The dimension of the state space for information encoding offered by the transverse structure of light is usually limited by the finite size of apertures. The widely used orbital angular momentum (OAM) number of Laguerre-Gaussian (LG) modes in free-space communications cannot achieve the theoretical maximum transmission capacity unless the radial degree of freedom is multiplexed into the protocol. While the methodology to sort the radial quantum number has been developed, the application of radial modes in quantum communications requires an additional ability to efficiently measure the superposition of LG modes in the mutually unbiased basis. Here we develop and implement a generic mode sorter that is capable of sorting the superposition of LG modes through the use of a mode converter. As a consequence, we demonstrate an 8-dimensional quantum key distribution experiment involving all three transverse degrees of freedom: spin, azimuthal, and radial quantum numbers of photons. Our protocol presents an important step towards the goal of reaching the capacity limit of a free-space link and can be useful to other applications that involve spatial modes of photons.
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