userVan Hove Singularities and Excited-State Quantum Phase Transitions in Graphene-like Microwave Billiards
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We discuss solutions of an algebraic model of the hexagonal lattice vibrations, which point out interesting localization properties of the eigenstates at van Hove singularities (vHs), whose energies correspond to Excited-State Quantum Phase Transitions (ESQPT). We show that these states form stripes oriented parallel to the zig-zag direction of the lattice, similar to the well-known edge states found at the Dirac point, however the vHs-stripes appear in the bulk. We interpret the states as lines of cell-tilting vibrations, and inspect their stability in the large lattice-size limit. The model can be experimentally realized by superconducting 2D microwave resonators containing triangular lattices of metallic cylinders, which simulate finite-sized graphene flakes. Thus we can assume that the effects discussed here could be experimentally observed.
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Concentrating on bosonic lattice systems, we ask whether and how Excited State Quantum Phase Transition (ESQPT) singularities occur in condensed matter systems with ground state QPTs. We study in particular the spectral singularities above the ground-state phase diagram of the boson Hubbard model. As a general prerequisite, we point out the analogy between ESQPTs and van Hove singularities (vHss).
Understanding and tuning correlated states is of great interest and significance to modern condensed matter physics. The recent discovery of unconventional superconductivity and Mott-like insulating states in magic-angle twisted bilayer graphene (tBLG) presents a unique platform to study correlation phenomena, in which the Coulomb energy dominates over the quenched kinetic energy as a result of hybridized flat bands. Extending this approach to the case of twisted multilayer graphene would allow even higher control over the band structure because of the reduced symmetry of the system. Here, we study electronic transport properties in twisted trilayer graphene (tTLG, bilayer on top of monolayer graphene heterostructure). We observed the formation of van Hove singularities which are highly tunable by twist angle and displacement field and can cause strong correlation effects under optimum conditions, including superconducting states. We provide basic theoretical interpretation of the observed electronic structure.
Electronic instabilities at the crossing of the Fermi energy with a Van Hove singularity in the density of states often lead to new phases of matter such as superconductivity, magnetism or density waves. However, in most materials this condition is difficult to control. In the case of single-layer graphene, the singularity is too far from the Fermi energy and hence difficult to reach with standard doping and gating techniques. Here we report the observation of low-energy Van Hove singularities in twisted graphene layers seen as two pronounced peaks in the density of states measured by scanning tunneling spectroscopy. We demonstrate that a rotation between stacked graphene layers can generate Van Hove singularities, which can be brought arbitrarily close to the Fermi energy by varying the angle of rotation. This opens intriguing prospects for Van Hove singularity engineering of electronic phases.
Extensive scanning tunnelling microscopy and spectroscopy experiments complemented by first principles and parameterized tight binding calculations provide a clear answer to the existence, origin and robustness of van Hove singularities (vHs) in twisted graphene layers. Our results are conclusive: vHs due to interlayer coupling are ubiquitously present in a broad range (from 1{deg} to 10{deg}) of rotation angles in our graphene on 6H-SiC(000-1) samples. From the variation of the energy separation of the vHs with rotation angle we are able to recover the Fermi velocity of a graphene monolayer as well as the strength of the interlayer interaction. The robustness of the vHs is assessed both by experiments, which show that they survive in the presence of a third graphene layer, and calculations, which test the role of the periodic modulation and absolute value of the interlayer distance. Finally, we clarify the origin of the related moire corrugation detected in the STM images.
We study distributions of the ratios of level spacings of a rectangular and an Africa-shaped superconducting microwave resonator containing circular scatterers on a triangular grid, so-called Dirac billiards (DBs). The high-precision measurements allowed the determination of all 1651 and 1823 eigenfrequencies in the first two bands, respectively. The resonance densities are similar to that of graphene. They exhibit two sharp peaks at the van Hove singularities, that separate the band structure into regions with a linear and a quadratic dispersion relation, respectively. In their vicinity we observe rapid changes, e.g., in the wavefunction structure. Accordingly, the question arose, whether there the spectral properties are still determined by the shapes of the DBs. The commonly used statistical measures, however, are no longer applicable whereas, as demonstrated in this Letter, the ratio distributions provide most suitable ones.
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