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Fast-responding detector arrays are commonly used for imaging rapidly-changing scenes. Besides array detectors, a single-pixel detector combined with a broadband optical spectrum can also be used for rapid imaging by mapping the spectrum into a spatial coordinate grid and then rapidly measuring the spectrum. Here, optical frequency combs generated from high-$Q$ silica microresonators are used to implement this method. The microcomb is dispersed in two spatial dimensions to measure a test target. The target-encoded spectrum is then measured by multi-heterodyne beating with another microcomb having a slightly different repetition rate, enabling an imaging frame rate up to 200 kHz and fillrates as high as 48 MegaPixels/s. The system is used to monitor the flow of microparticles in a fluid cell. Microcombs in combination with a monolithic waveguide grating array imager could greatly magnify these results by combining the spatial parallelism of detector arrays with spectral parallelism of optics.
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Rapid and large scanning of a dissipative Kerr-microresonator soliton comb with the characterization of all comb modes along with the separation of the comb modes is imperative for the emerging applications of the frequency-scanned soliton combs. However, the scan speed is limited by the gain of feedback systems and the measurement of the frequency shift of all comb modes has not been demonstrated. To overcome the limitation of the feedback, we incorporate the feedback with the feedforward. With the additional gain of > 40 dB by a feedforward signal, a dissipative Kerr-microresonator soliton comb is scanned by 70 GHz in 500 $mu$s, 50 GHz in 125 $mu$s, and 25 GHz in 50 $mu$s (= 500 THz/s). Furthermore, we propose and demonstrate a method to measure the frequency shift of all comb modes, in which an imbalanced Mach-Zehnder interferometer with two outputs with different wavelengths is used. Because of the two degrees of freedom of optical frequency combs, the measurement at the two different wavelengths enables the estimation of the frequency shift of all comb modes.
Cavity ring-down spectroscopy is a ubiquitous optical method used to study light-matter interactions with high resolution, sensitivity and accuracy. However, it has never been performed with the multiplexing advantages of direct frequency comb spectroscopy without sacrificing orders of magnitude of resolution. We present dual-comb cavity ring-down spectroscopy (DC-CRDS) based on the parallel heterodyne detection of ring-down signals with a local oscillator comb to yield absorption and dispersion spectra. These spectra are obtained from widths and positions of cavity modes. We present two approaches which leverage the dynamic cavity response to coherently or randomly driven changes in the amplitude or frequency of the probe field. Both techniques yield accurate spectra of methane - an important greenhouse gas and breath biomarker. The high sensitivity and accuracy of broadband DC-CRDS, shows promise for applications like studies of the structure and dynamics of large molecules, multispecies trace gas detection and isotopic composition.
With demonstrated applications ranging from metrology to telecommunications, soliton microresonator frequency combs have emerged over the past decade as a remarkable new technology. However, standard implementations only allow for the generation of combs whose repetition rate is tied close to the fundamental resonator free-spectral range (FSR), offering little or no dynamic control over the comb line spacing. Here we propose and experimentally demonstrate harmonic and rational harmonic driving as novel techniques that allow for the robust generation of soliton frequency combs with discretely adjustable frequency spacing. By driving an integrated Kerr microresonator with a periodic train of picosecond pulses whose repetition rate is set close to an integer harmonic of the 3.23 GHz cavity FSR, we deterministically generate soliton frequency combs with frequency spacings discretely adjustable between 3.23 GHz and 19.38 GHz. More remarkably, we also demonstrate that driving the resonator at rational fractions of the FSR allows for the generation of combs whose frequency spacing corresponds to an integer harmonic of the pump repetition rate. By measuring the combs radio-frequency spectrum, we confirm operation in the low-noise soliton regime with no supermode noise. The novel techniques demonstrated in our work provide new degrees of freedom for the design of synchronously pumped soliton frequency combs.
Four-wave-mixing-based quantum cascade laser frequency combs (QCL-FC) are a powerful photonic tool, driving a recent revolution in major molecular fingerprint regions, i.e. mid- and far-infrared domains. Their compact and frequency-agile design, together with their high optical power and spectral purity, promise to deliver an all-in-one source for the most challenging spectroscopic applications. Here, we demonstrate a metrological-grade hybrid dual comb spectrometer, combining the advantages of a THz QCL-FC with the accuracy and absolute frequency referencing provided by a free-standing, optically-rectified THz frequency comb. A proof-of-principle application to methanol molecular transitions is presented. The multi-heterodyne molecular spectra retrieved provide state-of-the-art results in line-center determination, achieving the same precision as currently available molecular databases. The devised setup provides a solid platform for a new generation of THz spectrometers, paving the way to more refined and sophisticated systems exploiting full phase control of QCL-FCs, or Doppler-free spectroscopic schemes.
Dissipative solitons are stable localized coherent structures with linear frequency chirp generated in normal-dispersion mode-locked lasers. The soliton energy in fiber lasers is limited by the Raman effect, but implementation of intracavity feedback for the Stokes wave enables synchronous generation of a coherent Raman dissipative soliton. Here we demonstrate a new approach for generating chirped pulses at new wavelengths by mixing in a highly-nonlinear fiber of two frequency-shifted dissipative solitons, as well as cascaded generation of their clones forming a dissipative soliton comb in the frequency domain. We observed up to eight equidistant components in a 400-nm interval demonstrating compressibility from ~10 ps to ~300 fs. This approach, being different from traditional frequency combs, can inspire new developments in fundamental science and applications.
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