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Register a new userMicron-scale measurements of low anisotropic strain response of local $T_c$ in Sr$_2$RuO$_4$
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Strontium ruthenate (Sr$_2$RuO$_4$) is a multiband superconductor that displays evidence of topological superconductivity, although a model of the order parameter that is consistent with all experiments remains elusive. We integrated a piezoelectric-based strain apparatus with a scanning superconducting quantum interference device (SQUID) microscope to map the diamagnetic response of single-crystal Sr$_2$RuO$_4$ as a function of temperature, uniaxial pressure, and position with micron-scale spatial resolution. We thereby obtained local measurements of the superconducting transition temperature $T_c$ vs. anisotropic strain $epsilon$ with sufficient sensitivity for comparison to theoretical models that assume a uniform $p_xpm ip_y$ order parameter. We found that $T_c$ varies with position and that the locally measured $T_c$ vs. $epsilon$ curves are quadratic ($T_cproptoepsilon^2$), as allowed by the C$_4$ symmetry of the crystal lattice. We did not observe the low-strain linear cusp ($T_cpropto left| epsilon right|$) that would be expected for a two-component order parameter such as $p_xpm ip_y$. These results provide new input for models of the order parameter of Sr$_2$RuO$_4$.
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Sr$_2$RuO$_4$ is a leading candidate for chiral $p$-wave superconductivity. The detailed mechanism of superconductivity in this material is still the subject of intense investigations. Since superconductivity is sensitive to the topology of the Fermi surface (the contour of zero-energy quasi-particle excitations in the momentum space in the normal state), changing this topology can provide a strong test of theory. Recent experiments tuned the Fermi surface topology efficiently by applying planar anisotropic strain. Using functional renormalization group theory, we study the superconductivity and competing orders in Sr$_2$RuO$_4$ under strain. We find a rapid initial increase in the superconducting transition temperature $T_c$, which can be associated with the evolution of the Fermi surface toward a Lifshitz reconstruction under increasing strain. Before the Lifshitz reconstruction is reached, however, the system switches from the superconducting state to a spin density wave state. The theory agrees well with recent strain experiments showing an enhancement of $T_c$ followed by an intriguing sudden drop.
We analyze the spin anisotropy of the magnetic susceptibility of Sr$_2$RuO$4$ in presence of spin-orbit coupling and anisotropic strain using quasi-two-dimensional tight-binding parametrization fitted to the ARPES results. Similar to the previous observations we find the in-plane polarization of the low ${bf q}$ magnetic fluctuations and the out-of-plane polarization of the incommensurate magnetic fluctuation at the nesting wave vector ${bf Q}_1 = (2/3 pi ,2/3 pi)$ but also nearly isotropic fluctuations near ${bf Q}_2=(pi/6,pi/6)$. Furthermore, one finds that apart from the high-symmetry direction of the tetragonal Brillouin zone the magnetic anisotropy is maximal, i.e. $chi^{xx} eq chi^{yy} eq chi^{zz}$. This is the consequence of the orbital anisotropy of the $xz$ and $yz$ orbitals in the momentum space. We also study how the magnetic anisotropy evolves in the presence of the strain and find strong Ising-like ferromagnetic fluctuations near the Lifshitz transition for the $xy$-band.
Motivated by the success of experimental manipulation of the band structure through biaxial strain in Sr$_2$RuO$_4$ thin film grown on a mismatched substrate, we investigate theoretically the effects of biaxial strain on the electronic instabilities, such as superconductivity (SC) and spin density wave (SDW), by functional renormalization group. According to the experiment, the positive strain (from lattice expansion) causes charge transfer to the $gamma$-band and consequently Lifshitz reconstruction of the Fermi surface. Our theoretical calculations show that within a limited range of positive strain a p-wave superconducting order is realized. However, as the strain is increased further the system develops into the SDW state well before the Lifshitz transition is reached. We also consider the effect of negative strains (from lattice constriction). As the strain increases, there is a transition from p-wave SC state to nodal s-wave SC state. The theoretical results are discussed in comparison to experiment and can be checked by further experiments.
We present an implementation of the rotationally invariant slave boson technique as an impurity solver for density functional theory plus dynamical mean field theory (DFT+DMFT). Our approach provides explicit relations between quantities in the local correlated subspace treated with DMFT and the Bloch basis used to solve the DFT equations. In particular, we present an expression for the mass enhancement of the quasiparticle states in reciprocal space. We apply the method to the study of the electronic correlations in Sr$_2$RuO$_4$ under anisotropic strain. We find that the spin-orbit coupling plays a crucial role in the mass enhancement differentiation between the quasi-one-dimensional $alpha$ and $beta$ bands, and on its momentum dependence over the Fermi surface. The mass enhancement, however, is only weakly affected by either uniaxial or biaxial strain, even across the Lifshitz transition induced by the strain.
It is widely believed that the perovskite Sr$_2$RuO$_4$ is an unconventional superconductor with broken time reversal symmetry. It has been predicted that superconductors with broken time reversal symmetry should have spontaneously generated supercurrents at edges and domain walls. We have done careful imaging of the magnetic fields above Sr$_2$RuO$_4$ single crystals using scanning Hall bar and SQUID microscopies, and see no evidence for such spontaneously generated supercurrents. We use the results from our magnetic imaging to place upper limits on the spontaneously generated supercurrents at edges and domain walls as a function of domain size. For a single domain, this upper limit is below the predicted signal by two orders of magnitude. We speculate on the causes and implications of the lack of large spontaneous supercurrents in this very interesting superconducting system.
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