Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userFrustrated Magnetism from Local Moments in FeSe
129
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
We investigate properties of a spin-1 Heisenberg model with extended and biquadratic interactions, which captures crucial aspects of the low energy physics in FeSe. While we show that the model exhibits a rich phase diagram with four different magnetic ordering tendencies, we identify a parameter regime with strong competition between N`eel, staggered dimer, and stripe-like magnetic fluctuations, accounting for the physical properties of FeSe. Through the comparison of numerically evaluated spin and Raman response with experiments, we find evidence for enhanced magnetic frustration between N`eel and co-linear stripe ordering tendencies, which increases with increasing temperature. The explanation of these spectral behaviors with this frustrated spin model supports the idea of local spin interactions in FeSe.
rate research
Read More
Recently measurements on various spin-1/2 quantum magnets such as H$_3$LiIr$_2$O$_6$, LiZn$_2$Mo$_3$O$_8$, ZnCu$_3$(OH)$_6$Cl$_2$ and 1T-TaS$_2$ -- all described by magnetic frustration and quenched disorder but with no other common relation -- nevertheless showed apparently universal scaling features at low temperature. In particular the heat capacity C[H,T] in temperature T and magnetic field H exhibits T/H data collapse reminiscent of scaling near a critical point. Here we propose a theory for this scaling collapse based on an emergent random-singlet regime extended to include spin-orbit coupling and antisymmetric Dzyaloshinskii-Moriya (DM) interactions. We derive the scaling $C[H,T]/T sim H^{-gamma} F_q[T/H]$ with $F_q[x] = x^{q}$ at small $x$, with $q in$ (0,1,2) an integer exponent whose value depends on spatial symmetries. The agreement with experiments indicates that a fraction of spins form random valence bonds and that these are surrounded by a quantum paramagnetic phase. We also discuss distinct scaling for magnetization with a $q$-dependent subdominant term enforced by Maxwells relations.
Understanding the origin of the magnetism of high temperature superconductors is crucial for establishing their unconventional pairing mechanism. Recently, theory predicts that FeSe is close to a magnetic quantum critical point, and thus weak perturbations such as impurities could induce local magnetic moments. To elucidate such quantum instability, we have employed scanning tunneling microscopy and spectroscopy. In particular, we have grown FeSe film on superconducting Pb(111) using molecular beam epitaxy and investigated magnetic excitation caused by impurities in the proximity-induced superconducting gap of FeSe. Our study provides a deep insight into the origin of the magnetic ordering of FeSe by showing the way local magnetic moments develop in response to impurities near the magnetic quantum critical point.
Recently synthesized metastable tetragonal CoSe, isostructural to the FeSe superconductor, offers a new avenue for investigating systems in close proximity to the iron-based superconductors. We present magnetic and transport property measurements on powders and single crystals of CoSe. High field magnetic susceptibility measurements indicate a suppression of the previously reported 10 K ferromagnetic transition with the magnetic susceptibility exhibiting time-dependence below the proposed transition. Dynamic scaling analysis of the time-dependence yields a critical relaxation time of $tau^{*} = 0.064 pm 0.008 $ s which in turn yields an activation energy of $E_{a}^{*}$ = 14.84 $pm$ 0.59 K and an ideal glass temperature $T_{0}^{*}$ = 8.91 $pm$ 0.09 K from Vogel-Fulcher analysis. No transition is observed in resistivity and specific heat measurements, but both measurements indicate that CoSe is metallic. These results are interpreted on the basis of CoSe exhibiting frustrated magnetic ordering arising from competing magnetic interactions. Arrott analysis of single crystal magnetic susceptibility has indicated that the magnetic moments lie in the $ab$-plane so frustration may arise from intralayer magnetic fluctuations as well as interlayer coupling. The results have implications for understanding the superconductivity in the iron chalcogenide systems as well as utilizing CoSe as a host for chemical and physical manipulation to tune and explore emergent phenomena within an expanding new class of transition metal chalcogenides.
The charge and spin dynamics of the structurally simplest iron-based superconductor, FeSe, may hold the key to understanding the physics of high temperature superconductors in general. Unlike the iron pnictides, FeSe lacks long range magnetic order in spite of a similar structural transition around 90,K. Here, we report results of Raman scattering experiments as a function of temperature and polarization and simulations based on exact diagonalization of a frustrated spin model. Both experiment and theory find a persistent low energy peak close to 500cm$^{-1}$ in $B_{1g}$ symmetry, which softens slightly around 100,K, that we assign to spin excitations. By comparing with results from neutron scattering, this study provides evidence for nearly frustrated stripe order in FeSe.
Identifying the time reversal symmetry of spins as a symplectic symmetry, we develop a large N approximation for quantum magnetism that embraces both antiferromagnetism and ferromagnetism. In SU(N), N>2, not all spins invert under time reversal, so we have introduced a new large N treatment which builds interactions exclusively out of the symplectic subgroup [SP(N)] of time reversing spins, a more stringent condition than the symplectic symmetry of previous SP(N) large N treatments. As a result, we obtain a mean field theory that incorporates the energy cost of frustrated bonds. When applied to the frustrated square lattice, the ferromagnetic bonds restore the frustration dependence of the critical spin in the Neel phase, and recover the correct frustration dependence of the finite temperature Ising transition.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
