No Arabic abstract
The phase diagrams of the frustrated classical spin model with Dzyaloshinskii-Moriya (DM) interaction on the Shastry-Sutherland (S-S) lattice are studied by means of Monte Carlo simulation. For ferromagnetic next-nearest-neighboring (J2) interactions, the introduced exchange frustration enhances the effect of the DM interaction, which enlarges the magnetic field-range with the skyrmion lattice phase and increases the skyrmion density. For antiferromagnetic J2 interactions, the so-called 2q phase (two-sublattice skyrmion crystal) and the spin-flop phase are observed in the simulated phase diagram, and their stabilizations are closely dependent on the DM interaction and J2 interaction, respectively. The simulated results are qualitatively explained from the energy landscape, which provides useful information for understanding the intriguing phases in S-S magnets.
Weyl semimetal is a topologically non-trivial phase of matter with pairs of Weyl nodes in the k-space, which act as monopole and anti-monopole pairs of Berry curvature. Two hallmarks of the Weyl metallic state are the topological surface state called the Fermi arc and the chiral anomaly. It is known that the chiral anomaly yields anomalous magneto-transport phenomena. In this study, we report the emergence of the type-II Weyl semimetallic state in the geometrically frustrated non-collinear antiferromagnetic Shastry-Sutherland lattice (SSL) GdB4 crystal. When we apply magnetic fields perpendicular to the noncollinear moments in SSL plane, Weyl nodes are created above and below the Fermi energy along the M-A line (tau-band) because the spin tilting breaks the time-reversal symmetry and lifts band degeneracy while preserving C4z or C2z symmetry. The unique electronic structure of GdB4 under magnetic fields applied perpendicular to the SSL gives rise to a non-trivial Berry phase, detected in de Haas-van Alphen experiments and chiral-anomaly-induced negative magnetoresistance. The emergence of the magnetic field-induced Weyl state in SSL presents a new guiding principle to develop novel types of Weyl semimetals in frustrated spin systems.
We show that temperature and magnetic field properties of the entanglement between spins on the two-dimensional Shastry-Sutherland lattice can be qualitatively described by analytical results for a qubit tetramer. Exact diagonalization of clusters with up to 20 sites reveals that the regime of fully entangled neighboring pairs coincides with the regime of finite spin gap in the spectrum. Additionally, the results for the regime of vanishing spin gap are discussed and related to the Heisenberg limit of the model.
Frustration represents an essential feature in the behavior of magnetic materials when constraints on the microscopic Hamiltonian cannot be satisfied simultaneously. This gives rise to exotic phases of matter including spin liquids, spin ices, and stripe phases. Here we demonstrate an approach to understanding the microscopic effects of frustration by computing the phases of a 468-spin Shastry-Sutherland Ising Hamiltonian using a quantum annealer. Our approach uses mean-field boundary conditions to mitigate effects of finite size and defects alongside an iterative quantum annealing protocol to simulate statistical physics. We recover all phases of the Shastry-Sutherland Ising model -- including the well-known fractional magnetization plateau -- and the static structure factor characterizing the critical behavior at these transitions. These results establish quantum annealing as an emerging method in understanding the effects of frustration on the emergence of novel phases of matter and pave the way for future comparisons with real experiments.
We studied the electronic structure of a Shastry-Sutherland lattice system, HoB4 employing high resolution photoemission spectroscopy and ab initio band structure calculations. The surface and bulk borons exhibit subtle differences, and loss of boron compared to the stoichiometric bulk. However, the surface and bulk conduction bands near Fermi level are found to be similar. Evolution of the electronic structure with temperature is found to be similar to that observed in a typical charge-disordered system. A sharp dip is observed at the Fermi level in the low temperature spectra revealing signature of antiferromagnetic gap. Asymmetric spectral weight transfer with temperature manifests particle-hole asymmetry that may be related to the exotic properties of these systems.
The Shastry-Sutherland model and its generalizations have been shown to capture emergent complex magnetic properties from geometric frustration in several quasi-two-dimensional quantum magnets. Using an $sd$ exchange model, we show here that metallic Shastry-Sutherland magnets can exhibit topological Hall effect driven by magnetic skyrmions under realistic conditions. The magnetic properties are modelled with competing symmetric Heisenberg and asymmetric Dzyaloshinskii-Moriya exchange interactions, while a coupling between the spins of the itinerant electrons and the localized moments describes the magnetotransport behavior. Our results, employing complementary Monte Carlo simulations and a novel machine learning analysis to investigate the magnetic phases, provide evidence for field-driven skyrmion crystal formation for extended range of Hamiltonian parameters. By constructing an effective tight-binding model of conduction electrons coupled to the skyrmion lattice, we clearly demonstrate the appearance of topological Hall effect. We further elaborate on effects of finite temperatures on both magnetic and magnetotransport properties.