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Register a new userCharacterization of Gadolinium-loaded Plastic Scintillator for Use as a Neutron Veto
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David-Michael Poehlmann
Publication date
2018
fields
Physics
and research's language is
English
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Scintillator doped with a high neutron-capture cross-section material can be used to detect neutrons via their resulting gamma rays. Examples of such detectors using liquid scintillator have been successfully used in high-energy physics experiments. However, a liquid scintillator can leak and is not as amenable to modular or complex shapes as a solid scintillator. Polystyrene-based scintillators from a variety of gadolinium compounds with varying concentrations were polymerized in our laboratory. The light output, emission spectra, and attenuation length of our samples were measured and light collection strategies using a wavelength shifting (WLS) fiber were evaluated. The measured optical parameters were used to tune a Geant4-based optical Monte Carlo, enabling the trapping efficiency to be calculated. This technology was also evaluated as a possible neutron veto for the direct detection dark matter experiment, Super Cryogenic Dark Matter Search (SuperCDMS).
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Organic scintillators doped with capture agents provide a detectable signal for neutrons over a broad energy range. This work characterizes the fast and slow neutron response of EJ-254, an organic plastic scintillator with 5% natural boron loading by weight. For fast neutrons, the primary mechanism for light generation in organic scintillators is n-p elastic scattering. To study the fast neutron response, the proton light yield of EJ-254 was measured at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a broad-spectrum neutron source and a double time-of-flight technique, the EJ-254 proton light yield was obtained over the energy range of approximately 270 keV to 4.5 MeV and determined to be in agreement with other plastic scintillators comprised of the same polymer base. To isolate the slow neutron response, an AmBe source with polyethylene moderator was made incident on the EJ-254 scintillator surrounded by an array of EJ-309 observation detectors. Events in the EJ-254 target coincident with the signature 477.6 keV $gamma$ ray (resulting from deexcitation of the residual $^{7}$Li nucleus following boron neutron capture) were identified. Pulse shape discrimination was used to evaluate the temporal differences in the response of EJ-254 scintillation signals arising from $gamma$-ray and fast/slow neutron interactions. Clear separation between $gamma$-ray and fast neutrons signals was not achieved and the neutron capture feature was observed to overlap both the $gamma$-ray and fast neutron bands. Taking into account the electron light nonproportionality, the neutron-capture light yield in EJ-254 was determined to be 89.4$pm$1.1 keVee.
We present an in-situ method of measuring the relative attenuation length of gadolinium-loaded liquid scintillator in the RENO detectors using radioactive source calibration data without requiring any PMT performance model. We observed the degradation of the attenuation length of the gadolinium-loaded liquid scintillator in the RENO detectors by ~50% over a period of about 4 years.
A new experiment, which is called as NEOS (NEutrino Oscillation at Short baseline), is proposed on the site of Hanbit reactors at Yonggwang, South Korea, to investigate a reactor antineutrino anomaly. A homogeneous NEOS detector having a 1000-L target volume has been constructed and deployed at the tendon gallery ~25 m away from the reactor core. A linear alkylbenzene (LAB) is used as a main base solvent of the NEOS detector. Furthermore, a di-isopropylnaphthalene (DIN) is added to improve the light output and pulse shape discrimination (PSD) ability. The ratio of LAB to DIN is 90:10. PPO (3 g/L) and bis-MSB (30 mg/L) are dissolved to formulate the mixture of LAB- and DIN-based liquid scintillator (LS). Then, ~0.5% gadolinium (Gd) is loaded into the LS by using the solvent-solvent extraction technique. In this paper, we report the characteristics of Gd-loaded LS (GdLS) for the NEOS detector and the handling during mass production.
We developed a segmented reactor-antineutrino detector made of plastic scintillators for application as a tool in nuclear safeguards inspection and performed mostly unmanned field operations at a commercial power plant reactor. At a position outside the reactor building, we measured the difference in reactor antineutrino flux above the ground when the reactor was active and inactive.
This paper describes the design and performance of a 50 liter, two-segment $^{6}$Li-loaded liquid scintillator detector that was designed and operated as prototype for the PROSPECT (Precision Reactor Oscillation and Spectrum) Experiment. The two-segment detector was constructed according to the design specifications of the experiment. It features low-mass optical separators, an integrated source and optical calibration system, and materials that are compatible with the $^{6}$Li-doped scintillator developed by PROSPECT. We demonstrate a high light collection of 850$pm$20 PE/MeV, an energy resolution of $sigma$ = 4.0$pm$0.2% at 1 MeV, and efficient pulse-shape discrimination of low $dE/dx$ (electronic recoil) and high $dE/dx$ (nuclear recoil) energy depositions. An effective scintillation attenuation length of 85$pm$3 cm is measured in each segment. The 0.1% by mass concentration of $^{6}$Li in the scintillator results in a measured neutron capture time of $tau$ = 42.8$pm$0.2 $mu s$. The long-term stability of the scintillator is also discussed. The detector response meets the criteria necessary for achieving the PROSPECT physics goals and demonstrates features that may find application in fast neutron detection.
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