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Register a new userFormation of localized magnetic states in graphene in hollow-site adsorbed adatoms
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Sebastian Ardenghi JSA
Publication date
2018
fields
Physics
and research's language is
English
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By applying tight binding model of adatoms in graphene, we study theoretically the localized aspects of the interaction between transition metal atoms and graphene. Considering the electron-electron interaction by adding a Hubbard term in the mean-field approximation, we find the spin-polarized localized and total density of states. We obtain the coupled system of equations for the occupation number for each spin in the impurity and we study the fixed points of the solutions. By comparing the top site and hollow site adsorption, we show that the anomalous broadening of the latter allows to obtain magnetization for small values of the Hubbard parameter. Finally, we model the magnetic boundaries in order to obtain the range of Fermi energies at which magnetization starts.
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We examine the exchange Hamiltonian for magnetic adatoms in graphene with localized inner shell states. On symmetry grounds, we predict the existence of a class of orbitals that lead to a distinct class of quantum critical points in graphene, where the Kondo temperature scales as $T_{K}propto|J-J_{c}|^{1/3}$ near the critical coupling $J_{c}$, and the local spin is effectively screened by a emph{super-ohmic} bath. For this class, the RKKY interaction decays spatially with a fast power law $sim1/R^{7}$. Away from half filling, we show that the exchange coupling in graphene can be controlled across the quantum critical region by gating. We propose that the vicinity of the Kondo quantum critical point can be directly accessed with scanning tunneling probes and gating.
We examine theoretically the signatures of magnetic adatoms in graphene probed by scanning tunneling spectroscopy (STS). When the adatom hybridizes equally with the two graphene sublattices, the broadening of the local adatom level is anomalous and can scale with the cube of the energy. In contrast to ordinary metal surfaces, the adatom local moment can be suppressed by the proximity of the probing scanning tip. We propose that the dependence of the tunneling conductance on the distance between the tip and the adatom can provide a clear signature for the presence of local magnetic moments. We also show that tunneling conductance can distinguish whether the adatom is located on top of a carbon atom or in the center of a honeycomb hexagon.
It is generally believed that free-standing graphene does not demonstrate any ferroic properties. In the present work we revise this statement and show that single graphene sheet with a pair of magnetic adatoms can be driven into ferroelectric (FE) and multiferroic (MF) phases by tuning the Dirac cones slope. The transition into the FE phase occurs gradually, but an anomalous MF phase appears abruptly by means of a Quantum Phase Transition. Our findings suggest that such features should exist in graphene recently investigated by Scanning Tunneling Microscopy (Science 352, 437 (2016)).
In this paper, we describe the formation of local resonances in graphene in the presence of magnetic adatoms containing localized orbitals of arbitrary symmetry, corresponding to any given angular momentum state. We show that quantum interference effects which are naturally inbuilt in the honeycomb lattice in combination with the specific orbital symmetry of the localized state lead to the formation of fingerprints in differential conductance curves. In the presence of Jahn-Teller distortion effects, which lift the orbital degeneracy of the adatoms, the orbital symmetries can lead to distinctive signatures in the local density of states. We show that those effects allow scanning tunneling probes to characterize adatoms and defects in graphene.
Probing techniques with spatial resolution have the potential to lead to a better understanding of the microscopic physical processes and to novel routes for manipulating nanostructures. We present scanning-gate images of a graphene quantum dot which is coupled to source and drain via two constrictions. We image and locate conductance resonances of the quantum dot in the Coulomb-blockade regime as well as resonances of localized states in the constrictions in real space.
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