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Register a new userThermal Diffusivity Above Mott-Ioffe-Regel Limit
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We present high-resolution thermal diffusivity measurements on several near optimally doped electron- and hole-doped cuprate systems in a temperature range that passes through the Mott-Ioffe-Regel limit, above which the quasiparticle picture fails. Our primary observations are that the inverse thermal diffusivity is linear in temperature and can be fitted to $D_Q^{-1}=aT+b$. The slope $a$ is interpreted through the Planckian relaxation time $tauapproxhbar/k_BT$ and a thermal diffusion velocity $v_B$, which is close, but larger than the sound velocity. The intercept $b$ represent a crossover diffusion constant that separates coherent from incoherent quasiparticles. These observations suggest that both phonons and electrons participate in the thermal transport, while reaching the Planckian limit for relaxation time.
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The absence of resistivity saturation in many strongly correlated metals, including the high-temperature superconductors, is critically examined from the viewpoint of optical conductivity measurements. Coherent quasiparticle conductivity, in the form of a Drude peak centred at zero frequency, is found to disappear as the mean free path (at $omega$ = 0) becomes comparable to the interatomic spacing. This basic loss of coherence at the so-called Mott-Ioffe-Regel (MIR) limit suggests that the universality of the MIR criterion is preserved even in the presence of strong electron correlations. We argue that the shedding of spectral weight at low frequencies, induced by strong correlation effects, is the primary origin of the extended positive slope of the resistivity to high temperatures observed in all so-called bad metals. Moreover, in common with those metals which exhibit resistivity saturation at high temperatures, the scattering rate itself, as extracted from optical spectra, saturates at a value consistent with the MIR limit. We consider possible implications that this ceiling in the scattering rate may have for our understanding of transport within a wide variety of bad metals and suggest a better method for analysing their optical response.
Many metals display resistivity saturation - a substantial decrease in the slope of the resistivity as a function of temperature, that occurs when the electron scattering rate $tau^{-1}$ becomes comparable to the Fermi energy $E_F/hbar$ (the Mott-Ioffe-Regel limit). At such temperatures, the usual description of a metal in terms of ballistically propagating quasiparticles is no longer valid. We present a tractable model of a large $N$ number of electronic bands coupled to $N^2$ optical phonon modes, which displays a crossover behavior in the resistivity at temperatures where $tau^{-1}sim E_F/hbar$. At low temperatures, the resistivity obeys the familiar linear form, while at high temperatures, the resistivity still increases linearly, but with a modified slope (that can be either lower or higher than the low-temperature slope, depending on the band structure). The high temperature non-Boltzmann regime is interpreted by considering the diffusion constant and the compressibility, both of which scale as the inverse square root of the temperature.
We show that viscoelastic effects play a crucial role in the damping of vibrational modes in harmonic amorphous solids. The relaxation of a given plane wave is described by a memory function of a semi-infinite one-dimensions mass-spring chain. The initial vibrational energy spreads from the first site of the chain to infinity. In the beginning of the chain, there is a barrier, which significantly reduces the decay of vibrational energy below the Ioffe-Regel frequency. To obtain the parameters of the chain, we present a numerically stable method, based on the Chebyshev expansion of the local vibrational density of states.
We consider diffusion of vibrations in 3d harmonic lattices with strong force-constant disorder. Above some frequency w_IR, corresponding to the Ioffe-Regel crossover, notion of phonons becomes ill defined. They cannot propagate through the system and transfer energy. Nevertheless most of the vibrations in this range are not localized. We show that they are similar to diffusons introduced by Allen, Feldman et al., Phil. Mag. B 79, 1715 (1999) to describe heat transport in glasses. The crossover frequency w_IR is close to the position of the boson peak. Changing strength of disorder we can vary w_IR from zero value (when rigidity is zero and there are no phonons in the lattice) up to a typical frequency in the system. Above w_IR the energy in the lattice is transferred by means of diffusion of vibrational excitations. We calculated the diffusivity of the modes D(w) using both the direct numerical solution of Newton equations and the formula of Edwards and Thouless. It is nearly a constant above w_IR and goes to zero at the localization threshold. We show that apart from the diffusion of energy, the diffusion of particle displacements in the lattice takes place as well. Above w_IR a displacement structure factor S(q,w) coincides well with a structure factor of random walk on the lattice. As a result the vibrational line width Gamma(q)=D_u q^2 where D_u is a diffusion coefficient of particle displacements. Our findings may have important consequence for the interpretation of experimental data on inelastic x-ray scattering and mechanisms of heat transfer in glasses.
We establish a phase diagram of a model in which scalar waves are scattered by resonant point scatterers pinned at random positions in the free three-dimensional (3D) space. A transition to Anderson localization takes place in a narrow frequency band near the resonance frequency provided that the number density of scatterers $rho$ exceeds a critical value $rho_c simeq 0.08 k_0^{3}$, where $k_0$ is the wave number in the free space. The localization condition $rho > rho_c$ can be rewritten as $k_0 ell_0 < 1$, where $ell_0$ is the on-resonance mean free path in the independent-scattering approximation. At mobility edges, the decay of the average amplitude of a monochromatic plane wave is not purely exponential and the growth of its phase is nonlinear with the propagation distance. This makes it impossible to define the mean free path $ell$ and the effective wave number $k$ in a usual way. If the latter are defined as an effective decay length of the intensity and an effective growth rate of the phase of the average wave field, the Ioffe-Regel parameter $(kell)_c$ at the mobility edges can be calculated and takes values from 0.3 to 1.2 depending on $rho$. Thus, the Ioffe-Regel criterion of localization $kell < (kell)_c = mathrm{const} sim 1$ is valid only qualitatively and cannot be used as a quantitative condition of Anderson localization in 3D.
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