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Register a new userAtomic-scale tailoring of spin susceptibility via non-magnetic spin-orbit impurities
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Following the discovery of topological insulators, there has been a renewed interest in superconducting systems that have strong spin-orbit (SO) coupling. Here we address the fundamental question of how the spin properties of a otherwise spin-singlet superconducting ground state evolve with increasing SO impurity density. We have mapped out the Zeeman critical field phase diagram of superconducting Al films that were deposited over random Pb cluster arrays of varying density. These phase diagrams give a direct measure of the Fermi liquid spin renormalization, as well as the spin orbit scattering rate. We find that the spin renormalization is a linear function of the average Pb cluster-to-cluster separation and that this dependency can be used to tune the spin susceptibility of the Al over a surprisingly wide range from 0.8$chi_0$ to 4.0$chi_0$, where $chi_0$ is the non-interacting Pauli susceptibility.
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The influence of La non magnetic impurities on the spin dynamics of CeCoIn$_{5}$ was studied by inelastic neutron scattering. In La-substituted systems, the spin resonance peak (observed at $Omega_{res}=0.55 meV$ in the pure system) is shifted to lower energies but the ratio $Omega_{res}/k_{B}T_{c}$ remains unchanged. The excitation broadens till it reaches 0.3 meV equal to the value of the quasi-elastic signal in the normal state. The evolution of La substitution is compared with the evolution of the magnetic resonance in Ni and Zn substituted YBa$_{2}$Cu$_{3}$O$_{7}$.
Magnetic anisotropy (MA) is one of the most important material properties for modern spintronic devices. Conventional manipulation of the intrinsic MA, i.e. magnetocrystalline anisotropy (MCA), typically depends upon crystal symmetry. Extrinsic control over the MA is usually achieved by introducing shape anisotropy or exchange bias from another magnetically ordered material. Here we demonstrate a pathway to manipulate MA of 3d transition metal oxides (TMOs) by digitally inserting non-magnetic 5d TMOs with pronounced spin-orbit coupling (SOC). High quality superlattices comprised of ferromagnetic La2/3Sr1/3MnO3 (LSMO) and paramagnetic SrIrO3 (SIO) are synthesized with the precise control of thickness at atomic scale. Magnetic easy axis reorientation is observed by controlling the dimensionality of SIO, mediated through the emergence of a novel spin-orbit state within the nominally paramagnetic SIO.
The effect of non-magnetic impurities is discussed for both the two-leg Heisenberg ladder system and other spin liquids with excitation gap. It is shown that the random depletion of spins introduces a random Berry phase term to the non-linear sigma model. The classical nature of the antiferromagnetic correlation is enhanced by the topological decoherence, and the staggered susceptibility shows more singular behavior at low temperatures than the uniform antiferromagnetic Heisenberg chain.
We calcuate electronic spin susceptibility and spin-lattice relaxation rate in singlet superconductor near a pairbreaking surface, or in a domain wall of the order parameter. We directly link presence of high-density Andreev bound states in the inhomogeneous region, combined with coherence factors, to enhancement of the susceptibility above the normal states value for certain $bf q$ vectors. Beside the dominant peak at ferromagnetic vector $q=0$, we find significant enhancement of antiferromagnetic correlations at vectors $qlesssim 2 k_f$, with $bf q$ $along$ the domain wall in $S$-wave superconductor, and $across$ domain wall in $D$-wave (nodes along the wall). These features are destroyed by applying moderate Zeeman field that splits the zero-energy peak. We solve Bogoliubov-de Gennes equations in momentum space and our results deviate from the lattice models investigated previously. Large enhancement of the spin-lattice relaxation rate $T_1^{-1}$ at the domain wall provides clear signature of the quasiparticle bound states, and is in good agreement with recent experiment in organic superconductor $kappa$-(BEDT-TTF)$_2$Cu(NCS)$_2$.
Spin susceptibility of Anderson impurities is a key quantity in understanding the physics of Kondo screening. Traditional numerical renormalization group (NRG) calculation of the impurity contribution $chi_{textrm{imp}}$ to susceptibility, defined originally by Wilson in a flat wide band, has been generalized before to structured conduction bands. The results brought about non-Fermi-liquid and diamagnetic Kondo behaviors in $chi_{textrm{imp}}$, even when the bands are not gapped at the Fermi energy. Here, we use the full density-matrix (FDM) NRG to present high-quality data for the local susceptibility $chi_{textrm{loc}}$ and to compare them with $chi_{textrm{imp}}$ obtained by the traditional NRG. Our results indicate that those exotic behaviors observed in $chi_{textrm{imp}}$ are unphysical. Instead, the low-energy excitations of the impurity in arbitrary bands only without gap at the Fermi energy are still a Fermi liquid and paramagnetic. We also demonstrate that unlike the traditional NRG yielding $chi_{textrm{loc}}$ less accurate than $chi_{textrm{imp}}$, the FDM method allows a high-precision dynamical calculation of $chi_{textrm{loc}}$ at much reduced computational cost, with an accuracy at least one order higher than $chi_{textrm{imp}}$. Moreover, artifacts in the FDM algorithm to $chi_{textrm{imp}}$, and origins of the spurious non-Fermi-liquid and diamagnetic features are clarified. Our work provides an efficient high-precision algorithm to calculate the spin susceptibility of impurity for arbitrary structured bands, while negating the applicability of Wilsons definition to such cases.
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