Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userTuning toroidal dipole resonances in dielectric metamolecules by an additional electric dipolar response
66
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
With the rise of artificial magnetism and metamaterials, the toroidal family recently attracts more attention for its unique properties. Here we propose an all-dielectric pentamer metamolecule consisting of nano-cylinders with two toroidal dipolar resonances, whose frequencies, EM distributions and Q factor can be efficiently tuned due to the additional electric dipole mode offered by a central cylinder. To further reveal the underlying coupling effects and formation mechanism of toroidal responses, the multiple scattering theory is adopted. It is found that the first toroidal dipole mode, which can be tuned from 2.21 to 3.55 $mu$m, is mainly induced by a collective electric dipolar resonance, while the second one, which can be tuned from 1.53 to 1.84 $mu$m, relies on the cross coupling of both electric and magnetic dipolar responses. The proposed low-loss metamolecule and modes coupling analyses may pave the way for active design of toroidal responses in advanced optical devices.
rate research
Read More
We demonstrate that the toroidal dipolar response can be realized in the optical regime by designing a feasible nanostructured metamaterial, comprising asymmetric double-bar magnetic resonators assembled into a toroid-like configuration. It is confirmed numerically that an optical toroidal dipolar moment dominates over other moments. This response is characterized by a strong confinement of an E-field component at the toroid center, oriented perpendicular to the H-vortex plane. The resonance-enhanced optical toroidal response can provide an experimental avenue for various interesting optical phenomena associated with the elusive toroidal moment.
The toroidal response is numerically investigated in a multifold double-ring metamaterials at the antibonding magnetic-dipole mode (i.e., antiparallel magnetic dipoles in one double-ring fold). This intriguing toroidal resonance in metamaterials is considered as a result of the magnetoelectric effect due to the broken balance of the electric near-field environment. We demonstrate that the toroidal dipole response in metamaterials can improve the quality factor of the resonance spectrum. In viewing of the design flexibility on the double-ring geometry, such toroidal metamaterials will offer advantages in application potentials of toroidal dipolar moment.
We demonstrate hierarchical assembly of plasmonic toroidal metamolecules, which exhibit tailored optical activity in the visible spectral range. Each metamolecule consists of four identical origami-templated helical building blocks. Such toroidal metamolecules show stronger chiroptical response than monomers and dimers of the helical building blocks. Enantiomers of the plasmonic structures yield opposite circular dichroism spectra. The experimental results agree well with the theoretical simulations. We also demonstrate that given the circular symmetry of the structures, distinct chiroptical response along their axial orientation can be uncovered via simple spin-coating of the metamolecules on substrates. Our work provides a new strategy to create plasmonic chiral platforms with sophisticated nanoscale architectures for potential applications such as chiral sensing using chemically-based assembly systems.
Selective configuration control of plasmonic nanostructures using either top-down or bottom-up approaches has remained challenging in the field of active plasmonics. We demonstrate the realization of DNA-assembled reconfigurable plasmonic metamolecules, which can respond to a wide range of pH changes in a programmable manner. This programmability allows for selective reconfiguration of different plasmonic metamolecule species coexisting in solution through simple pH tuning. This approach enables discrimination of chiral plasmonic quasi-enantiomers and arbitrary tuning of chiroptical effects with unprecedented degrees of freedom. Our work outlines a new blueprint for implementation of advanced active plasmonic systems, in which individual structural species can be programmed to perform multiple tasks and functions in response to independent external stimuli.
Hybrid dielectric metasurfaces have emerged as a promising approach to enhancing near field confinement and thus achieving high optical nonlinearity using low loss dielectrics. Additional flexibility in design and fabrication of hybrid metasurfaces allows dynamic control of light, which is value-added for a wider range of applications. Here, we demonstrate a tunable and efficient third harmonic generation (THG) via hybrid metasurfaces with phase change material Ge2Sb2Te5 (GST) deposited on top of amorphous silicon nanostructutes. Fano resonance is excited to confine the incident light inside the hybrid metasurfaces, and an experimental quality factor ($Q$-factor) of 125 is achieved at the fundamental pump wavelength around 1210 nm. We demonstrate the switching between a turn-on state of Fano resonance in the amorphous state of GST and a turn-off state in its crystalline state and also gradual multistate tuning of THG emission at its intermediate state. We achieve a high THG conversion efficiency of ${eta} = 2.9*10^{-6}$ %, which is more than ~32 times of that of a GST-based Fabry-P`erot cavity under a similar pump laser power, thanks to the enhanced field confinement due to the Fano resonance. Our results show the strong potential of GST-based hybrid dielectric metasurfaces for efficient and tunable nonlinear optical devices.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
